pre-breakdown currents from tungsten nanofuzz – the surface with a

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D.N. Sinelnikov , D.G. Bulgadaryan, D.V. Kolodko, M.S. Lobov and N.A. Solovev National Research Nuclear University MEPhI (Moscow Engineering Physics Institute) Unipolar arcing Experimental procedure Experimental results Unipolar arcs in thermonuclear devices are negative phenomenon in plasma-surface interaction. The arcs significantly modify the wall surface, change local potential of plasma, contaminate plasma by microscopic particle injection in a solid and liquid state. This phenomenon was observed in several modern tokamaks, which simulate ITER exploitation: JET, JT-60U, DIII-D and ASDEX Upgrade. Moreover, there are propositions that the unipolar arcs limit plasma confinement with high parameters with increasing incoming power per square unit. Conclusion Pre-breakdown currents from tungsten nanofuzz – the surface with a high unipolar arc ignition probability 2 1 1 2 ln 5 , 0 e i i e e f T T m m kT V 2 4 ne kT e d 1 e i i e 2 e 1 T T 1 m m 2 ln ne kT E Tungsten “fuzz” structure W fuzz forms on a plasma-facing surface under the following conditions: •Tungsten surface temperature T in the range of 1000 - 2000 K •Irradiation by He + ions with energies 20-50 eV •Ion fluence > 10 25 m -2 and flux > 10 21 m -2 s -1 0,5 – 5 μm Ø 10 - 100 nm Field emission measurement 2. Focusing system 5. Keithley 6485 Ammeter Xe + , 5 keV 4. W Fuzz sample 3. Diaphragm 1. Ion source Surface modification on the “Large MEPhI Mass-Monochromator” Simulation of the electric field strength distribution in the vacuum gap Traces from unipolar arc on tungsten Mechanism of the unipolar arc initiation Plasma is positively charged due to hot electrons escape up to potential: This potential forms on several Debye radii: but in the dense plasma it can be rather small (~μm) => significant for autoemission electric field to accrue: Without emission site: With emission site: Field emission leads to the intensive heating of the emission site and results in its exploding which can be the initiator of unipolar arc. This structure contains a lot of helium bubbles with a diameter ~10 nm. Conditions for W fuzz formation are expected to be met in the divertor zone of ITER. W fuzz facilitates unipolar arcing, which could result in significant surface erosion and plasma contamination during ELMs in ITER. Experimental parameters: •Pressure under irradiation P=10 -5 Torr •Ion beam Xe + 5 keV •Ion current density j=3 μA/cm 2 Fuzzy sample after irradiation 1 2 3 4 5 6 7 8 Experimental scheme : 1. Membrane pump 2. Turbomolecular pump 3. Gate 4. Vacuum chamber 5. Pressure gauge 6. Ballast resistance 7. High voltage source 8. Nano ammeter Photo of the vacuum diode •The design of vacuum diode allows the cathode-sample ejection for a SEM observation and an ion beam irradiation without changing of the vacuum gap. •The vacuum gaps were in the range from 0.1 to 0.5 mm. •A spherical shape of the anode (d=10mm) was used for reducing field enhancement on the sample edges. •Working pressure 10 -7 Torr Vacuum gap 0.1 mm – emission area ~0,8 cm 2 Vacuum gap 0.5 mm – emission area ~1,8 cm 2 Dynamic of fuzz modification under the influence of the ion beam Ф=0 Ф=10 17 cm -2 Ф=5•10 17 cm -2 N f , μm -2 100±30 d f , μm 0.04±0.01 h f , μm ±0.2 ν f , μm 0.13±0.08 N b , μm -2 6±1 d b , μm 0.35±0,07 ν b , μm 0.17±0.11 Ф, μm -2 4.4±0.5·10 9 ν s , μm 0.021±0.002 Where ν f is a nanofibre volume, ν b is a ball volume and ν s is sputtered volume per 1 μm 2 of the smooth surface area. N f is the number of fuzz fibres per unit area, N b is the number of balls per unit area, d f is the fibre diameter, d b is the ball diameter, h f is the height above the smooth surface. ν f ≈ ν b and ν s << ν b This means that the balls are the result of nanofibre merging, however, redeposition due to sputtering is not the key process in the formation of balls. It is assumed that irradiation-induced He release from the bubbles is a major factor in the formation of ball-like structures. Fowler-Nordheim plots of the fuzzy surfaces 9 3/2 2 2 1/ 2 2.818 10 1 4.406 lg +lg 5.854 I S β = + E β E Slope Emission currents significantly decreased after the irradiation. Amplification of the electric field factors β were calculated for both surfaces: 370 (before irradiation) and 140 (after irradiation) using Fowler-Nordheim formula. They seem to be rather high for the observed surface relief. •Thermo-field emission could be the reason of such a high emission intensity. Irradiation can vanish emission sites on the surface formatted after field emission measurement: Ball-like structures were observed on a W fuzzy surface as a result of irradiation with the 5 keV Xe + beam. The threshold fluence for ball formation was estimated at ~10 17 сm -2 and redeposition due to sputtering can only account for 10% of the ball volume. Irradiation of the W fuzz structure by 5keV Xe + beam significantly decreases field emission currents and could reduce unipolar arc ignition probability. Fowler-Nordheim formula: Low erosion method of fuzzy surface modification is needed to reduce the emission current!

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D.N. Sinelnikov, D.G. Bulgadaryan, D.V. Kolodko, M.S. Lobov and N.A. SolovevNational Research Nuclear University MEPhI (Moscow Engineering Physics Institute)

Unipolar arcing

Experimental procedure

Experimental results

Unipolar arcs in thermonuclear devices are negativephenomenon in plasma-surface interaction. The arcssignificantly modify the wall surface, change localpotential of plasma, contaminate plasma bymicroscopic particle injection in a solid and liquidstate. This phenomenon was observed in severalmodern tokamaks, which simulate ITER exploitation:JET, JT-60U, DIII-D and ASDEX Upgrade. Moreover,there are propositions that the unipolar arcs limitplasma confinement with high parameters withincreasing incoming power per square unit.

Conclusion

Pre-breakdown currents from tungsten nanofuzz – the surface with a high unipolar arc ignition probability

2112ln5,0

e

i

i

eef T

TmmkTV

24 nekT e

d

1

e

i

i

e2e 1

TT1

mm2lnnekTE

Tungsten “fuzz” structureW fuzz forms on a plasma-facing surface underthe following conditions:

•Tungsten surface temperature T in the range of1000 - 2000 K•Irradiation by He+ ions with energies 20-50 eV•Ion fluence > 1025 m-2 and flux > 1021 m-2s-1

0,5 – 5 μm

Ø 10 - 100 nm

Field emission measurement

2. Focusing system

5. Keithley 6485 Ammeter

Xe+, 5 keV

4. W Fuzz sample

3. Diaphragm1. Ion source

Surface modification on the “Large MEPhI Mass-Monochromator”

Simulation of the electric field strength distribution in the vacuum gap

Traces from unipolar arc on tungsten

Mechanism of the unipolar arc initiationPlasma is positively charged due to hot electrons escape upto potential:

This potential forms on several Debye radii:

but in the dense plasma it can be rather small (~μm) =>significant for autoemission electric field to accrue:

Without emission site:

With emission site:

Field emission leads to the intensive heating of the emissionsite and results in its exploding which can be the initiator ofunipolar arc.

This structure contains a lot of helium bubbles with adiameter ~10 nm.Conditions for W fuzz formation are expected tobe met in the divertor zone of ITER.

W fuzz facilitates unipolar arcing, whichcould result in significant surface erosionand plasma contamination during ELMs inITER.

Experimental parameters:•Pressure under irradiation P=10-5 Torr•Ion beam Xe+ 5 keV•Ion current density j=3 μA/cm2

Fuzzy sampleafter irradiation

1

2

3

45 6

78 Experimental scheme :

1. Membrane pump2. Turbomolecular pump3. Gate4. Vacuum chamber5. Pressure gauge6. Ballast resistance7. High voltage source8. Nano ammeter

Photo of the vacuum diode

•The design of vacuum diode allows thecathode-sample ejection for a SEMobservation and an ion beam irradiationwithout changing of the vacuum gap.•The vacuum gaps were in the range from0.1 to 0.5 mm.•A spherical shape of the anode (d=10mm)was used for reducing field enhancement onthe sample edges.•Working pressure 10-7 Torr

Vacuum gap 0.1 mm – emission area ~0,8 cm2 Vacuum gap 0.5 mm – emission area ~1,8 cm2

Dynamic of fuzz modification under the influence of the ion beamФ=0 Ф=1017 cm-2 Ф=5•1017 cm-2

Nf, μm-2 100±30

df, μm 0.04±0.01

hf, μm ±0.2

νf, μm 0.13±0.08

Nb, μm-2 6±1

db, μm 0.35±0,07

νb, μm 0.17±0.11

Ф, μm-2 4.4±0.5·109

νs, μm 0.021±0.002

Where νf is a nanofibre volume, νb is a ball volume and νs is sputtered volume per 1 μm2of the smooth surface area.Nf is the number of fuzz fibres per unit area, Nb is the number of balls per unit area, df is the fibre diameter, db is the balldiameter, hf is the height above the smooth surface.

νf ≈ νb and νs << νbThis means that the balls are the result of nanofibre merging, however, redeposition due to sputtering is not the key process in the formation of balls.It is assumed that irradiation-induced He release from the bubbles is a major factor in the formation of ball-like structures.

Fowler-Nordheim plots of the fuzzy surfaces

9 3/2 2

2 1/2

2.818 10 1 4.406lg +lg 5.854I S β= +E β E

Slope

•Emission currents significantly decreasedafter the irradiation.•Amplification of the electric field factors βwere calculated for both surfaces: 370 (beforeirradiation) and 140 (after irradiation) usingFowler-Nordheim formula. They seem to berather high for the observed surface relief.•Thermo-field emission could be the reason ofsuch a high emission intensity.

Irradiation can vanish emission sites on the surfaceformatted after field emission measurement:

Ball-like structures were observed on a W fuzzy surface as a result of irradiation with the 5 keV Xe+ beam. The threshold fluence for ball formation was estimated at ~1017 сm-2 and redeposition due to sputtering can only

account for 10% of the ball volume.

Irradiation of the W fuzz structure by 5keV Xe+ beam significantly decreases field emission currents and could reduceunipolar arc ignition probability.

Fowler-Nordheim formula:

Low erosion method of fuzzy surface modification is needed to reduce the emission current!