part ii. p-orbital physics in optical lattices
TRANSCRIPT
![Page 1: Part II. p-orbital physics in optical lattices](https://reader033.vdocuments.us/reader033/viewer/2022042403/625d8000c02011623a550e89/html5/thumbnails/1.jpg)
Novel p-orbital physics in the honeycomb optical lattices
Congjun Wu
Department of Physics, UC San Diego
C. Wu, D. Bergman, L. Balents, S. Das Sarma, PRL 99, 70401 (2007);C. Wu, S. Das Sarma, PRB 77, 235107(2008);C. Wu, PRL 100, 200406 (2008);C. Wu, PRL 101, 186807 (2008);S. Zhang, H. Hung, and C. Wu, PRA, 053618 (2010);W. C. Lee, C. Wu, and S. Das Sarama, PRA 82, 053611(2010);M. C. Zhang, H. H. Hung, C. W. Zhang, and C. Wu, PRA 83, 023615 (2011).
![Page 2: Part II. p-orbital physics in optical lattices](https://reader033.vdocuments.us/reader033/viewer/2022042403/625d8000c02011623a550e89/html5/thumbnails/2.jpg)
Hsiang-hsuan Hung (UCSD)
Shizhong Zhang (OSU)
Machi Zhang (Tsinghua)
Leon Balents (UCSB)
S. Das Sarma (UMD)
2
Collaborators:
Thank I. Bloch, A. Hemmerich, T. L. Ho for helpful discussions.
Thank G. W. Chern (U Wisconsin), Y. P. Wang (IOP) for collaborations on various projects of orbital physics with cold atoms.
![Page 3: Part II. p-orbital physics in optical lattices](https://reader033.vdocuments.us/reader033/viewer/2022042403/625d8000c02011623a550e89/html5/thumbnails/3.jpg)
Outline
• Introduction: cold atoms in high orbital bands.
3
• Orbital fermions in the honeycomb lattice (fundamentally different from graphene)
Why orbital physics with cold atoms is interesting?
Flat band physics: exact results of Wigner crystal (single component) and ferromagnetism (two-component).
Exotic Mott insulator: frustrated orbital exchange; 120 degree model Kitaev model
Exotic band insulator: topological quantum anomalous Hall insulator
Unconventional f-wave Cooper pairing.
![Page 4: Part II. p-orbital physics in optical lattices](https://reader033.vdocuments.us/reader033/viewer/2022042403/625d8000c02011623a550e89/html5/thumbnails/4.jpg)
Research progress of cold atom physics
• Great successes of cold atom physics: BEC, BCS-BEC, etc…
• Orbital Physics: new physics of bosons and fermions in high-orbital bands in optical lattices.
Good timing: experiments on orbital-bosons.
Square lattice (Mainz); double well lattice (NIST, Hamburg); polariton lattice (Stanford).
J. J. Sebby-Strabley, et al., PRA 73, 33605 (2006); T. Mueller et al., Phys. Rev. Lett. 99, 200405 (2007); C. W. Lai et al., Nature 450, 529 (2007).
Here orbital refers to the different energy levels (e.g. s, p) of each optical site.
s
p
4
![Page 5: Part II. p-orbital physics in optical lattices](https://reader033.vdocuments.us/reader033/viewer/2022042403/625d8000c02011623a550e89/html5/thumbnails/5.jpg)
5
Fundamental features of orbital physics
• Orbital: a degree of freedom independent of charge and spin.
Tokura, et al., science 288, 462, (2000).
• Orbital degeneracy.
crystal field splitting
ge
gt
2
s-bond p-bond
p-orbitals: zyxppp ,, d-orbitals: xzyzxyzryx
ddddd ,,,, 2222 3
tt//
• Spatial anisotropy.
![Page 6: Part II. p-orbital physics in optical lattices](https://reader033.vdocuments.us/reader033/viewer/2022042403/625d8000c02011623a550e89/html5/thumbnails/6.jpg)
6
Transition metal oxide orbital systems
orbital charge
spin lattice
Manganite: La1-xSr1+xMnO4 Iron-pnictide: LaOFeAs
• Orbitals play an important role in magnetism, superconductivity, and transport properties.
![Page 7: Part II. p-orbital physics in optical lattices](https://reader033.vdocuments.us/reader033/viewer/2022042403/625d8000c02011623a550e89/html5/thumbnails/7.jpg)
• Solid state orbital systems: orbital physics only of fermions .
7
• Cold atom orbital systems: both fermions and bosons.
What is new? (I) Orbital bosons have no counterparts in solids
The ordinary many-body ground states of bosons satisfy the
“no-node” theorem, i.e., the wavefunction is positive-
definite.
Orbital bosons: (meta-stable excited states of bosons).
New materials of bosons beyond the “no-node” theorem.
Unconventional BECs with spontaneous time-reversal
symmetry breaking.
C. Wu, Mod. Phys. Lett. B 23, 1 (2009) —a short review.
![Page 8: Part II. p-orbital physics in optical lattices](https://reader033.vdocuments.us/reader033/viewer/2022042403/625d8000c02011623a550e89/html5/thumbnails/8.jpg)
s-bond p-bond
• Solid state: strongly correlated orbital systems are usually d-orbital transition metal oxides and f-orbital rare-earth compounds.
• Cold atom orbital systems:
(II) New materials of strongly correlated p-orbitals
• Most p-orbital solid state materials are weakly correlated (e.g.
semiconductors).
• Not many p-orbital Mott-insulators. Exceptions: Cs3C60, …
P-orbital has even stronger anisotropy than d and f ; Combination of strong anisotropy with strong correlation.
tt//
8
![Page 9: Part II. p-orbital physics in optical lattices](https://reader033.vdocuments.us/reader033/viewer/2022042403/625d8000c02011623a550e89/html5/thumbnails/9.jpg)
Outline
• Introduction: cold atoms in high orbital bands.
9
• Orbital fermions in the honeycomb lattice (fundamentally different from graphene)
Why orbital physics with cold atoms is interesting?
Flat band physics: exact results of Wigner crystal (single component)
Exotic Mott insulator: frustrated orbital exchange; 120 degree model Kitaev model
Exotic band insulator: topological quantum anomalous Hall insulator
Unconventional Cooper pairing: f-wave.
![Page 10: Part II. p-orbital physics in optical lattices](https://reader033.vdocuments.us/reader033/viewer/2022042403/625d8000c02011623a550e89/html5/thumbnails/10.jpg)
10
The p-orbital honeycomb lattice
• Three coherent laser beams polarizing in the z-direction.
G. Grynberg et al., Phys. Rev. Lett. 70, 2249 (1993).
also K. Sengstock’s recent work.
![Page 11: Part II. p-orbital physics in optical lattices](https://reader033.vdocuments.us/reader033/viewer/2022042403/625d8000c02011623a550e89/html5/thumbnails/11.jpg)
11
px;py-orbitals: flat bands; interaction effects dominate
ferromagnetism.
p-orbital fermions in the honeycomb lattice
C. Wu, D. Bergman, L. Balents,
and S. Das Sarma, PRL 99,
70401 (2007).
cf. graphene: pz-orbital; Dirac cones.
Our interest!
Not our interest
![Page 12: Part II. p-orbital physics in optical lattices](https://reader033.vdocuments.us/reader033/viewer/2022042403/625d8000c02011623a550e89/html5/thumbnails/12.jpg)
12
px, py-physics: get rid of the hybridization with s
• pz-orbital band is not a good system for orbital physics.
• However, in graphene, 2px and 2py are close to 2s, thus strong hybridization occurs.
• In optical lattices, px and py-orbital bands are well separated from s.
• Interesting orbital physics in the px, py-orbital bands.
isotropic within 2D; non-degenerate.
1s
2s
2p1/r-like potential
s
p
![Page 13: Part II. p-orbital physics in optical lattices](https://reader033.vdocuments.us/reader033/viewer/2022042403/625d8000c02011623a550e89/html5/thumbnails/13.jpg)
13
p-orbital honeycomb optical lattice
].)ˆ()([
].)ˆ()([
.].)ˆ()([
333
212
111//
cherprp
cherprp
cherprptHAr
t
• Band Hamiltonian (s-bonding) for spin-polarized fermions.
1p2p
3p
yx ppp2
1
2
3
1
yx ppp2
1
2
3
2
ypp
3
1e2e
3e
A
B B
B
0321 ppp
![Page 14: Part II. p-orbital physics in optical lattices](https://reader033.vdocuments.us/reader033/viewer/2022042403/625d8000c02011623a550e89/html5/thumbnails/14.jpg)
14
• If p-bonding is included, the flat bands acquire small width at the order of . Realistic band structures show
Flat bands from localized eigenstates
• Flat band + Dirac cone. • localized eigenstates.
t
p-bond
tt//
%1/ // tt
![Page 15: Part II. p-orbital physics in optical lattices](https://reader033.vdocuments.us/reader033/viewer/2022042403/625d8000c02011623a550e89/html5/thumbnails/15.jpg)
15
Realistic Band structure with the sinusoidal optical potential
3~1
22
)cos(2 i
i rpVm
H
s-orbital bands
px,y-orbital bands
• Excellent band flatness.
![Page 16: Part II. p-orbital physics in optical lattices](https://reader033.vdocuments.us/reader033/viewer/2022042403/625d8000c02011623a550e89/html5/thumbnails/16.jpg)
16
Exact solution for spinless fermions: Wigner crystallization
6
1n
• The result is also good for bosons.
• Close-packed hexagons; avoiding repulsion.
• The crystalline ordered state is stable even with small .t
gapped state
![Page 17: Part II. p-orbital physics in optical lattices](https://reader033.vdocuments.us/reader033/viewer/2022042403/625d8000c02011623a550e89/html5/thumbnails/17.jpg)
17
Orbital ordering with strong repulsions
10/ // tU
2
1n
• Various orbital ordering insulating states at commensurate fillings.
• Dimerization at <n>=1/2! Each dimer is an entangled state of empty and occupied states.
![Page 18: Part II. p-orbital physics in optical lattices](https://reader033.vdocuments.us/reader033/viewer/2022042403/625d8000c02011623a550e89/html5/thumbnails/18.jpg)
18
C. Wu, PRL 101, 186807 (2008).
Zhang, Hung, Zhang, Wu, PRA 83, 023615 (2011).
Exotic quantum anomalous Hall insulators
The required experimental technique was available in Nate Gemelke and Steven Chu’s group at Stanford.
c.f. Condensed matter systems: Nagaosa et al,
Na2IrO3, PRL 2009; Fang and Dai, science 2010.
Ir4+
![Page 19: Part II. p-orbital physics in optical lattices](https://reader033.vdocuments.us/reader033/viewer/2022042403/625d8000c02011623a550e89/html5/thumbnails/19.jpg)
19
• Landau levels quantization from external magnetic fields.
A brief review: quantum Hall effect (QHE)
• Insulating bulk with chiral gapless edge modes. Quantized Hall conductance; dissipationless charge transport through edge states.
BQuantum Hall state
• Haldane: Landau level is not necessary for QHE. The key point is the non-trivial wavefunction topology ---- 1st Chern number.
![Page 20: Part II. p-orbital physics in optical lattices](https://reader033.vdocuments.us/reader033/viewer/2022042403/625d8000c02011623a550e89/html5/thumbnails/20.jpg)
h
en
dddkde
yx k
FBZ
k
H
xy
2
2
2
2
)ˆˆ.(ˆ8
1
p
s
Quantum Anomalous Hall (QAHE)– QHE without Landau levels
• Example: a two-band system. The pseudo-spin vector exhibits a non-trivial configuration in the Brillouin zone.
20X. L Qi, et al, PRB 74,85308 (2006)
xk
yk
)()()(
)()()()()(
321
213
kdkidkd
kidkdkdkdkH
)coscos2()(
,sin)(,sin)(
3
21
yx
yx
kkmkd
ktkdktkd
d
• Hall conductance is quantized to n/2p.
![Page 21: Part II. p-orbital physics in optical lattices](https://reader033.vdocuments.us/reader033/viewer/2022042403/625d8000c02011623a550e89/html5/thumbnails/21.jpg)
Haldane’s Quantum Anomalous Hall model
• Topological insulator if . Mass changes sign at K1,2.
p ,01K 2K
• Honeycomb lattice with complex-valued next-nearest neighbor hopping.
..)()({ chrcrctH B
Ar
ANN
.}.
)()()()({
ch
rcrcercrcetHBB
i
rAA
i
NNN
21
A
Bt
iet
• QAHE has not been experimentally realized yet in both CM and AMO systems.
F. D. M. Haldane, Phys. Rev. Lett. 61, 2015 (1988)
![Page 22: Part II. p-orbital physics in optical lattices](https://reader033.vdocuments.us/reader033/viewer/2022042403/625d8000c02011623a550e89/html5/thumbnails/22.jpg)
Rotate each site around its own center
N. Gemelke • Phase modulation on laser beams: a fast overall oscillation of the lattice. Atoms cannot follow and feel a slightly distorted averaged potential.
• The oscillation axis slowly precesses at the angular frequency of .)()()()({
)(
rprprprpi
rLH
xyyAr
x
Arzzmn
• Orbital Zeeman term.
22
![Page 23: Part II. p-orbital physics in optical lattices](https://reader033.vdocuments.us/reader033/viewer/2022042403/625d8000c02011623a550e89/html5/thumbnails/23.jpg)
Large rotation angular velocity
2/)( 23/2 pitet
• The second order perturbation generates the NNN complex hopping.
//t
ipp
ipp
6
pi
e
6
5pi
e
ipp
ipp
ipp
23
//t
ipp
ipp
ipp
p3/2itep3/2ite
![Page 24: Part II. p-orbital physics in optical lattices](https://reader033.vdocuments.us/reader033/viewer/2022042403/625d8000c02011623a550e89/html5/thumbnails/24.jpg)
Small rotation angular velocity
0//3.0 t
1C
0C
Berry curvature and Chern numbers
1
0
0
1C
24
![Page 25: Part II. p-orbital physics in optical lattices](https://reader033.vdocuments.us/reader033/viewer/2022042403/625d8000c02011623a550e89/html5/thumbnails/25.jpg)
25
Large rotation angular velocity
//2
3t
//3t
1C
1C
Berry curvature.
1C
11
125
![Page 26: Part II. p-orbital physics in optical lattices](https://reader033.vdocuments.us/reader033/viewer/2022042403/625d8000c02011623a550e89/html5/thumbnails/26.jpg)
2
1
1
2
3
2 density profile: local density approx. works well.
Soft confining potential: exact diagonalization for the non-interacting system
• Density plateaus in the insulating regimes.
• Metallic region between density plateaus.
22
02
1)( rmrVt
)()( rVrtr
26
![Page 27: Part II. p-orbital physics in optical lattices](https://reader033.vdocuments.us/reader033/viewer/2022042403/625d8000c02011623a550e89/html5/thumbnails/27.jpg)
Equilibrium Anomalous Hall currents in the trap
27
![Page 28: Part II. p-orbital physics in optical lattices](https://reader033.vdocuments.us/reader033/viewer/2022042403/625d8000c02011623a550e89/html5/thumbnails/28.jpg)
conductance profile
Quantized and non-quantized Hall conductance
• Normalized conductance is quantized in the plateaus.
),(2
/ )(
yxnn
r
rV
HkkBdk
h
mj tr
ps
• Metallic regime: reversed Hall current. Extra contribution from Hall diffusion current.
)(ln))(()(
)(/)]())([(
)(
rErr
rnrnErF
FFj
rbr
br
diffdriftHH
s
28
![Page 29: Part II. p-orbital physics in optical lattices](https://reader033.vdocuments.us/reader033/viewer/2022042403/625d8000c02011623a550e89/html5/thumbnails/29.jpg)
29
• Orbital exchange in the Mott-insulating state; orbital frustration: quantum 120 degree model; solvable quantum orbital ice.
Outline
C. Wu, PRL 100, 200406 (2008).; G-W Chern, C. Wu, arix1104.1614
A B
B
B)ˆ()ˆ(
11ee
)ˆ)(ˆ(22
ee
)ˆ)(ˆ(33
ee
c.f. Khaliullin et al, PRL 2009
![Page 30: Part II. p-orbital physics in optical lattices](https://reader033.vdocuments.us/reader033/viewer/2022042403/625d8000c02011623a550e89/html5/thumbnails/30.jpg)
Mott insulator of SPINLESS fermions: orbital exchange
)()(int
rnrnUHyx p
rp
U
30
• Pseudo-spin representation.
)(2
1
1 yyxx pppp )(2
1
2 xyyx pppp )(23 xyyx
ipppp
• Orbital exchange: no orbital flipping process.
0J
UtJ /2 2
UtJ /2 2
)ˆ()( 11 xrrJH ex
![Page 31: Part II. p-orbital physics in optical lattices](https://reader033.vdocuments.us/reader033/viewer/2022042403/625d8000c02011623a550e89/html5/thumbnails/31.jpg)
• Non-triviality: Ising quantization axis depends on bond orientation. For a bond along the general direction ,
xp
: eigen-states of yxe 2sin2cosˆ2
e
2e
)ˆ)ˆ()(ˆ)(( 22 eererJHex
Hexagon lattice: quantum model120
)ˆ)(()ˆ)((,
ijjiji
rr
ex ererJH
• After a suitable transformation, the Ising quantization axes can be chosen just as the three bond orientations.
A B
B
B
11 ))(( 22
3
12
1
22
3
12
1
))(( 22
3
12
1
22
3
12
1
ypyx pp ,
31
C. Wu et al, arxiv0701711v1; C. Wu, PRL
100, 200406 (2008). E. Zhao, and W. V.
Liu, Phys. Rev. Lett. 100, 160403 (2008)
![Page 32: Part II. p-orbital physics in optical lattices](https://reader033.vdocuments.us/reader033/viewer/2022042403/625d8000c02011623a550e89/html5/thumbnails/32.jpg)
From the Kitaev model to 120 degree model
A B
B
B
xxssyy
ss
zzss
• cf. Kitaev model: Ising quantization axes form an orthogonal triad.
))()(
)()()()((
3
21
err
errerrJH
zz
yyxx
Ar
kitaev
ss
ssss
Kitaev
cos02
1
120
32
120
![Page 33: Part II. p-orbital physics in optical lattices](https://reader033.vdocuments.us/reader033/viewer/2022042403/625d8000c02011623a550e89/html5/thumbnails/33.jpg)
33
Large S picture: heavy-degeneracy (frustration) of classic ground states
• Ground state constraint: the two -vectors have the same projection along the bond orientation.
or
rzrr
rrex
rJerrJH )(}ˆ)]()({[( 22
,
• Ferro-orbital configurations. • Loop config: -vectors along the tangential directions.
![Page 34: Part II. p-orbital physics in optical lattices](https://reader033.vdocuments.us/reader033/viewer/2022042403/625d8000c02011623a550e89/html5/thumbnails/34.jpg)
Heavy-degeneracy of the classic ground states
• General loop configurations
34
![Page 35: Part II. p-orbital physics in optical lattices](https://reader033.vdocuments.us/reader033/viewer/2022042403/625d8000c02011623a550e89/html5/thumbnails/35.jpg)
35
Global rotation degree of freedom
• Each loop config remains in the ground state manifold by a suitable arrangement of clockwise/anticlockwise rotation patterns.
![Page 36: Part II. p-orbital physics in optical lattices](https://reader033.vdocuments.us/reader033/viewer/2022042403/625d8000c02011623a550e89/html5/thumbnails/36.jpg)
36
“Order from disorder”: 1/S orbital-wave correction
![Page 37: Part II. p-orbital physics in optical lattices](https://reader033.vdocuments.us/reader033/viewer/2022042403/625d8000c02011623a550e89/html5/thumbnails/37.jpg)
37
Zero energy flat band orbital fluctuations
42 )(6 JSE
• Each un-oriented loop has a local zero energy model up to the quadratic level.
• The above config. contains the maximal number of loops, thus is selected by quantum fluctuations at the 1/S level.
• Project under investigation: the quantum limit (s=1/2)? A very promising system to arrive at orbital liquid state? What is the physics after doping? Add rotation Topo Mott Insulator.
![Page 38: Part II. p-orbital physics in optical lattices](https://reader033.vdocuments.us/reader033/viewer/2022042403/625d8000c02011623a550e89/html5/thumbnails/38.jpg)
38
Outline
• Orbital bosons: unconventional BEC beyond the “no-node” theorem.
• Orbital fermions in the hexagonal lattice.
• Introduction: orbital physics is an interesting research direction of cold atoms.
Ferromagnetism from band flatness.
The unconventional f-wave Cooper pairing of the spinless fermions.
W. C. Lee, C. Wu, S. Das Sarma, arXiv:0905.1146, to appear in PRA.
![Page 39: Part II. p-orbital physics in optical lattices](https://reader033.vdocuments.us/reader033/viewer/2022042403/625d8000c02011623a550e89/html5/thumbnails/39.jpg)
39
Conventional v.s. unconventional Cooper pairings
• Conventional superconductivity:
k
k
s-wave: pairing amplitude does not
change over the Fermi surface.
• d-wave (high Tc cuprates). Pairing amplitude changes sign on the Fermi surface.
22 yxd
++
--
--
k
k
![Page 40: Part II. p-orbital physics in optical lattices](https://reader033.vdocuments.us/reader033/viewer/2022042403/625d8000c02011623a550e89/html5/thumbnails/40.jpg)
40
Unconventional Cooper pairing
p-wave: superfluid 3He-A and B; Sr2RuO4;
d-wave: high Tc cuprates;
Extended s-wave: iron-pnictide superconductors (?);
• Most of unconventional pairing states arise from strong correlation effects. Predictions and analysis are difficult.
• Can we arrive at unconventional pairing in a simpler way, say, from nontrivial band structures but with conventionalinteractions?
• No strong correlation effects. Analysis is controllable.
• f-wave pairing with spinless fermions in the p-orbital hexagonal optical lattice.
C. W. Zhang et al., Phys. Rev. Lett. 101, 160401 (2008).
![Page 41: Part II. p-orbital physics in optical lattices](https://reader033.vdocuments.us/reader033/viewer/2022042403/625d8000c02011623a550e89/html5/thumbnails/41.jpg)
41
Nontrivial orbital configurations between time reversal (TR) partners
• Along the three middle lines of Brillouin zone, eigen-orbitals are real.
• At K and K’, eigen-orbitals are complex and orthognoal.
K K
yxipp
yxipp
yxipp
yxipp
k
k
A
B
A
B
A
B
A
B
![Page 42: Part II. p-orbital physics in optical lattices](https://reader033.vdocuments.us/reader033/viewer/2022042403/625d8000c02011623a550e89/html5/thumbnails/42.jpg)
The f-wave structure because of the symmetry reason
• Along middle lines, TR pairs cannot be paired nodal lines.
• The TR pair at K and K’ has the largest pairing.
• Odd parity.nodal lines
• The mean-field gap value can reach 10nK; and the 2D Kosterlitz-Thouless temperature can reach 1nK.
42
K K
yxipp
yxipp
yxipp
yxipp
k
k
A
B
A
B
A
B
A
B
![Page 43: Part II. p-orbital physics in optical lattices](https://reader033.vdocuments.us/reader033/viewer/2022042403/625d8000c02011623a550e89/html5/thumbnails/43.jpg)
43
Phase sensitive detection: zero energy Andreev bound states
inkout
k
in
k
outk
With zero energy Andreev Bound States
No Andreev Bound States
![Page 44: Part II. p-orbital physics in optical lattices](https://reader033.vdocuments.us/reader033/viewer/2022042403/625d8000c02011623a550e89/html5/thumbnails/44.jpg)
• Strong correlation effect from band flatness: Exact results of Wigner crystal and ferromagnetism.
• Mott-insulator: a new type of frustrated magnet-like model.
• Band insulator (topological): quantum anomalous Hall effect.
• Novel mechanism for the f-wave Cooper pairing.
44
Summary: p-orbital fermions in the honeycomb lattice – Novel physics beyond graphene