cross-sections of neutron threshold reactions studied by activation method
DESCRIPTION
Nuclear Physics Institute, Academy of Sciences of Czech Republic Department of Nuclear Reactors, Faculty of Nuclear Sciences and Physical Engineering, Czech Technical University in Prague. Cross-sections of Neutron Threshold Reactions studied by activation method. Diploma Thesis - PowerPoint PPT PresentationTRANSCRIPT
Cross-sections of Neutron Threshold Reactions studied
by activation method
Diploma ThesisVrzalová Jitka
Supervisor: RNDr. Vladimír Wagner, CSc.
Nuclear Physics Institute, Academy of Sciences of Czech RepublicDepartment of Nuclear Reactors, Faculty of Nuclear Sciences and Physical Engineering, Czech Technical University in Prague
2
Outline- Motivation
- Cross - section measurements
- Neutron sources
-Experiments-Řež
- Experiments- Uppsala
- Comparison Řež, Uppsala
- Conclusion
Motivation Nuclear data libraries Stochastic and deterministic codes Neutron sources Cross-section measurements Experiments on Cyclotron in Řež TSL Uppsala experiments Comparison Conclusion
3
Motivation for testing of the programs simulating ADS, it is
necessary to determine neutron fields
the neutron fields can be determined using the activation detectors
for neutron detection are used threshold reactions on Au, Al, Bi, In, Ta, Ni, Zn, Y, I
almost no experimental cross-section data for most of observed threshold reactions are available for higher neutron energies (E>20MeV)→it is necessary to perform new cross-section measurements
- Motivation• Introduction• Libraries• Stochastic and deterministic codes• Detection of neutrons• Evaluation
- Cross - section measurements
- Neutron sources
-Experiments-Řež
- Experiments- Uppsala
- Comparison Řež, Uppsala
- Conclusion
4
Evaluated nuclear data libraries x EXFOR
nuclear data are summarized in the libraries of nuclear data and gradually updated
data form ENDF-6
general libraries (BROND-russian, CENDL-chinese, ENDF-american, JEFF- european, JENDL-japanese)
specialized libraries (MENDL, WIND, LA 100, LA 150, NRG-2003)
cross-sections are for the major part of measured isotopes published up to (n,4n) reaction (100 MeV) in ENDF, in EXFOR up to 40 MeV
- Motivation• Introduction• Libraries• Stochastic and deterministic codes• Detection of neutrons• Evaluation
- Cross - section measurements
- Neutron sources
-Experiments-Řež
- Experiments- Uppsala
- Comparison Řež, Uppsala
- Conclusion
5
Stochastic codesMCNP a MCNPX MCNP simulates transport of neutrons (photons and
electrons) in energy range from 10-11 MeV to 20 MeV
MCNPX-connects and improves possibilities of MCNP, which is intended for lower energies and code LAHET, which is advisable for simulation of spallation reaction
LAHET simulates spallation reaction and transport nucleons,
pions, muons with energy E≥20 MeV
More Monte Carlo-based codes: FLUKA, HETC, NUCLEUS, SHIELD, NMTC, GEM, JAM
- Motivation• Introduction• Libraries• Stochastic and deterministic codes• Detection of neutrons• Evaluation
- Cross - section measurements
- Neutron sources
-Experiments-Řež
- Experiments- Uppsala
- Comparison Řež, Uppsala
- Conclusion
6
Deterministic codesTALYS 1.0 deterministic code
provides complete calculation of the nuclear reactions in the energy range from 1 keV to 200 MeV
with TALYS code can be obtained the complete
overview of cross-sections
the output file contains all usually demanded information, more than 200 keywords could be used in the input file
More codes: GNASH, ALICE, STAPRE, EMPIRE, MEND
- Motivation• Introduction• Libraries• Stochastic and deterministic codes• Detection of neutrons• Evaluation
- Cross - section measurements
- Neutron sources
-Experiments-Řež
- Experiments- Uppsala
- Comparison Řež, Uppsala
- Conclusion
7
TALYS 1.0 – nuclear models
- Motivation• Introduction• Libraries• Stochastic and deterministic codes• Detection of neutrons• Evaluation
- Cross - section measurements
- Neutron sources
-Experiments-Řež
- Experiments- Uppsala
- Comparison Řež, Uppsala
- Conclusion
Bi-207
0
0,2
0,4
0,6
0,8
1
1,2
1,4
1,6
1,8
2
15 20 25 30 35 40
E [MeV]
XS
[ba
rn]
ld1 ld2 ld3 ld4 ld5 EXFOR MENDL-2
8
TALYS 1.0 – nuclear models- Motivation• Introduction• Libraries• Stochastic and deterministic codes• Detection of neutrons• Evaluation
- Cross - section measurements
- Neutron sources
-Experiments-Řež
- Experiments- Uppsala
- Comparison Řež, Uppsala
- Conclusion
Bi-207
-60
-40
-20
0
20
40
60
80
15 20 25 30 35
E [MeV]
odch
ylka
[%
]ld2 ld3 ld4 ld5
Difference between cross-sections models with different nuclear level density and default Fermi model, reaction 209Bi(n,3n)207Bi
9
Detection of neutrons
- Motivation• Introduction• Libraries• Stochastic and deterministic codes• Detection of neutrons• Evaluation
- Cross - section measurements
- Neutron sources
-Experiments-Řež
- Experiments- Uppsala
- Comparison Řež, Uppsala
- Conclusion
Al Au Bi Co In Ta
ReactionE thresh [MeV]
Half-life
197Au (n,2n) 196Au 8.1 6.183 d197Au (n,3n) 195Au 14.8 186.1 d197Au (n,4n) 194Au 23.2 38.02 h
209Bi (n,3n) 207Bi 14.42 31.56 y209Bi (n,4n) 206Bi 22.55 6.243 d
115In (n,2n) 114In 9.12 1.2 min
10
Evaluation- Motivation• Introduction• Libraries• Stochastic and deterministic codes• Detection of neutrons• Evaluation
- Cross - section measurements
- Neutron sources
-Experiments-Řež
- Experiments- Uppsala
- Comparison Řež, Uppsala
- Conclusion
)()(
)(
11
1
)(
0
irrreal tirr
t
t
foillive
real
areaP
irrabspyield e
t
e
e
mt
t
CCoiEI
CCSN
• decay during cooling, irradiation
• unstable irradiation
• coincidences
• non point-like emitters
• detector dead time
• detector efficiency
• self-absorption
11
Cross-section measurements
- Motivation• Introduction• Libraries• Stochastic and deterministic codes• Detection of neutrons• Evaluation
- Cross - section measurements
- Neutron sources
-Experiments-Řež
- Experiments- Uppsala
- Comparison Řež, Uppsala
- Conclusion
Requirements for -measurements by activation method:
high energy neutron source with good intensity
monoenergetic (quasi-monoenergetic) neutrons or well known spectrum
pure monoisotopic samples
good spectroscopic equipment – and X-rays detectors
Then we can calculate Nyield and finally :An
yield
NN
ASN
Evaluation process:
Irradiation→HPGe→Deimos→Corrections→Yield→Cross-section
Number of neutrons in peak
12
- Motivation• Introduction• Libraries• Stochastic and deterministic codes• Detection of neutrons• Evaluation
- Cross - section measurements
- Neutron sources
-Experiments-Řež
- Experiments- Uppsala
- Comparison Řež, Uppsala
- Conclusion
Neutron sources source with wide spectrum of neutrons-time of flight method-determination energy of neutrons (system n_TOF in CERN), unsuitable for activation foils
quasi-monoenergetic neutron source - target + accelerator of particles - high-frequency source 7Li(p,n)7Be, 2H(d,n)3He
source CYRIC with energy range from 40 to 90 MeV in „Cyclotron and Radioisotope Center“ in Tohok
new source SPIRAL-2 is under construction in laboratory GANIL in Caen (France) (energy range to 40 MeV, high intensity)
13
- Motivation• Introduction• Libraries• Stochastic and deterministic codes• Detection of neutrons• Evaluation
- Cross - section measurements
- Neutron sources
-Experiments-Řež
- Experiments- Uppsala
- Comparison Řež, Uppsala
- Conclusion
Neutron sources
Neutron source on cyclotron U-120M
Blue Hall, UppsalaQuasi-monoenergetic neutron source
14
- Motivation• Introduction• Libraries• Stochastic and deterministic codes• Detection of neutrons• Evaluation
- Cross - section measurements
- Neutron sources
-Experiments-Řež
- Experiments- Uppsala
- Comparison Řež, Uppsala
- Conclusion
Experiments in Řež April, May 2009,
irradiation of the foils on cyclotron U-120M
quasi-monoenergetic neutron source based on reaction 7Li(p,n)7Be, energy range of this neutron source is 10-37 MeV
proton beam energies 32.5 and 37 MeV
irradiation time about 20 h.,irradiated foils: Ni, Zn, Bi, Cu, In, Al, Au, Ta, Fe and I
15
- Motivation• Introduction• Libraries• Stochastic and deterministic codes• Detection of neutrons• Evaluation
- Cross - section measurements
- Neutron sources
-Experiments-Řež
- Experiments- Uppsala
- Comparison Řež, Uppsala
- Conclusion
Experiments in Řež
16
- Motivation• Introduction• Libraries• Stochastic and deterministic codes• Detection of neutrons• Evaluation
- Cross - section measurements
- Neutron sources
-Experiments-Řež
- Experiments- Uppsala
- Comparison Řež, Uppsala
- Conclusion
Experiments in Uppsala February 2010, June
2008
quasi-monoenergetic neutron source based on reaction 7Li(p,n)7Be, energy range of this neutron source is 11-175 MeV
proton beam energies 25, 50, 100 MeV (June 2008); 62, 70, 80, and 93 MeV (February 2010)
irradiation time about 8 h.,irradiated foils: Au, Bi, In, Al, Ta, Co, Y and I
17
- Motivation• Introduction• Libraries• Stochastic and deterministic codes• Detection of neutrons• Evaluation
- Cross - section measurements
- Neutron sources -Experiments-Řež
- Experiments- Uppsala
- Comparison Řež, Uppsala
- Conclusion
Experiments in Uppsala
samples for irradiation
HPGe detector
placing samples toward detector
18
- Motivation• Introduction• Libraries• Stochastic and deterministic codes• Detection of neutrons• Evaluation
- Cross - section measurements
- Neutron sources
-Experiments-Řež
- Experiments- Uppsala
- Comparison Řež, Uppsala
- Conclusion
Comparison Řež, Uppsala
Řež
Uppsala
Au-196
0
0,5
1
1,5
2
2,5
3
0 10 20 30 40 50 60 70 80 90E [MeV]
XS
[ba
rn]
EXFOR TALYS ÚJF Řež TSL Uppsala
Comparison of cross-section reaction (n,2n) 197Au with EXFOR and TALYS
Řež
Uppsala
19
- Motivation• Introduction• Libraries• Stochastic and deterministic codes• Detection of neutrons• Evaluation
- Cross - section measurements
- Neutron sources
-Experiments-Řež
- Experiments- Uppsala
- Comparison Řež, Uppsala
- Conclusion
Comparison Řež, Uppsala
Řež
Uppsala
Uppsala
In-114m
0
0,3
0,6
0,9
1,2
1,5
1,8
8 18 28 38 48 58 68 78 88 98
E [MeV]
XS
[ba
rn]
EXFOR TALYS ÚJF Řež TSL Uppsala
Comparison of cross-section reaction (n,xn) natIn with EXFOR and TALYS
Řež
Uppsala
20
- Motivation• Introduction• Libraries• Stochastic and deterministic codes• Detection of neutrons• Evaluation
- Cross - section measurements
- Neutron sources
-Experiments-Řež
- Experiments- Uppsala
- Comparison Řež, Uppsala
- Conclusion
Comparison Řež, Uppsala
Řež
Uppsala
Uppsala
Comparison of cross-section reaction (n,2n) 64Zn with EXFOR and TALYS
Zn-63
0
0,05
0,1
0,15
0,2
0,25
0,3
0,35
0,4
0,45
0,5
12 17 22 27 32 37
E [MeV]
XS
[b
arn
]TALYS ÚJF Řež EXFOR, Y. Uwamino, 1992 EXFOR, A.A.Lapenas, 1975
Řež
21
- Motivation• Introduction• Libraries• Stochastic and deterministic codes• Detection of neutrons• Evaluation
- Cross - section measurements
- Neutron sources
-Experiments-Řež
- Experiments- Uppsala
- Comparison Řež, Uppsala
- Conclusion
Conclusion Our cross-section measurements in Uppsala and Řež
cover wide spectrum of energies
Our results for well known cross-sections agree with
other experimental data
We measured also a lot of new experimental data
Near future: publish the measured cross-sections from
Uppsala at February 2010
Thanks for attention