superconducting mechanisms of iron-based and cuprate superconductorsnqs2014.ws/archive/presen... ·...
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M. IMADA
November 20, 2014, Kyoto
Superconducting mechanisms of
iron-based and cuprate superconductors
Masatoshi ImadaCollaborator: Takahiro Misawa
Shiro Sakai
Marcello Civelli
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M. IMADA
Topological states in iridium oxides
A2Ir2O7
Weak topological
insulator:
Protected metallic
state at domain wall
Edge state of 1D weak Chern insulator
⇒ controllability
Na2IrO3
Ab initio study
Zig-zag order in agreement with experiment
How can we approach Kitaev spin liquid?
Yamaji, Nomura, Kurita, Ryotaro Arita, Imada
Phys. Rev. Lett. 113, 107201 (2014)
Yamaji, Imada, Phys. Rev. X 4, 021035 (2014)
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M. IMADA
Outline
1. Introduction
2. How to identify the mechanism of high-Tc?
Hidden fermion theory for the cupratesarXiv:1411.4365
3. Ab initio studies on iron-based superconductors
arXiv:1409.6536
Phys. Rev. Lett. 108, 177007 (2012)
4. Mechanism of superconductivity for 2D Hubbard
Phys. Rev. B 90, 115137 (2014)
5. Outlook
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M. IMADA
Introduction
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M. IMADA
High-Tc superconductors
© Kitagawa &Kittaka
© Atsushi Fujimori
© Y. Kamihara et al.
Superconductivity above 50K
2D anisotropy, square lattice
close to antiferromagnetic order
cuprates, iron-based superconductors
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M. IMADA
Outline
1. Introduction
Ab initio Approach
2. How to identify the mechanism of high-Tc?
Hidden fermion theory for the cuprates
arXiv:1411.4365
3. Mechanism of superconductivity for 2D Hubbard
4. Ab initio studies on iron-based superconductors
5. Outlook
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M. IMADA
How was the mechanism of the conventional BCS electron-phonon superconductivity solved?
strong-coupling superconductivity
McMillan-Rowell
1965, 1969
N(E
)
E
Eliashberg
eq. α2F
(E)
Emeasured phonon
density of states
neutron scattering
data
anomalous
self-energy
D (E)
S
Pb
dI/
dE
Bosonic (phonon)
glue makes peaks
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M. IMADA
Similar peak of anomalous self-energy & gap functionin cuprate models
Maier, Poilblanc,Scalapino
PRL 100, 237001 (2008)
Σano
Origin of peaks is not clear
Le Tacon et al.
Nat. Phys. 7, 725 (2011)
cf. Spin fluctuation scenariot-J model
Gap function
D(w) = z Σano
Kyung et al(08), Civelli(09)
cluster DMFT
2x2 cluster
exact
diagonalization
for T > 0
Hubbard model
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M. IMADA
Peak indeed generates high Tc
0
2 Im ( , ')Re ( , 0) '
'd
ww w
w
DD = =
kk
0
2 Im ( , ')( , ) '
Re ( , 0) 'I d
ww
w w
D =
D = k
kk
cf. Maier, Poiblanc,
Scalapino, PRL’08
I(kAN,=0.5)=0.8: 80% of the gap is attributed to the peak!
Gap function
What makes this peak?
Gap function
D(w) = z Σano
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M. IMADA
Poles of Snor and Sano
n=0.95
Perfect agreement
Peak in Im Sano comes from
the pole of Sano
arXiv:1411.4365
ImS nor and ImS ano are peaked at the same energy!
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M. IMADA
Pole cancellation between Snor and Sano
If the peak directly comes from
bosonic excitations such as
spin fluctuations,
the cancellation cannot happen.
U=8t t’=-0.2tn=0.95T=0.01k=kAN
Poles of Snor/ano are
invisible in A(k,w).
1nor
ano 2
nor *
( , ) ( , ) ( , )
( , )( , )
( , )
G W
W
w w w w
ww
w w
= S
S=
S
k
k
k k k
kk
k
Snor cancels with W !
1( , ) Im ( , )A Gw w
= k k
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M. IMADA
Two-component fermion
†
1
1
2
22
[ ( ) ( )( . ) '( ) ]
'1( )
' ( )( ')
' 1
( )( ')( )
'
k k k k k k
k
cc
H k c c k c d h c k d d
G H
G
w w w
w w w w
w
w w w
w
=
= = =
= =
† † †
S=
w
1G
2
'w
S =
mutually hybridizing
c and d fermions
c d
origin of mean field gap
of CDW, SDW(AF), ....
hybridization gap =
zero of Gc = pole of Sc= pole of Gd
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M. IMADA
Two-component fermion II
† † † †
[ ( ) ( )( . ) ( )
+ H.c.]
c k k k k d k k
k
c k k d k k
H k c c k c d h c k d d
c c d d
=
D D
† † †
for Λ=0
becomes complicated, but
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M. IMADA
Zeros of Green’s function
Poles of Σcnor and Vc completely cancel
⇒ G does not have zeros at the poles of the self-energy!
This cancellation disappears in the pseudogap phase
⇒ Zeros of the quasiparticle Green’s function emerge
at the poles of d-fermion Green’s function
= pseudogap
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M. IMADA
Origin of pseudogap
pole of hidden fermion
→ pole of Snor
Below Tc it disappears
because of the cancellation by Sano
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M. IMADA
Excellent agreement between CDMFT and TCFT
U=8t’=-0.2n=0.96T=0.01
( ) ~ ( ), ( , ).f c =k k Q Q
-A(k,w): d-wave
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M. IMADA
What is the hidden fermion d ?
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M. IMADA
Candidate: Quasiparticle vs. Composite fermion
quasiparticle:
kinetic energy gain interaction energy gain
life time
hybridization composite fermion:
Yamaji & Imada
PRL101 (2011) 016404
PRB 83 (2011) 214522
natural extension of exciton
† † 11
(1 ), mi i i im m
d c n m n
( )† † †(1 ) (1 ) 1(1 ) 1
4 2(1 2 ) 2 1 2
m m m m m mUn n U c d d c U d d U n
m m
=
cf. L. Zhu & J.-X. Zhu PRB (2013) hybridizatoin
incoherent part of fermion
d and f satisfy fermion anticommutation approximately
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M. IMADA
Origin of high Tc
Peak of Im D = pole of hidden fermion (composite fermion)
Nearly localized incoherent electron
acquire local large binding energy
of pair
hybridization
proximity to quasiparticle
not boson but fermion
boosts up Tc
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M. IMADA
Outline
1. Introduction
Ab initio Approach
2. How to identify the mechanism of high-Tc?
Hidden fermion theory for the cuprates
3. Ab initio studies on iron-based superconductors
arXiv:1409.6536,
Phys. Rev. Lett. 108, 177007 (2012)
4. Mechanism of superconductivity for 2D Hubbard
5. Outlook
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M. IMADA
Experimental Discovery
Ln = La, Pr, Sm, …
Tc ~ 26K-55K
Kamihara et al, JACS
130, 3296 (2008)
Antiferro-
magnetic
metal
LnFeAs(O1-xFx)
Mukuda et al. PRB
89 (2013) 064511
Zhao et al. Nat .Mat.
7,963 (2008)
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M. IMADA
downfolding;
Fe 3d 5 band models
(d model)
First Principles Approach
dimensional
downfolding
→ 2 D effective model
Review: Imada, Miyake:
J. Phys. Soc. Jpn. 79 (2010) 112001
MACEtarget bands
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M. IMADA
Ab initio derivation of U by constrained RPA
U / t :d model dp model
LaFePO 8 20
LaFeAsO 9 20
FeTe 11 26
FeSe 14 30 Miyake, Nakamura, Arita, Imada
JPSJ 79 (2010) 044705
smaller size of Wannier
⇒ larger bare Coulomb
smaller covalency
⇒ poor screening
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M. IMADA
Variational Monte Carlo Tahara, MI
JPSJ 77 (2008)
114701
fij : pair-dependent variational parameter
optimization of 1000-10000 variables to overcome bias
Gutzwiller factor
quantum number
projection
Gros
Sorella et al.
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M. IMADA
variational Monte Carlo; accuracy
Capello et al. PRB 72(2005) 085121
Tomonaga Luttinger liquid
S(0)S(r)∝(logr)1/21/r1+Kρ
R. Kaneko, S. Morita, MI
algebraic decay
∝1/r
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M. IMADA
Solution of low-energy solver
ordered magnetic moment
see also Yin Haule Kotliar Nat. Mat. (2011)
Misawa et al.
JPSJ 80 (2011) 023704
PRL 108 (2012) 177007near magnetic quantum critical point
VMC result for
ab initio models of
mother compounds
★ experiment
◇ ab initio model
● λ scaled model
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M. IMADA
Detailed Study on Doping Effect
Orbital Selective Mottnessand
Charge Inhomogeneity
arXiv:1409.6536, Nat. Commun. in press
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M. IMADA
dx2-y2 Mottness and Stripe Order
Orbital selective Mott insulator
Ishida, Liebsch
Misawa, Imada
2 2X Yd
stays at half filling
for δ<0.05
2 2X Yd
Stripe order
driven by
high-spin to low-spin transition by JH
⇒ strong first order transition
two first-order transitions of
stripe order cf. nematic
LAF
SAF
order
LAF
SAF
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M. IMADA
Phase Separation
Phase separation necessarily
appears around the first-order
transitions
0.1 < δ < 0.16
Takeshita, Kadono
New J. Phys. 11 (2009) 1367.
Charnukha et al. PRL 109, 017003 (2012)
Lang et al. PRL 104, 097001 (2010)
Park et al. PRL 102 (2009) 117006
Inosov et al. PRB 79, 224503 (2009)
Lang et al.
Maxwell
construction
NQR
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M. IMADA
Superconducting Mechanism
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M. IMADA
Superconductivity
s±symmetry (3s)orbital gives
dominant contribution
2 2X Yd
2 2 2 23 , 3 ,lim ( )
s X Y s X YrP r
D =
2 2X Yd
0.08<d<0.32;
SC, N
two local minima
governs magnetism
& superconductivity
⇒ similarity to cuprates
0.2 < d < 0.32
SC ground state
Superconducting order has domes
near first-order jumps
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M. IMADA
Role of Electron Correlation
λ
λ = 0.95
Sensitive dependence
on λ
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M. IMADA
Phase Diagram
λ~0.96 ⇔ experiment
Possible small role of
electron phonon int.
LaFeAsO1-xHx
Yamaura et al.
QCP
LaFePO
Nomura et al. (2013)
0.4 eV attraction within 0.02 eV
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M. IMADA
Smoking Gun of Superconducting Mechanism
and -d2E/dδ2 show
same peak structure:
One-to-one correspondence
2 23 ,s X YD
Superconductivity around
1st order trans. and PS
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M. IMADA
Summary
1. Ab intio electronic model shows s± superconducting phase
by electron doping into stripe AF phase of LaFeAsO.
Agreement with experiment
2. Orbital selective Mottness of dx2-y2 orbital holds an underlying
key for the emergence of the high-Tc superconductivity.
Major role for both magnetism and superconductivity.
3. Superconductivity emerges because of the charge instability
accompanied by the PS caused by the strong 1st order
AF/nematic transition.
Smoking gun is found in one-to-one correspondence between
charge compressibility and superconductivity in various cases.
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M. IMADA
Single band Hubbard modelMisawa & Imada
Phys. Rev. B 90, 115137 (2014)
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M. IMADA
Single band Hubbard model Misawa & Imada
Phys. Rev. B 90, 115137 (2014)
Charge fluctuation
has one-to-one
correspondence to SC
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M. IMADA
Conclusion
1. “Hidden fermion” boosts up D and hence Tc
2. Cancellation of Snor and Sano in A(k,w)
3. Hidden fermion may represent incoherent
and excitonic electron ⇔ large gap
proximity to QP
4. Iron-based SC emerges from density fluct.
5. Hubbard model has a similar origin of SC
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M. IMADA
Thank you