quantum galvanometer by interfacing a vibrating nanowire

5
Quantum Galvanometer by Interfacing a Vibrating Nanowire and Cold Atoms O. Ka ́ lma ́ n, T. Kiss, J. Forta ́ gh, and P. Domokos* ,Research Institute for Solid State Physics and Optics of the Hungarian Academy of Sciences, H-1525 Budapest P.O. Box 49, Hungary Physikalisches Institut, Universita t Tubingen, Auf der Morgenstelle 14, 72076 Tubingen, Germany ABSTRACT: We evaluate the coupling of a BoseEinstein condensate (BEC) of ultracold, paramagnetic atoms to the magnetic field of the current in a mechanically vibrating carbon nanotube within the frame of a full quantum theory. We find that the interaction is strong enough to sense quantum features of the nanowire current noise spectrum by means of hyperfine-state- selective atom counting. Such a nondestructive measurement of the electric current via its magnetic field corresponds to the classical galvanometer scheme, extended to the quantum regime of charge transport. The calculated high sensitivity of the interaction in the nanowireBEC hybrid systems opens up the possibility of quantum control, which may be further extended to include other relevant degrees of freedom. KEYWORDS: Carbon nanotubes, nanowires, cold atoms, Bose-Einstein condensates, quantum sensors, quantum noise C arbon nanotube (CNT) technology has evolved to the point where CNTs can be produced with a variety of mechanical and electrical properties. 1 Besides applications in chemical, 2 biological, 3 and mass sensing with up to single atom resolution, 4 high-quality nanomechanical resonators, 5 one- dimensional electric transport effects, and their coupling to mechanical motion of the CNTs have been observed. 6,7 The increasingly fine control of these degrees of freedom anticipates the manipulation of CNTs at a quantum mechanical level that has been recently achieved in other nanomechanical systems. 8 Atomic physics has undergone a breathtaking evolution since laser cooling and trapping techniques allowed for the preparation of localized and isolated atom samples. 9 The thermal noise has been reduced to the ultimate quantum noise level where the ultracold atoms (below 1 K) form a degenerate quantum gas, called a BoseEinstein condensate (BEC). 10 This cloud of atoms can be controlled in all relevant degrees of freedom with an unprecedented precision. The cloud can be positioned on the submicrometer scale in magnetic 11 or optical traps. 12 The internal electron dynamics can be driven by external laser or microwave fields, which allow for the precise preparation as well as the high-efficiency detection of the electronic state. The system of trapped neutral atoms in the collective BEC state is an ideal probe of external fields. 13 The first attempts to make a BEC interact with a CNT have been reported only recently. Atom scattering from the CNTs van der Waals potential 14 and the field ionization due to charged suspended nanotubes have been observed. 15 Recent proposals have discussed how to make use of the CNT as a current-carrying thin nanowire to tighten the magnetic trapping potential for cold atoms 16 and how to form nanoscale plasmonic atom traps along silver-decorated CNTs. 17 The integration of CNTs and atomic BECs opens up new avenues toward hybrid systems coupling these objects at a quantum level in a controlled way. One can envisage the coherent interfacing of very different degrees of freedom such as electronic, mechanical, and spin variables. A variety of novel nanodevices for precision sensing, quantum measurement, and quantum information processing could be developed on the basis of CNT-BEC coupling. The question is whether there is a suitable interaction between selected degrees of freedom and whether the cross-coupling is strong enough to design useful quantum devices. In this Letter we theoretically evaluate the interaction between the current through the nanowire and atoms in a condensate. We describe how the internal atomic dynamics in the hyperfine states couples to the magnetic field generated by the CNT current. Starting from a fully quantum model, we calculate the time evolution of the atomic system and construct a scheme to measure the current via an atomic observable. All this leads to the conclusion that quantum dynamical properties of the CNT are detectable by making use of the mature technology of ultracold atoms. A more general implication is that the other degrees of freedom of the CNT and BEC that take part in the dynamics can also be accessed and possibly manipulated in variants of this scheme. For the sake of concreteness, we focus on the measurement of the current through the CNT in the galvanometer scheme, Received: October 25, 2011 Letter pubs.acs.org/NanoLett © XXXX American Chemical Society A dx.doi.org/10.1021/nl203762g | Nano Lett. XXXX, XXX, XXXXXX

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Page 1: Quantum Galvanometer by Interfacing a Vibrating Nanowire

Quantum Galvanometer by Interfacing a Vibrating Nanowire andCold AtomsO. Kalman,

†T. Kiss,

†J. Fortagh,

‡and P. Domokos*,†

†Research Institute for Solid State Physics and Optics of the Hungarian Academy of Sciences, H-1525 Budapest P.O. Box 49, Hungary‡Physikalisches Institut, Universita �t Tu�bingen, Auf der Morgenstelle 14, 72076 Tu �bingen, Germany

ABSTRACT: We evaluate the coupling of a Bose−Einsteincondensate (BEC) of ultracold, paramagnetic atoms to the magneticfield of the current in a mechanically vibrating carbon nanotubewithin the frame of a full quantum theory. We find that theinteraction is strong enough to sense quantum features of thenanowire current noise spectrum by means of hyperfine-state-selective atom counting. Such a nondestructive measurement of theelectric current via its magnetic field corresponds to the classicalgalvanometer scheme, extended to the quantum regime of chargetransport. The calculated high sensitivity of the interaction in thenanowire−BEC hybrid systems opens up the possibility of quantumcontrol, which may be further extended to include other relevantdegrees of freedom.KEYWORDS: Carbon nanotubes, nanowires, cold atoms, Bose-Einstein condensates, quantum sensors, quantum noise

Carbon nanotube (CNT) technology has evolved to thepoint where CNTs can be produced with a variety of

mechanical and electrical properties.1 Besides applications inchemical,2 biological,3 and mass sensing with up to single atomresolution,4 high-quality nanomechanical resonators,5 one-dimensional electric transport effects, and their coupling tomechanical motion of the CNTs have been observed.6,7 Theincreasingly fine control of these degrees of freedom anticipatesthe manipulation of CNTs at a quantum mechanical level thathas been recently achieved in other nanomechanical systems.8

Atomic physics has undergone a breathtaking evolution sincelaser cooling and trapping techniques allowed for thepreparation of localized and isolated atom samples.9 Thethermal noise has been reduced to the ultimate quantum noiselevel where the ultracold atoms (below 1 �K) form adegenerate quantum gas, called a Bose−Einstein condensate(BEC).10 This cloud of atoms can be controlled in all relevantdegrees of freedom with an unprecedented precision. Thecloud can be positioned on the submicrometer scale inmagnetic11 or optical traps.12 The internal electron dynamicscan be driven by external laser or microwave fields, which allowfor the precise preparation as well as the high-efficiencydetection of the electronic state. The system of trapped neutralatoms in the collective BEC state is an ideal probe of externalfields.13

The first attempts to make a BEC interact with a CNT havebeen reported only recently. Atom scattering from the CNT’svan der Waals potential14 and the field ionization due tocharged suspended nanotubes have been observed.15 Recentproposals have discussed how to make use of the CNT as acurrent-carrying thin nanowire to tighten the magnetic trapping

potential for cold atoms16 and how to form nanoscaleplasmonic atom traps along silver-decorated CNTs.17 Theintegration of CNTs and atomic BECs opens up new avenuestoward hybrid systems coupling these objects at a quantumlevel in a controlled way. One can envisage the coherentinterfacing of very different degrees of freedom such aselectronic, mechanical, and spin variables. A variety of novelnanodevices for precision sensing, quantum measurement, andquantum information processing could be developed on thebasis of CNT-BEC coupling. The question is whether there is asuitable interaction between selected degrees of freedom andwhether the cross-coupling is strong enough to design usefulquantum devices.In this Letter we theoretically evaluate the interaction

between the current through the nanowire and atoms in acondensate. We describe how the internal atomic dynamics inthe hyperfine states couples to the magnetic field generated bythe CNT current. Starting from a fully quantum model, wecalculate the time evolution of the atomic system and constructa scheme to measure the current via an atomic observable. Allthis leads to the conclusion that quantum dynamical propertiesof the CNT are detectable by making use of the maturetechnology of ultracold atoms. A more general implication isthat the other degrees of freedom of the CNT and BEC thattake part in the dynamics can also be accessed and possiblymanipulated in variants of this scheme.For the sake of concreteness, we focus on the measurement

of the current through the CNT in the galvanometer scheme,

Received: October 25, 2011

Letter

pubs.acs.org/NanoLett

© XXXX American Chemical Society A dx.doi.org/10.1021/nl203762g | Nano Lett. XXXX, XXX, XXX−XXX

Page 2: Quantum Galvanometer by Interfacing a Vibrating Nanowire

i.e., when the electric current is sensed in a nondestructive wayvia its magnetic effect. We are interested in the quantumtransport limit of a mesoscopic conductor. In principle, aquantum object such as a spin-1/2 particle precessing in themagnetic field is sensitive to the quantum properties of thecurrent. The full counting statistics of the charge transportprocess18 can be reconstructed from the density matrix of thespin.19 This scheme is sometimes referred to as the “quantumgalvanometer”.20 However, its realization has to meet severalconditions (stability, sensitivity, and detectability; see below),which has seemed out of the question so far.In our scheme, the fictitious spin of the quantum

galvanometer is realized by a cloud of long-term trappedatoms. One can make use of the collective BEC state, whichgreatly enhances the sensitivity of the internal hyperfinedynamics to external magnetic fields.21 Moreover, a directreadout method for the spin state is available since thepopulations in the magnetic sublevels can be counted by stateselective ionization with single-atom resolution.22 The pop-ulations are expressed in the diagonal elements of the spindensity matrix. In principle, the off-diagonal elements couldalso be measured, which is required to determine thegenerating function of the full counting statistics. Here wepropose a simpler measurement restricted to the diagonalelements, since it is already enough to characterize some of thequantum features of the current. In particular, we will show thatthe ordinarily defined current noise spectrum

(1)

is directly related to the time evolution of the populations inthe given magnetic sublevels. The proposed galvanometerallows for the measurement of the spectrum by scanning theadjustable variable ω, which spans both the negative andpositive frequency ranges. Asymmetry of the measuredspectrum around ω = 0 would reveal quantum features.23

This is due to the fact that asymmetry of S(ω) is equivalentwith the noncommutativity of the current operator at differentinstances, as one can easily check in the above equation.The scheme is presented in Figure 1 for a possible

architecture of building the galvanometer on an integratedplatform, the so-called “atomchip”.11,24 It is a compact,substrate-based electric circuit of currents that create highlytunable magnetic traps for the neutral atoms. The chip maysupport a contacted CNT on the side facing the BEC. Thesuspended CNT is a high-Q mechanical oscillator,5,8,25,26 whichis driven to oscillate coherently with large amplitude. We notethat, in order to simplify our calculations, here we assume thatthe vibration of the CNT is driven by a mechanical source (e.g.,a piezo crystal) instead of electric fields. Therefore the CNTcurrent generates a harmonically time-varying magnetic field. Inthe neighboring BEC, this field may excite transitions betweenthe hyperfine states. The key role of the mechanical vibration ofthe CNT consists in creating the resonance conditions suchthat the low-frequency components of the current noisespectrum be close to resonance with the hyperfine transitions(Zeeman splitting), c.f., Figure 2. Initializing the atoms in theBEC in a well-defined hyperfine state, the number of atomstransferred to another state follows a statistics determined bythe low-frequency part of the current noise spectrum. Thenoise source can be arbitrary, e.g., thermal or intrinsic quantumnoise; for generality, we will represent the current as a quantumoperator in the derivation. Finally, the measurement is

accomplished by detecting the number of transferred atomsin a given time period, which can be performed by means ofstate-selective ionization technique at the single-atom reso-lution level.22

To be specific, we consider ultracold 87Rb atoms in thehyperfine state F = 1. The atomic spin F� interacts with themagnetic field according to the Zeeman term HZ = gF�BF�B(r),where �B = e�/2me is the Bohr magneton, the Lande factor is gF= −1/2, and F� is measured in units of �. The dominantcomponent of the magnetic field is a homogeneous offset fieldBoffs in the z direction. The eigenstates of the spin componentF�z are then well separated by the Zeeman shift. These are themagnetic sublevels labeled by m = −1,0,1. On top of the offsetfield, there is an inhomogeneous term that creates an ellipsoidalpotential around the minimum of the total magnetic field. Theatoms are then subject to the static potential Vm(r) = −mVT(r)+ gF�BmBoffs, where VT(r) = M/2[ωr

2(x2 + y2)+ωz2z2], with M

being the atomic mass. The potential is diagonal on the F�z basis,and is confining only for m = −1.

Figure 1. The quantum galvanometer on an atomchip. A BEC isloaded into the magnetic microtrap created by the classical electriccurrents through integrated conductors on a dielectric substrate11

(represented on the bottom of the chip). A suspended CNT is alsopart of the electric circuit16 and transports the quantum current. Theoscillating CNT creates a magnetic field in the 10 MHz rangeinteracting with the hyperfine transitions of the atoms. Atomstransferred to untrapped states are detected by a single-atomdetector.22

Figure 2. Level scheme of the 87Rb atoms. The inset shows theresonance condition for the m = −1↔0 rf transition induced by thetime-varying magnetic field component due to the oscillating CNT.The shaded region corresponds to the band of energies in theThomas−Fermi approximation. The detection of atoms in the spatiallyseparated state F = 1, m = 0 is performed by a resonant microwaveexcitation to F = 2, m = 0 (curly arrow), and then by a photoionizationprocess22 (double arrow).

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Let us consider a single CNT of length L that is electronicallycontacted and carries a current I �(t). It generates a magneticfield that interacts with the atomic spin. Similar coupling hasbeen considered27 between a vibrating nanomagnet and a BEC.The CNT is aligned with the z axis (see Figure 1) having amean distance y0 from the condensate. This distance is largeenough (y0 ≥ 1 �m to avoid van der Waals-type interactionsbetween the atoms and the CNT14,15,28−30). The CNT isdriven to mechanically oscillate harmonically at an angularfrequency ωcnt in the 10 MHz range25,26 and with an amplitudea in the y−z plane (a � y0). The resulting time-dependentmagnetic field B�cnt(r,t) is an operator, since its source is thecurrent operator I �. With a proper tuning of the Zeemansplitting via the offset Boffs, the x and y components of B�cnt canquasi-resonantly generate transitions between the magneticsublevels m. Such a transfer of trapped atoms into untrappedones is the underlying mechanism of the radio frequency (rf)outcoupler of an atom laser.31 Here a fast detection of thespatially separated component m = 0 will be required by meansof combined microwave transition and photoionizationprocess22 via the state F = 2, m = 0 (see Figure 2).In the following, we will describe the BEC−CNT interaction

based on a model Hamiltonian (eq 2), which treats all therelevant degrees of freedom quantized. Within the Thomas−Fermi approximation (large condensate limit, eq 3) and to firstorder in perturbation theory (eq 4), we will solve the dynamicsfor the time evolution of the atomic state populations (eq 8).Thereby, we will obtain a relation between the population inthe externally monitored hyperfine state and the current noisespectrum in a closed form (eq 12). This relation is aconvolution that includes a detection spectral functioncharacterizing the resolution of the measurement (eq 11).We will present its functional form in Figure 3 and discuss howits magnitude depends on the physical parameters of the setup.

The ultracold atom cloud can be described by the spinorfield32 ∑mΨ� m|F = 1,m�. The very general many-bodyHamiltonian is given by

(2)

where the first term is the kinetic energy. The atom−atominteraction in this ultracold regime is s-wave scattering, and spinflipping collisions are negligible. In principle, the coupling terminduces a dynamical back action on the current and thevibration of the CNT. Here we will disregard the back action;however, we note that it could be the source of interesting neweffects in similar schemes.We assume that there is a condensate of a number of N

atoms in the trapped m = −1 magnetic sublevel. Forconvenience, we separate the condensate part (N1/2ϕBEC)from the excitations (δΨ�m), which will be treated perturba-tively. The condensate wave function is ϕBEC(r,t) =e−i�′t/�ϕBEC(r) where �′ is the chemical potential, and ϕBEC(r)obeys the Gross−Pitaevskii equation.31 We restrict ourselves tothe Thomas−Fermi approximation, i.e., we neglect the kineticenergy term in the Gross−Pitaevskii equation. Then thecondensate wave function is

(3a)

(3b)

The condensate shape is an ellipsoid with principal semiaxes b= (2�/Mωr

2)1/2 and c = (2�/Mωz2)1/2. The atom−atom

collisions are accounted for by g = 4π�2as/M, where as is thes-wave scattering length (as = 5.4 nm for 87Rb). We will neglectthe back action of the other spin components onto thecondensate and assume that the condensate is intact during theinteraction time.To first order in the perturbations, the equation of motion

for the component δΨ� 0, after some straightforward calculation,is obtained as

(4)

where we have omitted the subscript “cnt” when writing thecomponents of the magnetic field created by the currentthrough the nanotube, which for a� y0 can be approximated asB�i(r,t) ≈ B�i0(r,t) + δB�i(r,t) cos(ωcntt), (i = x,y). The last termwith the quantum field δΨ� −1 in eq 4 is small compared to thatof the condensate part, and will be neglected. In accordancewith the Thomas−Fermi approximation of the condensate, weneglect the kinetic energy of the excited field, too. By moving toa frame rotating at the frequency �′/� − ωcnt we get a simple,spatially local driving equation:

(5a)

Figure 3. The dotted curve shows the approximation d (ω) from eq11a, compared to the exact (ω) in units of ndet for different numberof trapped atoms N for a trap with radial and axial frequencies ωr = 2π× 500 s−1, and ωz = 2π × 109 s−1, respectively. The correspondinglongitudinal extent c of the atom cloud and the chemical potential arepresented in the table. Note that the radial confinement of the cloud isdetermined by b/c = ωz/ωr. Here we assumed the lengths of the CNTand the CNT−BEC distance to be L = 2 �m, and y0 = 4 �m,respectively.

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Page 4: Quantum Galvanometer by Interfacing a Vibrating Nanowire

with a spatially inhomogeneous detuning

(5b)

and driving amplitude

(5c)

The time independence of the driving is due to neglecting allterms that oscillate with ωcnt or 2ωcnt in the rotating frame andaverage out on time scales longer than 1/ωcnt. The magneticfields B�i0 also average out. The dimensionless function U(r)expresses the spatial variation of the magnetic field modulationdue to the CNT:

(6)

where all the length quantities in the integrand are in units ofthe CNT−BEC distance y0. We note that U(r) is obtained froman infinitely thin finite-length current-carrying wire that isoscillating as a string clamped at both ends.Starting with a pure condensate at t = 0, and letting the

system evolve to t = T (the measurement time), the integrationof eq 5a leads to

(7)

which expresses the relation between the quantized current I � inthe CNT and the atom field in the magnetic sublevel m = 0.Atom counting in this sublevel allows us to extract quantumstatistical properties of the current. We assume stationarycurrent, i.e., �I �(t′)I �(t″)� = �I �(0)I �(t″−t′)�. Then the spatiallyintegrated mean number of atoms transferred into the sublevelm = 0 during the measurement time T is

(8)

The transferred atom number, as being explicitly indicated, is afunction of the frequency � = ωcnt−�BBoffs/(2�), which can befinely tuned by the magnetic field Boffs. Note that ωcnt istypically around 2π × 50 MHz,25,26 whereas the Larmorfrequency �BBoffs/(2�) can be tuned in the range of 0.1−100MHz.The measurable N(�) is related to the current noise

spectrum S(ω) by a convolution with the spectral resolutionfunction, {f(τ) (τ)}, where {...} denotes Fourier trans-form. The mapping involves a triangular pulse function

(9)

which originates from the finite measurement time. Allproperties of the BEC−CNT coupling are embedded in

(10)

Because of the exponential term, the variation range of thepotential energy VT(r) determines the intrinsic bandwidth ofthe BEC as a probe system (see also Figure 3). This bandwidthis the chemical potential �, which is typically in the range ofkHz for a BEC on a chip.For very short measurement time T � �/�, the exponential

in the integrand of eq 10 can be approximated by 1, so thespectral resolution is dominated solely by f(τ). On the otherhand, for long measurement time T � �/� ∼1 ms, theapproximation f(τ) = 1 − |τ|/T ≈ 1 holds in eq 8 since thefunction (τ) introduces a cutoff at about �/�. In this limit,the CNT-BEC coupling function (τ) determines thequantum efficiency of the scheme.

(τ) can be approximated by neglecting the variation of themagnetic field within the condensate, U(r) ≈ U(0) ≡ U. Thisleads to the Fourier transform

(11a)

(11b)

(11c)

where the normalization ∫ −∞∞ dwd (w) = 1 is obeyed. In Figure3, the approximate (ω) (dotted curve) is compared to exactones which are obtained numerically for different atomnumbers N when the CNT length and the CNT−BECdistance is fixed. It can be seen that eq 11a gives the correctorder of magnitude and shape of the exact (ω) for a broadrange of the BEC size.The detectable atom number spectrum, from eq 11a is

expressed in the form of the convolution

(12)

where ω and � are in units of �/�. Measuring the atomnumber at a single value of �, the current noise spectrum isreadily obtained around this frequency with a kilohertzresolution, i.e., averaged in the bandwidth of the BEC chemicalpotential �/�. By fine-tuning � via the field Boffs and usingdeconvolution, the spectrum S(ω) can be deduced with a muchhigher resolution. We recall that � is a frequency relative to theCNT vibrational frequency ωcnt. Hence it can be set to bothpositive and negative values, which is substantial to the quantumgalvanometer. Finally we note that the maximum frequencyrange of S(ω) that can be accessed by the method is limited bythe vibrational frequency ωcnt to be conform with the rotatingwave approximation.The integral norm of S(ω) is �I �2�. Then, separating the �-

dependence given by the convolution of normalized spectralfunctions, the coupling strength is on the order of T�ndet�I �2�/�.For a numerical estimate, consider a system described in Figure3, where an L = 2 �m CNT is oscillating with an amplitude of a= 10 nm,25 at a distance y0 = 4 �m from the BEC, in which caseU2 ≈ 0.4. For a measurement time T ≈ 1s that conforms withthe BEC lifetime in atomchip microtraps, a single atomdetected, Nlong = 1, corresponds to quantum fluctuations of thecurrent on the order of �I �2�1/2 ≈ 1 �A.

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We note that the thermal magnetic near-field noise, which ispresent in the case of room-temperature atomchips due to thetrapping wires or metallic coatings on the substrate, has highfrequency components resonant with the hyperfine splittingand thus induces spin flips.33−36 This parasitic effect must besuppressed by moving the trap to sufficiently large distancefrom such field sources, while keeping the BEC−CNT distancey0 in the micrometer range, or by using superconductingatomchips.37

In conclusion, we have evaluated the coupling of trappedatoms to the magnetic field created by the electric current in amechanically vibrating CNT. The modeled coupling was foundto be strong enough to sense quantum features of the currentnoise spectrum by means of hyperfine-state-selective atomcounting. Hence, our calculations prove that a quantumgalvanometer could be realized on the basis of the interactionbetween a CNT and a BEC of ultracold alkali atoms. Besidesthe possibility for the experimental realization of a quantumgalvanometer, the proposed BEC−CNT coupling schemeopens the way to couple other degrees of freedom in thishybrid mesoscopic system. For example, one could devise“refrigeration” schemes38 in which heat is extracted from thevibrational motion of the CNT and transferred to the ultracoldgas of atoms. A mechanical/cold atom hybrid quantum systemwould provide an ideal platform to study thermally drivendecoherence mechanisms in nanoscaled quantum systems andwould push the sensitivity of mechanical sensors to the ultimatequantum limit.

■ AUTHOR INFORMATIONCorresponding Author*E-mail: [email protected].

■ ACKNOWLEDGMENTSThis work was supported by the Hungarian National Office forResearch and Technology under the contract ERC_HU_09OPTOMECH, the Hungarian Academy of Sciences (Lendu �letProgram, LP2011-016), and the Hungarian Scientific ResearchFund (OTKA) under Contract No. K83858. J.F. acknowledgessupport by the BMBF (NanoFutur 03X5506) and the DFGSFB TRR21.

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Nano Letters Letter

dx.doi.org/10.1021/nl203762g | Nano Lett. XXXX, XXX, XXX−XXXE