optimization of metallic magnetic calorimeters with...
TRANSCRIPT
Optimization of metallic magnetic calorimeters
with embedded 163Ho Loredana Gastaldo, Enss Christian, Fleischmann Andreas, Hassel Clemens, Hengstler Daniel, Hähnle Sebastian, Kempf Sebastian, Krantz Matthäus, Wegner Mathias Dorrer Holger, Düllmann Christoph, Eberhardt Klaus, Kieck Tom, Schneider Fabian, Wendt Klaus Köster Ulli Türler Andreas Marsh Bruce, Day Goodacre Tom, Johnston Karl, Rothe Sebastian, Stora Thierry, Veinhard Matthieu
163Ho and neutrino mass
n p p p n n
e-
e-
e-
e- n p p p n n n
e-
e-
p
eν
e-
e- e-
Atomic de-excitation: •X-ray emission •Auger electrons •Coster-Kronig transitions
A non- zero neutrino mass affects the de-excitation energy spectrum
Calorimetric measurement . . . . . . .
eν
C16366
*16366
e*163
6616367
DyDy
DyHo
E+→
+→ ν • τ1/2 ≅ 4570 years
• QEC = (2.555 ± 0.016) keV
(2*1011 atoms for 1 Bq)
M. Wang, G. Audi et al., Chinese Phys. C 36, 1603, (2012)
163Ho QEC-value
C16366
*16366
e*163
6616367
DyDy
DyHo
E+→
+→ ν • τ1/2 ≅ 4570 years
• QEC = (2.555 ± 0.016) keV
(2*1011 atoms for 1 Bq)
M. Wang, G. Audi et al., Chinese Phys. C 36, 1603, (2012)
Calorimetric measurements
Measurements of x-rays Gatti et al., 1997
ECHo, 2012
C16366
*16366
e*163
6616367
DyDy
DyHo
E+→
+→ ν • τ1/2 ≅ 4570 years
• QEC = (2.555 ± 0.016) keV
(2*1011 atoms for 1 Bq)
Penning Trap Mass Spectroscopy
Direct measurement of the mass difference of 163Ho and 163Dy as prerequisite to a determination of the electron neutrino mass S. Eliseev et al., Phys. Rev. Lett., in print (2015)
QEC = (2.833 ± 0.030stat ± 0.015syst) keV
M. Wang, G. Audi et al., Chinese Phys. C 36, 1603, (2012)
163Ho QEC-value
Calorimetric measurements
Measurements of x-rays Gatti et al., 1997
ECHo, 2012
C16366
*16366
e*163
6616367
DyDy
DyHo
E+→
+→ ν • τ1/2 ≅ 4570 years
• QEC = (2.555 ± 0.016) keV
(2*1011 atoms for 1 Bq)
Penning Trap Mass Spectroscopy
Direct measurement of the mass difference of 163Ho and 163Dy as prerequisite to a determination of the electron neutrino mass S. Eliseev et al., Phys. Rev. Lett., in print (2015)
QEC = (2.833 ± 0.030stat ± 0.015syst) keV
To reduce uncertainties in the analysis: QEC determination within 1 eV PENTATRAP (MPIK HD)
M. Wang, G. Audi et al., Chinese Phys. C 36, 1603, (2012)
163Ho QEC-value
Calorimetric measurements
Measurements of x-rays Gatti et al., 1997
ECHo, 2012
( )( )
( )( )
∑ Γ+−
Γ
−−−Α=
H2
H2HC
H
2H2
CEC
22
CECC
4
201
EE
BEQ
mEQ
dE
dWH
πϕν
MI MII
NI NII
OI OII
OI
QEC = 2.8 keV
163Ho QEC-value
Requirements for sub-eV sensitivity in ECHo
Statistics in the end point region • Nev > 1014 → A ≈ 1 MBq
Unresolved pile-up (fpu ~ a ⋅ τr) • fpu < 10-5 • τr < 1 µs a ~ 10 Bq • 105 pixels
Precision characterization of the endpoint region • ∆EFWHM < 3 eV
fpu = 10-5 ∆EFWHM = 3 eV
Statistics in the end point region • Nev > 1014 → A ≈ 1 MBq
Unresolved pile-up (fpu ~ a ⋅ τr) • fpu < 10-5 • τr < 1 µs a ~ 10 Bq • 105 pixels
Precision characterization of the endpoint region • ∆EFWHM < 3 eV
Low temperature
Metallic Magnetic Calorimeter
fpu = 10-5 ∆EFWHM = 3 eV
Requirements for sub-eV sensitivity in ECHo
∼ 1 %
Mea
sure
d en
ergy
E
[keV
]
Photon energy E [keV]
∆E [e
V]
MMCs: 1d-array for soft x-rays (T=20 mK)
Rise Time: 90 ns Non-Linearity < 1% @6keV
∆EFWHM = 1.6 eV @ 6 keV
250 µm
Reduction un-resolved pile-up
Definition of the energy scale
Reduced smearing in the end point region
Successful production and test of the first prototype
MMCs: Microwave SQUID multiplexing
Sebastian Kempf, talk on Tuesday
Meander
Source
Sensor
• Absorber for calorimetric measurement ion implantation @ ISOLDE-CERN in 2009 on-line process • About 0.01 Bq per pixel • Operated over more than 4 years
First detector prototype for 163Ho
L. Gastaldo et al., Nucl. Inst. Meth. A, 711 (2013) 150
P. C.-O. Ranitzsch et al., http://arxiv.org/abs/1409.0071v1
Absorber
• Rise Time ~ 130 ns • ∆EFWHM = 7.6 eV @ 6 keV (2013) • Non-Linearity < 1% @ 6keV • Synchronized measurement of 2 pixels
MII
MI
NII
NI
144Pm
OI
First calorimetric measurement of the OI-line
EH bind. EH exp. ΓH lit. ΓH exp
MI 2.047 2.040 13.2 13.7
MII 1.845 1.836 6.0 7.2
NI 0.420 0.411 5.4 5.3
NII 0.340 0.333 5.3 8.0
OI 0.050 0.048 5.0 4.3 P. C.-O. Ranitzsch et al ., http://arxiv.org/abs/1409.0071v1) L. Gastaldo et al., Nucl. Inst. Meth. A, 711, 150-159 (2013)
QEC = (2.843 ± 0.009stat - 0.06syst) keV
Calorimetric spectrum
MII
MI
NII
NI
144Pm
OI
Detector design and fabrication: • Increase activity per pixel • Stems between absorber and sensor
Understanding of the 163Ho spectrum: • Investigate undefined structures
High purity 163Ho source: • Background reduction
144Pm
Where to improve
NI
Requirement : >106 Bq >1017 atoms (n,γ)-reaction on 162Er
- High cross-section
- Radioactive contaminants Excellent chemical separation
Available 163Ho source:
~ 1018 atoms
Only 166mHo
: (n,γ)-reaction on 162Er High purity 163Ho source
ECHo requirements: 166mHo/ 163Ho < 10-9
Offline mass separation: RISIKO, Mainz University ISOLDE-CERN
Energy /keV
Coun
ts/c
hann
el
• Offline implantation @ISOLDE-CERN using GPS and RILIS • Chemically purified 163Ho source • maXs-20: - sandwich sensor design - absorber connected to sensor through stems - 16 pixels
Detector chip for second 163Ho implantation 250µm
0.
5 m
m
New detectors ready for … Mounted on a cold arm of a dry cryostat
Mounted on a cold arm of a dry cryostat
NI
OI MI
NII MII
preliminary
… first results NEW ( about 2 days)
… first results
MI
MII
NI
NII
OI
OLD (more then 1 month )
NI
OI MI
NII MII
preliminary
• Activity per pixel A ~ 0.2 Bq • Baseline resolution ∆EFWHM ~ 5 eV • Symmetric detector response • No strong evidence of radioactive contamination in the source
NEW ( about 2 days)
• Activity per pixel A ~ 0.2 Bq • Baseline resolution ∆EFWHM ~ 5 eV • Symmetric detector response • No strong evidence of radioactive contamination in the source
NI
OI MI
NII MII
preliminary
… first results
MI
MII
NI
NII
OI
NEW ( about 2 days)
Characterisation of spectral shape
MII
MI
NII
NI
144Pm
OI
Estimate the effect of • Higher order excitation in 163Dy • 163Ho ion embedded in Au
A. Faessler et al. J. Phys. G 42 (2015) 015108
R. G. H. Robertson Phys. Rev. C 91, 035504 (2015)
A. Faessler et al. Phys. Rev. C 91, 045505 (2015)
A. Faessler et al. Phys. Rev. C 91, 064302 (2015)
Characterisation of spectral shape
MII
MI
NII
NI
144Pm
OI
Estimate the effect of • Higher order excitation in 163Dy • 163Ho ion embedded in Au
Structures present also in new data
High purity 163Ho source has been produced
163Ho ions have been successfully implanted in offline process @ISOLDE-CERN
Conclusions and outlook
NI
OI MI
NII MII
preliminary
Prove scalability with medium large experiment ECHo-1K
• A ∼ 1000 Bq High purity 163Ho source (produced at reactor) • ∆EFWHM < 5 eV • τr< 1 µs • multiplexed arrays microwave SQUID multiplexing
• 1 year measuring time 1010 counts = Neutrino mass sensitivity mν < 10 eV Just approved Research Unit FOR 2202/1 „Neutrino Mass Determination by Electron Capture in Holmium-163 – ECHo“
ECHo-1M towards sub-eV sensitivity
Conclusions and outlook
Thank you! Department of Nuclear Physics, Comenius University, Bratislava, Slovakia Fedor Simkovic Department of Physics, Indian Institute of Technology Roorkee, India Moumita Maiti Goethe Universität Frankfurt am Main Udo Kebschull, Panagiotis Neroutsos Institute for Nuclear Chemistry, Johannes Gutenberg University Mainz Christoph E. Düllmann, Klaus Eberhardt, Holger Dorrer, Fabian Schneider Institute of Nuclear Research of the Hungarian Academy of Sciences Zoltán Szúcs Institute of Nuclear and Particle Physics, TU Dresden, Germany Kai Zuber Institute for Physics, Humboldt-Universität zu Berlin Alejandro Saenz Institute for Physics, Johannes Gutenberg-Universität Klaus Wendt, Sven Junck, Tom Kieck Institute for Theoretical and Experimental Physics Moscow, Russia Mikhail Krivoruchenko Institute for Theoretical Physics, University of Tübingen, Germany Amand Fäßler Institut Laue-Langevin, Grenoble, France Ulli Köster Kirchhoff-Institute for Physics, Heidelberg University, Germany Christian Enss, Loredana Gastaldo, Andreas Fleischmann, Clemens Hassel, Sebastian Kempf, Mathias Wegner Max-Planck Institute for Nuclear Physics Heidelberg, Germany Klaus Blaum, Andreas Dörr, Sergey Eliseev, Mikhail Goncharov, Yuri N. Novikov, Alexander Rischka, Rima Schüssler Petersburg Nuclear Physics Institute, Russia Yuri Novikov, Pavel Filianin Physics Institute, University of Tübingen, Germany Josef Jochum, Stephan Scholl Saha Institute of Nuclear Physics, Kolkata, India Susanta Lahiri
∆N
/N
6 10-13 above QEC-1eV
5 10-9 above QEC-20eV
163Ho and neutrino mass: sub-eV sensitivity
MI MII
NI NII
OI OII
OI
Statistics in the end point region • Nev > 1014 → A ≈ 1 MBq
QEC = 2.8 keV
163Ho and neutrino mass: sub-eV sensitivity
Statistics in the end point region • Nev > 1014 → A ≈ 1 MBq
Unresolved pile-up (fpu ~ a ⋅ τr) • fpu < 10-5 • τr < 1 µs a ~ 10 Bq • 105 pixels
3
2
1
0
1
3
2
1
0
1
3
2
1
0
1
∆t = 0.5 µs τr = 0.1 µs τr = 5 µs
163Ho and neutrino mass: sub-eV sensitivity
Statistics in the end point region • Nev > 1014 → A ≈ 1 MBq
Unresolved pile-up (fpu ~ a ⋅ τr) • fpu < 10-5 • τr < 1 µs a ~ 10 Bq • 105 pixels
Precision characterization of the endpoint region • ∆EFWHM < 2 eV
fpu = 10-5 ∆EFWHM = 3 eV
• Rise Time ~ 130 ns • ∆EFWHM = 7.6 eV @ 6 keV (2013) ∆EFWHM = 2.4 eV @ 0 keV (2014) • Non-Linearity < 1% @ 6keV
Calorimetric spectrum
IN OUT
Microwave SQUID Multiplexer for the Readout of Metallic Magnetic Calorimeters S.Kempf et al., J. Low. Temp. Phys. 175 (2014) 850-860
• Single HEMT amplifier and 2 coaxes to read out 100 - 1000 detectors
No events
Event in 3
MMCs: Microwave SQUID multiplexing
9.1
mm
15.5 mm
Elbow coupler MMC rf-SQUID
MMCs: Microwave SQUID multiplexing
Microwave SQUID Multiplexer for the Readout of Metallic Magnetic Calorimeters S.Kempf et al., J. Low. Temp. Phys. 175 (2014) 850-860
QEC determination of 163Ho
Penning Trap mass spectrometry
Precise measurement of the 163Ho and 163Dy atomic mass
2222zc νννν ++= −+
Talk by Klaus Blaum yesterday
QEC determination of 163Ho
Penning Trap mass spectrometry
First experiments at TRIGA-TRAP (Uni-Mainz) in 2014 * • Development of efficient Ho ion source using laser ablation • Uncertainties on 163Dy and 163Ho mass reduced by a factor of 2 • Know-how to be applied in SHIPTRAP
Presently: SHIPTRAP (GSI) • QEC determination with smaller uncertainties • Define scale of the experiment
*Preparatory studies for a high-precision Penning trap measurement of the 163Ho electron capture Q-value F. Schneider et al., submitted to EPJ
Magnetic sector-field Mass Spect. 30 kV two stage acceleration
60° double focussing separator magnet
Mass resolution: 𝑚𝛥𝑚
= 500 - 1000
Suppression of neighboring masses > 105
• Optimized resonant laser ionization for Ho efficiency larger than 24%
• Successful tests using 165Ho
Mass separation @ RISIKO
• off-line mass separator
( )( )
( )( )
∑ Γ+−
Γ
−−−Α=
H2
H2HC
H
2H2
CEC
22
CECC
4
201
EE
BEQ
mEQ
dE
dWH
πϕν
163Ho and neutrino mass
MI MII
NI NII
QEC = 2.555 keV
OI OII
OI
( )( )
( )( )
∑ Γ+−
Γ
−−−Α=
H2
H2HC
H
2H2
CEC
22
CECC
4
201
EE
BEQ
mEQ
dE
dWH
πϕν
MI MII
NI NII
OI OII
OI
163Ho and neutrino mass
QEC = 2.8 keV
Detector chip for second 163Ho implantation • Offline implantation @ISOLDE-CERN using GPS and RILIS • Chemically purified 163Ho source • maXs-20: - sandwich sensor design - absorber connected to sensor through stems Optimization of photo-lithographic processes
1.5 µm 5 µm
5 µm
AZ NLOF2070
Background Background sources:
• Environmental radioactivity Material screening
• Cosmic rays Underground labs
• Induced secondary radiation by cosmic rays μ-Veto
• Radioactivity in the detector
Study of background sources through:
• Monte Carlo simulations • Dedicated experiments
Underground measurements in Modane
Screening facilities • Uni-Tübingen • Felsenkeller
Separation at CERN/ISOLDE December 2014 • Off-line process • 2 new chips to test! … each with 16 pixel detector arrays
Mass separation @ISOLDE-CERN
Chemically purified 163Ho source in ISOLDE GPS mass separtion systems
Material constants • W, x: Crystal field parameters
• A: Hyperfine coupling strength
Thermodynamical properties of Au:Ho
Gold (fcc)
4f-Electrons (Ho)
• Magnetic moment of Ho3+ • Crystal field • Zeeman effect • Hyperfine interaction
J = 8 B I = 7/2
B
• Investigation of solid state effects • Determination of the maximum activity per pixel
• Magnetization „High-T“ measurement (2K – 300K)
− easy − no influence from Hyperfine interaction Determine W = -0.112
x = -0.357 • Heat capacity
Determine A
Deriving material constants from measurements
Thermodynamical properties of Au:Ho
Heat capacity measurement of Au:Ho
• 165Ho implanted in MMC absorbers • Acceleration voltage 30 kV • 3 chips • Number of ions per chip :
2*1011 / 2*1012 / 2*1013
(1Bq / 10Bq / 100Bq)
163Ho 165Ho
J 8 8
I 7/2 7/2
HoCC+C
E
T
M
+∂∂
∝abssens
S ΔΦ
Define the maximum activity per pixel
Gold atoms in implanted volume (160*160*0.01 µm3): ~ 1013
1 Bq 10 Bq 100 Bq
Dilute alloy High concentrated Ho layer Thin Ho layer
Heat capacity measurement
Gold atoms in implanted volume (160*160*0.01 µm3): ~ 1013
1 Bq 10 Bq 100 Bq
Dilute alloy High concentrated Ho layer Thin Ho layer
Ready to be measured
Heat capacity measurement