the university of reading helen dacre agu dec 2008 boundary layer ventilation by convection and...

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The University of Reading Helen Dacre AGU Dec 2008 Boundary Layer Ventilation by Convection and Coastal Processes Helen Dacre, Sue Gray, Stephen Belcher Didcot power station, Oxfordshire

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Page 1: The University of Reading Helen Dacre AGU Dec 2008 Boundary Layer Ventilation by Convection and Coastal Processes Helen Dacre, Sue Gray, Stephen Belcher

The University of Reading Helen Dacre AGU Dec 2008

Boundary Layer Ventilation by Convection and Coastal Processes

Helen Dacre, Sue Gray, Stephen Belcher

Didcot power station, Oxfordshire

Page 2: The University of Reading Helen Dacre AGU Dec 2008 Boundary Layer Ventilation by Convection and Coastal Processes Helen Dacre, Sue Gray, Stephen Belcher

The University of Reading Helen Dacre AGU Dec 2008

Motivation

Boundary layer ~1km

Advection ?Convection ?

Mixing ?

Page 3: The University of Reading Helen Dacre AGU Dec 2008 Boundary Layer Ventilation by Convection and Coastal Processes Helen Dacre, Sue Gray, Stephen Belcher

The University of Reading Helen Dacre AGU Dec 2008

Talk Outline

• Modelling Experiment

• Case study – May 9th 2005– Results from modelling experiments– Comparison with observations– Ventilation estimate

• Conclusions

• Future Work

Page 4: The University of Reading Helen Dacre AGU Dec 2008 Boundary Layer Ventilation by Convection and Coastal Processes Helen Dacre, Sue Gray, Stephen Belcher

The University of Reading Helen Dacre AGU Dec 2008

Experimental Setup• Met Office Unified Model• Limited area domain over Europe, ∆x≈12km, ∆z≈100m in

boundary layer, 500m in mid-troposphere • Parameterized convection and boundary layer turbulent

mixing

• Pollution sources represented by constant emission of tracers over land emitted 20m above the surface

• Different ventilation mechanisms represented by advection, convection and turbulent mixing schemes

• Tracers transported by different combinations of transport schemes

Page 5: The University of Reading Helen Dacre AGU Dec 2008 Boundary Layer Ventilation by Convection and Coastal Processes Helen Dacre, Sue Gray, Stephen Belcher

The University of Reading Helen Dacre AGU Dec 2008

May 2005 Case Study OverviewUK Met Office surface pressure analysis 00UTC

Nimrod radar composite 13:00 UTC

Modis Aqua visible 12:45 UTC

Page 6: The University of Reading Helen Dacre AGU Dec 2008 Boundary Layer Ventilation by Convection and Coastal Processes Helen Dacre, Sue Gray, Stephen Belcher

The University of Reading Helen Dacre AGU Dec 2008

Advection

Tracer in free troposphere integrated over height

17 UTC

coastland sea

09 UTC

13 UTC

17 UTC

kg/m

2

wind direction

wind direction

Page 7: The University of Reading Helen Dacre AGU Dec 2008 Boundary Layer Ventilation by Convection and Coastal Processes Helen Dacre, Sue Gray, Stephen Belcher

The University of Reading Helen Dacre AGU Dec 2008

Advection and Mixing

Tracer in free troposphere integrated over height

17 UTC

coastland sea

09 UTC

13 UTC

17 UTCkg

/m2

Page 8: The University of Reading Helen Dacre AGU Dec 2008 Boundary Layer Ventilation by Convection and Coastal Processes Helen Dacre, Sue Gray, Stephen Belcher

The University of Reading Helen Dacre AGU Dec 2008

Advection, Mixing and Convection

09 UTC

13 UTC

17 UTC

land coast sea

kg/m

2

Tracer in free troposphere integrated over height

17 UTC

Page 9: The University of Reading Helen Dacre AGU Dec 2008 Boundary Layer Ventilation by Convection and Coastal Processes Helen Dacre, Sue Gray, Stephen Belcher

The University of Reading Helen Dacre AGU Dec 2008

AMPEP Observations

Downwind air measurements(mass flux of pollution coming off UK)

Upwind air measurements (background concentrations)

• Direct measurements of the mass budgets of pollutants in the boundary layer over the UK

(Aircraft Measurements of chemical Processing and Export fluxes of Pollutants)

Page 10: The University of Reading Helen Dacre AGU Dec 2008 Boundary Layer Ventilation by Convection and Coastal Processes Helen Dacre, Sue Gray, Stephen Belcher

The University of Reading Helen Dacre AGU Dec 2008

AMPEP flight

AMPEP flight path AMPEP flight height

IG

D

wind direction

Page 11: The University of Reading Helen Dacre AGU Dec 2008 Boundary Layer Ventilation by Convection and Coastal Processes Helen Dacre, Sue Gray, Stephen Belcher

The University of Reading Helen Dacre AGU Dec 2008

Boundary layer profile in central England

AMPEP CO profileModel tracer profile

17:24 UTC

boundary layer top

background concentration

Page 12: The University of Reading Helen Dacre AGU Dec 2008 Boundary Layer Ventilation by Convection and Coastal Processes Helen Dacre, Sue Gray, Stephen Belcher

The University of Reading Helen Dacre AGU Dec 2008

Polluted profile in English Channel

AMPEP CO profileModel tracer profile

15:34 UTC

elevated pollution

Page 13: The University of Reading Helen Dacre AGU Dec 2008 Boundary Layer Ventilation by Convection and Coastal Processes Helen Dacre, Sue Gray, Stephen Belcher

The University of Reading Helen Dacre AGU Dec 2008

Quantifying Ventilation

? ?

?

Page 14: The University of Reading Helen Dacre AGU Dec 2008 Boundary Layer Ventilation by Convection and Coastal Processes Helen Dacre, Sue Gray, Stephen Belcher

The University of Reading Helen Dacre AGU Dec 2008

Quantifying Ventilation

Percentage of tracer in free troposphere

Percentage of tracer above 2km

52%

26%

sunrise sunsetsunrisesunset

% o

f tr

acer

in f

ree

trop

osph

ere

% o

f tr

acer

abo

ve 2

km

Time of day (hours) Time of day (hours)

advadv + mixadv, mix + conv

Page 15: The University of Reading Helen Dacre AGU Dec 2008 Boundary Layer Ventilation by Convection and Coastal Processes Helen Dacre, Sue Gray, Stephen Belcher

The University of Reading Helen Dacre AGU Dec 2008

Case Study Summary

Transport process

Ventilation

AdvectionLarge-scale ascent transported pollution up to 3km

Coastal venting enhanced by sea-breeze → layer of polluted air over clean air along coast

ConvectionWidespread convection → layer of polluted air in mid-troposphere over whole of the UK

Turbulent mixingTurbulence mixes pollution within boundary layer → increases ventilation by large-scale ascent

Page 16: The University of Reading Helen Dacre AGU Dec 2008 Boundary Layer Ventilation by Convection and Coastal Processes Helen Dacre, Sue Gray, Stephen Belcher

The University of Reading Helen Dacre AGU Dec 2008

Conclusions• NWP model output is a useful tool and can complement

observational results in studying transport processes

• Assumption that ventilation of the boundary layer is negligible during non-frontal events is not always valid– Convection can transport polluted air out of bl and

form a distinct layer in the free troposphere– Coastal outflow can transport pollution above the

marine boundary layer– Sea-breeze can enhance coastal outflow and create

a layer of polluted air above a layer of clean air along the coast

• Turbulent mixing and convection can double the amount of pollution ventilated from the boundary layer

Page 17: The University of Reading Helen Dacre AGU Dec 2008 Boundary Layer Ventilation by Convection and Coastal Processes Helen Dacre, Sue Gray, Stephen Belcher

The University of Reading Helen Dacre AGU Dec 2008

Further Work• How sensitive are model simulations of the distribution of

pollutants to the representation of convective transport?

• How well is the sea-breeze represented at 12km resolution?

• Are Meteorological models suitable for chemical dispersion studies?

• What are the relative importance of these ventilation processes on pollution distribution on longer timescales?

ReferenceH.F.Dacre, S.L.Gray and S.E.Belcher (2007), A case study of boundary layer

ventilation by convection and coastal processes, J. Geophys. Res., 12, D17106, doi:10.1029/2006JD007984

Page 18: The University of Reading Helen Dacre AGU Dec 2008 Boundary Layer Ventilation by Convection and Coastal Processes Helen Dacre, Sue Gray, Stephen Belcher

The University of Reading Helen Dacre AGU Dec 2008

Schematic of boundary layer ventilation for 9th May 2005

Page 19: The University of Reading Helen Dacre AGU Dec 2008 Boundary Layer Ventilation by Convection and Coastal Processes Helen Dacre, Sue Gray, Stephen Belcher

The University of Reading Helen Dacre AGU Dec 2008

15 UTC over sea

11 UTC over land

Advection• Cross-sections of

potential temperature• Bold contours indicate

inversions• Dashed line indicates

boundary layer top

09 UTC

13 UTC land coast seaHei

ght a

bove

sur

face

(m

)

coast

Page 20: The University of Reading Helen Dacre AGU Dec 2008 Boundary Layer Ventilation by Convection and Coastal Processes Helen Dacre, Sue Gray, Stephen Belcher

The University of Reading Helen Dacre AGU Dec 2008

Introduction

• The dynamical processes that transport pollution within and above urban areas span a large range of spatial and temporal scales

100m10m

200m

Street scaleNeighbourhood scale

2km

City scale

20km

Regional scale

200km

1km10km

Page 21: The University of Reading Helen Dacre AGU Dec 2008 Boundary Layer Ventilation by Convection and Coastal Processes Helen Dacre, Sue Gray, Stephen Belcher

The University of Reading Helen Dacre AGU Dec 2008

Introduction• There are many transport processes responsible for the

ventilation of pollution from the boundary layer into the free troposphere