berry phase effects on electronic properties qian niu university of texas at austin collaborators:...
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Berry Phase Effects on Electronic Properties
Qian Niu
University of Texas at Austin
Collaborators:
D. Xiao, W. Yao, C.P. Chuu, D. Culcer, J.R.Shi, Y.G. Yao, G. Sundaram, M.C. Chang,
T. Jungwirth, A.H.MacDonald, J. Sinova, C.G.Zeng, H. Weitering
Supported by : DOE, NSF, Welch Foundation
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Outline
• Berry phase and its applications
• Anomalous velocity
• Anomalous density of states
• Graphene without inversion symmetry
• Nonabelian extension
• Polarization and Chern-Simons forms
• Conclusion
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tidti
nn
t
neett
0/
t
nnn id
0
Geometric phase:
In the adiabatic limit:
Berry Phase
1
2
0
t
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1 2 2 1
ii
21 ddn1
2
C
C
nnn id
Well defined for a closed path
Stokes theorem
Berry Curvature
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Berry curvature Magnetic field
Berry connection Vector potential
Geometric phase Aharonov-Bohm phase
Chern number Dirac monopole
Analogies
i
)(
)(rB
)( 2
did )( )( 2 rBrdrAdr
)(rA
integer)( 2
d ehBrd r /integer )( 2
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Applications
• Berry phaseinterference,
energy levels,
polarization in crystals
• Berry curvaturespin dynamics,
electron dynamics in Bloch bands
• Chern numberquantum Hall effect,
quantum charge pump
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Outline
• Berry phase and its applications
• Anomalous velocity
• Anomalous density of states
• Graphene without inversion symmetry
• Nonabelian extension
• Polarization and Chern-Simons forms
• Conclusion
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Anomalous Hall effect
• velocity
• distribution g( ) = f( ) + f( )
• current
Intrinsic
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Recent experiment Mn5Ge3 : Zeng, Yao, Niu & Weitering, PRL 2006
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Intrinsic AHE in other ferromagnets
• Semiconductors, MnxGa1-xAs– Jungwirth, Niu, MacDonald , PRL (2002)
• Oxides, SrRuO3
– Fang et al, Science , (2003).
• Transition metals, Fe
– Yao et al, PRL (2004)
– Wang et al, PRB (2006)
• Spinel, CuCr2Se4-xBrx
– Lee et al, Science, (2004)
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Outline
• Berry phase and its applications
• Anomalous velocity
• Anomalous density of states
• Graphene without inversion symmetry
• Nonabelian extension
• Polarization and Chern-Simons forms
• Conclusion
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Orbital magnetizationXiao et al, PRL 2005, 2006
Free energy:
Definition:
Our Formula:
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Anomalous Thermoelectric Transport
• Berry phase correction to magnetization
• Thermoelectric transport
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Anomalous Nernst Effectin CuCr2Se4-xBrx
Lee, et al, Science 2004; PRL 2004, Xiao et al, PRL 2006
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Outline
• Berry phase and its applications
• Anomalous velocity
• Anomalous density of states
• Graphene without inversion symmetry
• Nonabelian extension
• Polarization and Chern-Simons forms
• Conclusion
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Graphene without inversion symmetry
• Graphene on SiC: Dirac gap 0.28 eV • Energy bands
• Berry curvature
• Orbital moment
2 2 23 / 4q t q
em q q q
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2K1K
E2K1K
Valley Hall EffectValley Hall EffectAnd edge magnetizationAnd edge magnetization
R R1 2μ μL L
1 2μ μ
Left edge Right edge
Valley polarization induced on side edges Edge magnetization:
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Outline
• Berry phase and its applications
• Anomalous velocity
• Anomalous density of states
• Graphene without inversion symmetry
• Nonabelian extension
• Quantization of semiclassical dynamics
• Conclusion
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Degenerate bands
• Internal degree of freedom:
• Non-abelian Berry curvature:
• Useful for spin transport studies
Cucler, Yao & Niu, PRB, 2005Shindou & Imura, Nucl. Phys. B, 2005Chuu, Chang & Niu, 2006
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Outline
• Berry phase and its applications
• Anomalous velocity
• Anomalous density of states
• Graphene without inversion symmetry
• Nonabelian extension: spin transport
• Polarization and Chern-Simons forms
• Conclusion
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Electrical Polarization
• A basic materials property of dielectrics– To keep track of bound charges
– Order parameter of ferroelectricity
– Characterization of piezoelectric effects, etc.• A multiferroic problem: electric polarization
induced by inhomogeneous magnetic ordering
G. Lawes et al, PRL (2005)
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Thouless (1983): found adiabatic current in a crystal in terms of a Berry curvature in (k,t) space.
King-Smith and Vanderbilt (1993):
Led to great success in first principles calculations
Polarization as a Berry phase
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Inhomogeneous order parameter
• Make a local approximation and calculate Bloch states
• A perturbative correction to the KS-V formula
• A topological contribution (Chern-Simons)
|u>= |u(m,k)>, m = order parameter
Perturbation from the gradient
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ConclusionBerry phase
A unifying concept with many applications
Anomalous velocityHall effect from a ‘magnetic field’ in k space.
Anomalous density of statesBerry phase correction to orbital magnetization anomalous thermoelectric transport
Graphene without inversion symmetryvalley dependent orbital momentvalley Hall effect
Nonabelian extension for degenerate bands
Polarization and Chern-Simons forms