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Integrated assessment of enhanced weathering June 4th, 2015 Jessica Strefler, Nico Bauer, Thorben Amann, Elmar Kriegler, Jens Hartmann International Energy Workshop, Abu Dhabi

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Page 1: Integrated assessment of enhanced weathering 4_Jessica Strefler_WEB.pdf · Weathering ofsilicate rock consumesatmospheric CO 2 Fresh silicate rock + CO 2 + H 2 O clay + HCO 3-+ cations

Integrated assessment of enhanced weathering

June 4th, 2015

Jessica Strefler, Nico Bauer,Thorben Amann, Elmar Kriegler, Jens Hartmann

International Energy Workshop, Abu Dhabi

Page 2: Integrated assessment of enhanced weathering 4_Jessica Strefler_WEB.pdf · Weathering ofsilicate rock consumesatmospheric CO 2 Fresh silicate rock + CO 2 + H 2 O clay + HCO 3-+ cations

Outline1. Introduction

2. Preliminary considerations• Grain size• Limitations

3. Implementation

4. Model results• Standard implementation• Sensitivity analysis: grain size• Technological limitations: limited bioenergy, no CCS

5. Summary and Discussion

Page 3: Integrated assessment of enhanced weathering 4_Jessica Strefler_WEB.pdf · Weathering ofsilicate rock consumesatmospheric CO 2 Fresh silicate rock + CO 2 + H 2 O clay + HCO 3-+ cations

IntroductionWeathering of silicate rock consumes atmospheric CO2

Fresh silicate rock + CO2 + H2O clay + HCO3

- + cationsSlow process! Efficient on geological time scales to balance the atmospheric CO2 content

How can we enhance the natural process?• fast weathering minerals• small grain sizes (powder, flour)• warm and moist regions

Page 4: Integrated assessment of enhanced weathering 4_Jessica Strefler_WEB.pdf · Weathering ofsilicate rock consumesatmospheric CO 2 Fresh silicate rock + CO 2 + H 2 O clay + HCO 3-+ cations

Introduction

Mining of minerals

Grinding

Spreading on crop fields

Page 5: Integrated assessment of enhanced weathering 4_Jessica Strefler_WEB.pdf · Weathering ofsilicate rock consumesatmospheric CO 2 Fresh silicate rock + CO 2 + H 2 O clay + HCO 3-+ cations

Suitable application areas

100% cropland

50‐70% cropland

Warm, humidTemperate, humid

Warm, humid

Temperate, humid

Page 6: Integrated assessment of enhanced weathering 4_Jessica Strefler_WEB.pdf · Weathering ofsilicate rock consumesatmospheric CO 2 Fresh silicate rock + CO 2 + H 2 O clay + HCO 3-+ cations

Why enhanced weathering?IPCC AR5: negative emissions important for 2°target

4 options:1. Bioenergy + CCS (BECCS)2. Afforestation3. Direct air capture (DAC)4. Enhanced weathering of rocks (EW)

Problems of other options: • Pressure on land (BECCS, afforestation)• CCS not yet available (BECCS, DAC)

Page 7: Integrated assessment of enhanced weathering 4_Jessica Strefler_WEB.pdf · Weathering ofsilicate rock consumesatmospheric CO 2 Fresh silicate rock + CO 2 + H 2 O clay + HCO 3-+ cations

Side effects

Negative side effects:• Environmental costs of mining• Potential mobilization of trace metals

Positive side effects:• Increase of coastal zone water pH• Supply of nutrients

Basalt suitable for EW, application planned in India to fertilizesoil

Page 8: Integrated assessment of enhanced weathering 4_Jessica Strefler_WEB.pdf · Weathering ofsilicate rock consumesatmospheric CO 2 Fresh silicate rock + CO 2 + H 2 O clay + HCO 3-+ cations

Costs and RevenuesCosts• Mining, spreading: mass dependent (45‐75 $/ t CO2)• Grinding: 

‐ Energy demand  ~ . (x: grain size)‐ disproportional increase of capital costs for small grain size‐ capital + O&M costs: 6 $/ t CO2‐ electricity costs ~ 20 $/ t CO2 (dependent on grain size, electricity price)

Page 9: Integrated assessment of enhanced weathering 4_Jessica Strefler_WEB.pdf · Weathering ofsilicate rock consumesatmospheric CO 2 Fresh silicate rock + CO 2 + H 2 O clay + HCO 3-+ cations

Costs and RevenuesCosts• Mining, spreading: mass dependent (45‐75 $/ t CO2)• Grinding: 

‐ Energy demand  ~ . (x: grain size)‐ disproportional increase of capital costs for small grain size‐ capital + O&M costs: 6 $/ t CO2‐ electricity costs ~ 20 $/ t CO2 (dependent on grain size, electricity price)

Revenues• Amount of carbon removed x CO2 price• Weathering rate [%/yr] δ~ . (x: grain size)• Assumption: There is an upper limit to the mass per area• Weathering rate determines maximum potential of negative emissions

Page 10: Integrated assessment of enhanced weathering 4_Jessica Strefler_WEB.pdf · Weathering ofsilicate rock consumesatmospheric CO 2 Fresh silicate rock + CO 2 + H 2 O clay + HCO 3-+ cations

Is there an „optimal“ grain size?

no, the smaller the better

Page 11: Integrated assessment of enhanced weathering 4_Jessica Strefler_WEB.pdf · Weathering ofsilicate rock consumesatmospheric CO 2 Fresh silicate rock + CO 2 + H 2 O clay + HCO 3-+ cations

Limitations to grain size• Validity of functions

• Grain size vs. weathering rate, energy inputvalid down to about 2 µm (weathering rate ≈ 50%)

• Technical limitations• 10 µm close to current technical feasibility (weathering rate ≈ 9%) • Capital costs may increase disproportionally for grain sizes lower than

10‐20 µm

• Particulate matter pollution?• Water limitation? Amount of CO2 transported to material?

Explore with sensitivity analysis

Page 12: Integrated assessment of enhanced weathering 4_Jessica Strefler_WEB.pdf · Weathering ofsilicate rock consumesatmospheric CO 2 Fresh silicate rock + CO 2 + H 2 O clay + HCO 3-+ cations

Implementation• REMIND: energy‐economy model, perfect foresight, intertemporal 

optimization

• 11 world regions

• In each region: four grades• Warm or temperate climate• Continuous or fragmented crop fields

• Build up capacities for grinding; determine amount of ground stoneavailable for spreading in each time step

• Model will start using EW when carbon price is high enough to cover costs

Page 13: Integrated assessment of enhanced weathering 4_Jessica Strefler_WEB.pdf · Weathering ofsilicate rock consumesatmospheric CO 2 Fresh silicate rock + CO 2 + H 2 O clay + HCO 3-+ cations

Enhanced weathering as a mitigation option

• When and to which extent deployed?

• Interaction with energy system?• Energy demand• Negative CO2 emissions

• Interaction with other mitigation options?• Especially other carbon dioxide removal technologies as

bioenergy + CCS, afforestation, direct air capturecomplements or substitutes?

Page 14: Integrated assessment of enhanced weathering 4_Jessica Strefler_WEB.pdf · Weathering ofsilicate rock consumesatmospheric CO 2 Fresh silicate rock + CO 2 + H 2 O clay + HCO 3-+ cations

Outline• Introduction

• Preliminary considerations• Optimal grain size• Limitations

• Implementation

• Model results• Standard implementation• Sensitivity analysis: grain size• Technological limitations: limited bioenergy, no CCS

• Summary and Discussion

Page 15: Integrated assessment of enhanced weathering 4_Jessica Strefler_WEB.pdf · Weathering ofsilicate rock consumesatmospheric CO 2 Fresh silicate rock + CO 2 + H 2 O clay + HCO 3-+ cations

Negative Emissions from EW

Page 16: Integrated assessment of enhanced weathering 4_Jessica Strefler_WEB.pdf · Weathering ofsilicate rock consumesatmospheric CO 2 Fresh silicate rock + CO 2 + H 2 O clay + HCO 3-+ cations

Fossil fuel emissions

Page 17: Integrated assessment of enhanced weathering 4_Jessica Strefler_WEB.pdf · Weathering ofsilicate rock consumesatmospheric CO 2 Fresh silicate rock + CO 2 + H 2 O clay + HCO 3-+ cations

Total CO2 emissions

Page 18: Integrated assessment of enhanced weathering 4_Jessica Strefler_WEB.pdf · Weathering ofsilicate rock consumesatmospheric CO 2 Fresh silicate rock + CO 2 + H 2 O clay + HCO 3-+ cations

Radiative forcing

Page 19: Integrated assessment of enhanced weathering 4_Jessica Strefler_WEB.pdf · Weathering ofsilicate rock consumesatmospheric CO 2 Fresh silicate rock + CO 2 + H 2 O clay + HCO 3-+ cations

Carbon price in 2020

Page 20: Integrated assessment of enhanced weathering 4_Jessica Strefler_WEB.pdf · Weathering ofsilicate rock consumesatmospheric CO 2 Fresh silicate rock + CO 2 + H 2 O clay + HCO 3-+ cations

Primary energy mix

Without EW With EW

Page 21: Integrated assessment of enhanced weathering 4_Jessica Strefler_WEB.pdf · Weathering ofsilicate rock consumesatmospheric CO 2 Fresh silicate rock + CO 2 + H 2 O clay + HCO 3-+ cations

Scenarios

Limitations Grain size[µm]

Weathering rate [% / yr]

Lower limit for validitiy ofrelations between grain size, weathering rate, energy input

2 50

6 20

Current limit of technicalfeasibility?

10 14

Capital costs may increasedisproportionately

20 10

Technically already feasible 50 5

Page 22: Integrated assessment of enhanced weathering 4_Jessica Strefler_WEB.pdf · Weathering ofsilicate rock consumesatmospheric CO 2 Fresh silicate rock + CO 2 + H 2 O clay + HCO 3-+ cations

Negative emissions

Page 23: Integrated assessment of enhanced weathering 4_Jessica Strefler_WEB.pdf · Weathering ofsilicate rock consumesatmospheric CO 2 Fresh silicate rock + CO 2 + H 2 O clay + HCO 3-+ cations

Fossil fuel emissions

Page 24: Integrated assessment of enhanced weathering 4_Jessica Strefler_WEB.pdf · Weathering ofsilicate rock consumesatmospheric CO 2 Fresh silicate rock + CO 2 + H 2 O clay + HCO 3-+ cations

Total CO2 emissions

Page 25: Integrated assessment of enhanced weathering 4_Jessica Strefler_WEB.pdf · Weathering ofsilicate rock consumesatmospheric CO 2 Fresh silicate rock + CO 2 + H 2 O clay + HCO 3-+ cations

Radiative forcing

Page 26: Integrated assessment of enhanced weathering 4_Jessica Strefler_WEB.pdf · Weathering ofsilicate rock consumesatmospheric CO 2 Fresh silicate rock + CO 2 + H 2 O clay + HCO 3-+ cations

Change of carbon pools until 2100

Page 27: Integrated assessment of enhanced weathering 4_Jessica Strefler_WEB.pdf · Weathering ofsilicate rock consumesatmospheric CO 2 Fresh silicate rock + CO 2 + H 2 O clay + HCO 3-+ cations

Carbon price in 2020

Page 28: Integrated assessment of enhanced weathering 4_Jessica Strefler_WEB.pdf · Weathering ofsilicate rock consumesatmospheric CO 2 Fresh silicate rock + CO 2 + H 2 O clay + HCO 3-+ cations

Negative emissions

Page 29: Integrated assessment of enhanced weathering 4_Jessica Strefler_WEB.pdf · Weathering ofsilicate rock consumesatmospheric CO 2 Fresh silicate rock + CO 2 + H 2 O clay + HCO 3-+ cations

Carbon price in 2020

25 $/t CO2    ≈ 40%

14.6 $/t CO2 ≈ 34 %

4.75 $/t CO2 ≈ 20%

Page 30: Integrated assessment of enhanced weathering 4_Jessica Strefler_WEB.pdf · Weathering ofsilicate rock consumesatmospheric CO 2 Fresh silicate rock + CO 2 + H 2 O clay + HCO 3-+ cations

SummaryGrain size• Smaller grain size lead to higher profits per area• Smaller grain size leads to higher potential• Limited by technical feasibility, disproportionate cost increase

Integrated Assessment• Availability of EW reduces carbon price – partial substitute to

other mitigation measures• EW especially valuable if bioenergy is limited or CCS is not 

available

Page 31: Integrated assessment of enhanced weathering 4_Jessica Strefler_WEB.pdf · Weathering ofsilicate rock consumesatmospheric CO 2 Fresh silicate rock + CO 2 + H 2 O clay + HCO 3-+ cations

Thank you!

Page 32: Integrated assessment of enhanced weathering 4_Jessica Strefler_WEB.pdf · Weathering ofsilicate rock consumesatmospheric CO 2 Fresh silicate rock + CO 2 + H 2 O clay + HCO 3-+ cations
Page 33: Integrated assessment of enhanced weathering 4_Jessica Strefler_WEB.pdf · Weathering ofsilicate rock consumesatmospheric CO 2 Fresh silicate rock + CO 2 + H 2 O clay + HCO 3-+ cations

Carbon removal rate vs. Energy input

y = 42.887x0.7857

R² = 0.9994

y = 4.8572x0.8131

R² = 1

y = 0.4916x0.8158

R² = 1

0.001

0.01

0.1

1

10

100

0.001 0.01 0.1 1 10

% d

isso

lved

afte

r one

yea

r

grinding energy demand (GJ/t)

olivine WR1/10th speed1/100th speedLinear (olivine WR)

grinding energy demand

% dissolvedafter o

neyear

Page 34: Integrated assessment of enhanced weathering 4_Jessica Strefler_WEB.pdf · Weathering ofsilicate rock consumesatmospheric CO 2 Fresh silicate rock + CO 2 + H 2 O clay + HCO 3-+ cations

Temperature

Page 35: Integrated assessment of enhanced weathering 4_Jessica Strefler_WEB.pdf · Weathering ofsilicate rock consumesatmospheric CO 2 Fresh silicate rock + CO 2 + H 2 O clay + HCO 3-+ cations

Primary energy mix – no EW

Page 36: Integrated assessment of enhanced weathering 4_Jessica Strefler_WEB.pdf · Weathering ofsilicate rock consumesatmospheric CO 2 Fresh silicate rock + CO 2 + H 2 O clay + HCO 3-+ cations

Primary energy mix – with EW