nuclear data sheets for a = 222
TRANSCRIPT
Sukhjeet SinghDepartment of Physics, Maharishi Markandeshwar University,
Mullana, Haryana 133207, India
A. K. JainDepartment of Physics, Indian Institute of Technology,
Roorkee, Uttarakhand 247667, India
Jagdish K. TuliNational Nuclear Data Center, Brookhaven National
Laboratory, Upton, NY 11973 USA
(Received April 4, 2011; Revised October 14, 2011)
A b s t r a c t : T h e E N S D F e v a l u a t i o n f o r A = 2 2 2 m a s s c h a i n ( 1 9 9 6 E l 0 1 ) h a s b e e n u p d a t e d o n t h e b a s i s o f t h e
exper imenta l r esu l t s , s ince September 1995 ( l i t e ra ture cu to f f da te in 1996El01 ) , f r om var i ous reac t i on and
decay studies for all nuclides in A=222 mass chain (Z=84 to 92). A new nuclide (222Po) has since been observed.
In addition, new measurements have been reported in Rn, Th and Ra nuclides. The results obtained from various
theoret ical studies are g iven as comments . The updated level and decay schemes, and experimental decay and
reaction data on which they are based, are summarized and presented for all the nuclides with mass number A=
222. The adopted values o f level energies , leve l spins and par i t ies are g iven, and γ–ray energies , intensi t ies ,
as wel l as other nuclear properties are presented. The references, Jπ arguments, and necessary comments are
given in the text. All Q values have been adopted from 2011AuZZ. Theoretical work of 2009Mo27 was consulted.
Cutoff Date: March 31, 2011.
General Policies and Organization of Material: See the January issue of the Nuclear Data Sheets or
http: / /www.nndc.bnl.gov/nds/NDSPolicies.pdf.
Acknowledgments: Support from J.K. Sharma (M.M. University, Mullana, India) and BirBikram Singh (Institute of
Physics,Bhubaneswar, India) is gratefully acknowledged.
Nuclear Data Sheets for A = 222*
* The work at M.M. University, Mullana, India and at IIT Roorkee, Roorkee, India was supported by the Department
of Science and Technology, India.
Available online at www.sciencedirect.com
Nuclear Data Sheets 112 (2011) 2851–2886
0090-3752/$ – see front matter © 2011 Elsevier Inc. All rights reserved.
www.elsevier.com/locate/nds
doi:10.1016/j.nds.2011.10.002
2 8 5 2
NUCLEAR DATA SHEETS
Index for A = 222
Nuclide Data Type Page
Skeleton Scheme for A=222 2854222Po Adopted Levels 2856222At Adopted Levels 2856222Rn Adopted Levels, Gammas 2857
226Ra α Decay 2860
(HI,xnγ ) 2862222Fr Adopted Levels 2863
226Ac α Decay 2863222Ra Adopted Levels, Gammas 2864
222Fr β– Decay 2868226Th α Decay 2871232Th(136Xe,Xγ ) 2873
222Ac Adopted Levels 2874226Pa α Decay 2874
222Th Adopted Levels, Gammas 2875226U α Decay 2878
(HI,xnγ ) 2878222Pa Adopted Levels 2880
226Np α Decay 2880222U Adopted Levels 2881
2 8 5 4
NUCLEAR DATA SHEETS
Skeleton Scheme for A=222
0+ 0.0
550 s22
824Po138
Q– unknown
100%
0.0
54 s
S(n) 4090SY
228
25At137
Q–=4430SY
100%
0+ 0.0
3.8235 d
S(n) 61706
S(p) 7730SY
228
68Ra138
Qα=4870.6225100%
0+ 0.0
1600 y
228
26Rn136
Q–=2421
Qα=5590.33
100%
2– 0.0
14.2 min
S(n) 500022S(p) 541222
228
69Ac137
Qα=5536216×10–3% 2
(1) 0.0
29.37 h
228
27Fr135
Q–=202822
100%
0+ 0.0
38.0 s
S(p) 62466
S(n) 67146
229
60Th136
Qα=6450.922100%
0+ 0.0
30.57 min
228
28Ra134
Qα=66794
99% 11% 1
1– 0.0
5.0 s
0.0+x
S(p) 36317
S(n) 597050
229
61Pa135
Qα=69871074% 5
0.0
1.8 min
228
29Ac133
Q+=23007
Qα=7137.420
100%
0+ 0.0
2.8 ms
S(p) 461050
S(n) 780615
229
62U134
Qα=771514100%
0+ 0.0
0.35 s
229
20Th132
Q+=58213
Qα=81275
100%
0.0
2.9 ms
S(p) 2110SY
S(n) 6340SY
229
63Np133
Qα=820050100%
0.0
35 ms
229
21Pa131
Q+=4910SY
Qα=8850SY
2 8 5 5
NUCLEAR DATA SHEETS
Skeleton Scheme for A=222 (continued)
100%
0+ 0.0
1.0 μs
S(p) 3370SY
S(n) 8360SY
229
22U130
Q+=2180SY
Qα=9500SY
Ground–State and Isomeric–Level Properties
Nuclide Level Jπ T1/2 Decay Modes
222Po 0.0 0+ 550 s 430222At 0.0 54 s 10 %β–=100222Rn 0.0 0+ 3.8235 d 3 %α=100222Fr 0.0 2– 14.2 min 3 %β–=100222Ra 0.0 0+ 38.0 s 5 %α=100222Ac 0.0 1– 5.0 s 5 %α=99 1 ; %ε+%β+=1 1
0.0+x 63 s 3 %α≥88; %IT≤10; 0.7≤%ε+%β+≤2222Th 0.0 0+ 2.8 ms 3 %α=100222Pa 0.0 2.9 ms +6–4 %α=100222U 0.0 0+ 1.0 μs +12–4 %α=100226Ra 0.0 0+ 1600 y 7 %α=100226Ac 0.0 (1) 29.37 h 12 %α=6×10–3 2; . . .226Th 0.0 0+ 30.57 min 10 %α=100226Pa 0.0 1.8 min 2 %α=74 5 ; . . .226U 0.0 0+ 0.35 s 15 %α=100226Np 0.0 35 ms 10 %α=100
2 8 5 6
228
24Po138
228
24Po138NUCLEAR DATA SHEETS
Adopted Levels
See 2010Ch19 for 222Po isotope discovery and its mass measurements in the fragmentation of 238U beam at 670
MeV/nucleon with a 4g/cm2 9Be target fol lowed by separation by Fragment Recoil Separator facil ity at GSI.
Fragments were then injected into the cooler electron storage ring ESR. The mass and half–li fe was measured by
t ime–resolved Schottky Mass spectrometry technique. For the measurements of isotopic distributions of the
cross–sections, see 2010Al24.
222Po Levels
E(level) Jπ T1/2 Comments
0 . 0 0 + 5 5 0 s 4 3 0 T1/2: Uncertainty symmetrized (by evaluators) from the quoted value of 145 s +694–66 (2010Ch19).
Measured mass excess=22476 keV 67 (2010Ch19).
228
25At137 22
825At137
Adopted Levels
Q(β–)=4430 SY ; S(n)=4090 SY ; Q(α )=5040 SY 2003Au03,2011AuZZ.
Estimated: ΔQ(β–)=300, ΔS(n)=360, ΔQ(α )=200 (2003Au03,2011AuZZ).
The nucleus was produced by 1989Bu09 in 232Th (600–MeV p) by spallation with a negative ion source where chemically
pure beams of halogen elements were produced; the products were mass separated. The measured half–lives provided
the information for the definite nuclear assignment of the products.
The calculations of 1973Ta30 by using the β–gross theory yielded T1/2≈100 s for the β decay half–li fe of 222At;
1984Kl06 calculated this half–li fe as 21.5 s by using a microscopic theory. 2010Li02 measured mass values using
Schottky mass spectrometry.
See 2010Al24 for measurement of production cross–section using cold–fragmentation at relativistic energies.
222At Levels
E(level) T1/2 Comments
0 . 0 5 4 s 1 0 %β–=100.
Only β– decay was observed.
T1/2: measured by 1989Bu09.
2 8 5 7
228
26Rn136–1 22
826Rn136–1NUCLEAR DATA SHEETS
Adopted Levels, Gammas
Q(β–)=24 21 ; S(n)=6170 6 ; S(p)=7730 SY ; Q(α )=5590.3 3 2003Au03,2011AuZZ.
Estimated ΔS(p)=200 (2003Au03,2011AuZZ).
Potential energy and equilibrium deformations were calculated by 1994Li05, 1988So08, 1984Na22, 1983Ro14, 1982Le19,
1981Gy03. The nuclear binding energies were calculated and incipiency of deformation in this region is discussed
in 1986Ch23.
See 1983Ro14 for calculations of static quadrupole and hexadecapole moments.
2010Li02 measures mass values using Schottky mass spectrometry.
See 2009Qi07, 2004Re22 for predictions of cluster decay and its half–li fe. See 1989De11 for discussions on octupole
deformation and E1 transitions.
See 1987Ro08 for calculation of single–particle states and dipole moments as a function of octupole deformation, and
for B(E1)/B(E2) values at the equilibrium octupole deformation.
Higher order of deformations were considered by 1995De13; the level energies of the 2+, 4+ states in the g.s. band
and the 1–,3– states in the octupole–vibrational band were calculated. See 1995De13 for calculations, discussions
and comparison with experiments. See 1998Ra05 for calculations of level energies. Others: 2001Za04, 2001Za09. See
2003Ga34 for calculations of ground state properties.
222Rn Levels
The Kπ=0+ g.s. band and the Kπ=0– band at 600.66 keV have been interpreted as octupole parity–doublet bands. This
nucleus falls in the middle of the region of octupole deformation defined by the spin systematics for octupole
shapes (1990Ja11).
Cross Reference (XREF) Flags
A 226Ra α Decay
B (HI,xnγ )
E(level) Jπ† XREF T1/2 Comments
0 . 0 ‡ 0 + AB 3 . 8 2 3 5 d 3 %α=100.
%β–<1×10–4 for Eβ–=40 for log f1ut>8.5.
See 1986De32, 1986Ir01, 1986Pi11 for the calculations of partial half–li fe for 14C decay.
T1/2: from 1972Bu33, measured to ≈40 half–lives. Recent measurement: 3.8195 d 30
(2004Sc04) fol lowed to ≤5.2 half–lives. Other measurements: 3.825 d 5
(1951To25), 3.8229 d 17 (1956Ma64), 3.825 d 4 (1956Ro31), 3.83 d 3 (1958Sh69).
1 8 6 . 2 1 1 ‡ 1 3 2 + AB 0 . 3 2 n s 2 μ=+0.92 14 (2005St24,1970Or02).
See 1970Or02 for Gyromagnetic ratio g=0.45 7 by αγ (θ ,H).
T1/2: by (α ) (γ ) (t) (1960Be25). Other measurement: 0.31 ns (1961Fo08).
4 4 8 . 3 7 ‡ 1 2 4 + AB (α ) (262γ ) (θ ) data of 1989Po03 rule out J of 0, 1, 2 and 3. Jπ≠4– by requiring
parity conservation for the α transition from the 0+ parent.
6 0 0 . 6 6 § 5 1 – AB Jπ : γ to g.s . ; the (α ) (601γ ) (θ ) and (α ) (415γ ) (θ ) data rule out 2; Jπ≠1+ from the
parity–conservation requirement in α decays.
6 3 5 . 4 7 § 1 5 3 – AB (α ) (449γ ) (θ ) data of 1989Po03 rules out 0, 1, 2 and 4; Jπ≠1+, 2– by requiring
parity conservation in α decay from its 0+ parent.
7 6 8 . 5 ‡ 4 ( 6 + ) B
7 9 7 . 8 § 6 ( 5 – ) B
1 0 4 9 . 2 § 6 ( 7 – ) B
1 1 2 8 . 1 ‡ 4 ( 8 + ) B
1 3 5 6 . 9 § 6 ( 9 – ) B
1 5 1 3 . 0 ‡ 5 ( 1 0 + ) B
1 7 0 8 . 2 § 6 ( 1 1 – ) B
1 9 1 3 . 4 ? ‡ 6 ( 1 2 + ) B
2 0 8 9 . 1 § 8 ( 1 3 – ) B
2 3 1 7 . 2 ? ‡ 8 ( 1 4 + ) B
2 4 8 5 . 3 ? § 8 ( 1 5 – ) B
2 7 2 7 . 7 ? ‡ 9 ( 1 6 + ) B
2 8 8 1 . 9 ? § 1 0 ( 1 7 – ) B
3 2 8 5 . 9 ? § 1 1 ( 1 9 – ) B
3 6 9 6 . 1 ? § 1 2 ( 2 1 – ) B
† All levels above 635 based on band assignments in (HI,xnγ ) .
‡ (A): Kπ=0+ g.s. band.
§ (B): Kπ=0– octupole vibrational band.
2 8 5 8
228
26Rn136–2 22
826Rn136–2NUCLEAR DATA SHEETS
Adopted Levels, Gammas (continued)
γ (222Rn)
E(level) Eγ† Iγ‡ Mult.§ α I(γ+ce) Comments
1 8 6 . 2 1 1 1 8 6 . 4 2 1 0 0 1 5 E2 0 . 6 9 2 1 6 9 2 5 B(E2)(W.u.)=58 4 .
4 4 8 . 3 7 2 6 2 . 5 2 1 3 4 2 0 E2 1 6 2 1 0
6 0 0 . 6 6 4 1 4 . 6 0 5 6 0
6 0 0 . 6 6 5 1 0 0 E1 Mult. : assigned by evaluators, only E1 decay is possible.
6 3 5 . 4 7 4 4 8 . 6 5
7 6 8 . 5 3 1 9 . 6 2 1 1 8 2 6 E2 1 3 2 2 9
7 9 7 . 8 1 6 3 . 0 # 5
3 4 8 . 9 # 5
1 0 4 9 . 2 2 5 1 . 4 # 5
2 8 0 . 6 5 2 5 7 E1 2 6 7
1 1 2 8 . 1 3 5 9 . 6 2 7 5 1 4 E2 8 1 1 5
1 3 5 6 . 9 2 2 8 . 8 5 2 3 1 3 E1 2 4 1 4
3 0 7 . 7 5 3 1 1 3 E2 3 5 1 5
1 5 1 3 . 0 3 8 4 . 9 2 4 0 1 1 E2 4 3 1 1
1 7 0 8 . 2 1 9 5 . 4 5 2 2 1 4 E1 2 4 1 5
3 5 1 . 2 5 4 6 1 4 E2 5 0 1 5
1 9 1 3 . 4 ? 4 0 0 . 4 # 5
2 0 8 9 . 1 1 7 5 . 6 # 5
3 8 0 . 9 5 1 5 8 E2 1 6 9
2 3 1 7 . 2 ? 4 0 3 . 8 # 5
2 4 8 5 . 3 ? 3 9 6 . 3 # 5
2 7 2 7 . 7 ? 4 1 0 . 5 # 5
2 8 8 1 . 9 ? 3 9 6 . 6 # 5
3 2 8 5 . 9 ? 4 0 4 . 0 # 5
3 6 9 6 . 1 ? 4 1 0 . 2 # 5
† All γ properties are from 226Ra α decay.
‡ Relative photon intensity deexciting the level .
§ From GAMMASPHERE data (1999Co02).
# Placement of transition in the level scheme is uncertain.
(A) Kπ=0+ g.s. band
(B) Kπ=0- octupolevibrational band
0.00+
186.2112+
448.374+
768.5(6+)
1128.1(8+)
1513.0(10+)
1913.4(12+)
2317.2(14+)
2727.7(16+)
186
262
320
360
385
400
404
410
600.661-
635.473-
797.8(5-)
1049.2(7-)
1356.9(9-)
1708.2(11-)
2089.1(13-)
2485.3(15-)
2881.9(17-)
3285.9(19-)
3696.1(21-)
163
251
308
351
381
396
397
404
410
222
86Rn136
2 8 5 9
228
26Rn136–3 22
826Rn136–3NUCLEAR DATA SHEETS
2 8 6 0
228
26Rn136–4 22
826Rn136–4NUCLEAR DATA SHEETS
226Ra αααα Decay
Parent 226Ra: E=0.0; Jπ=0+; T1/2=1600 y 7 ; Q(g.s. )=4870.62 25 ; %α decay=100.
Eα (g.s . )=4784.34 25 gives Q(α ) (226Ra)=4870.54 25 ; from their mass adjustment, 2003Au03, 2011AuZZ recommend
Q(α ) (226Ra)=4870.62 25 ; the input value is l isted as Q(α )=4870.70 25 .
α γ ( θ ) : 1 9 8 9 P o 0 3
E γ E ( l e v e l ) d e d u c e d J π r e j e c t e d s p i n s
– – – – – – – – – – – – – – – – – – – – – – – – – – – – – – – – – – – – – – – – –
2 6 2 4 4 8 4 + 0 , 1 , 2 , 3
4 1 4 6 0 1 1 – 2 , 3
6 0 1 6 0 1 1 – 2 , 3
4 4 9 6 3 5 3 – 0 , 1 , 2 , 4
O t h e r α γ ( θ ) me a s u r eme n t s : 1 9 5 4R o 0 6 , 1 9 5 4Mi 5 3 .
( α ) ( α ) ( θ ) :
( 2 2 6Ra a ) ( 2 2 2Rn a ) ( θ ) : 1 9 6 8B i 0 8 o b s e r v e d i s o t r o p i c c o r r e l a t i o n .
α γ ( θ , H ) : s e e 1 9 7 0O r 0 2 , 1 9 7 4O r 0 2 .
α γ ( t ) : T 1 / 2 ( 1 8 6 l e v e l ) = 0 . 3 2 n s 2 ( 1 9 6 0B e 2 5 ) .
See 1994Da26 for Bremsstrahlung emission accompanying the 226Ra α decay.
222Rn Levels
E(level) Jπ T1/2
0 . 0 0 +
1 8 6 . 2 1 1 1 3 2 + 0 . 3 2 n s 2
4 4 8 . 3 7 1 2 4 +
6 0 0 . 6 6 5 1 –
6 3 5 . 4 7 1 5 3 –
α radiations
See 1992De44, 1987Be43, 1986Ch36, 1977Ba70, 1996De19 for theoretical calculations of α–decay widths.
Eα† E(level) Iα‡# HF§ Comments
4 1 6 0 2 6 3 5 . 4 7 0 . 0 0 0 2 7 5 8 . 6 1 6
4 1 9 1 2 6 0 0 . 6 6 0 . 0 0 1 0 1 4 . 4 5 Eα : 4194.4 3 from level energy and Eα (to g.s. ) .
4 3 4 0 1 4 4 8 . 3 7 0 . 0 0 6 5 3 1 0 . 3 5
4 6 0 1 1 1 8 6 . 2 1 1 6 . 1 6 3 0 . 8 5 7 6 Eα : the original energy has been increased by 3 keV, as recommended by
1991Ry01, because of a change in the calibration energy. I(α ) from
2007Ne01 Eα=4601.7 2 was recommended by 1983Co22 and 1987El01 from
measurements of 1958Wa16. Eα=4601.43 26 from Eα (g.s . )=4784.34 25 and
E(level) .
4 7 8 4 . 3 4 2 5 0 . 0 9 3 . 8 4 1 1 1 . 0 Eα : from 1971Gr17. The original energy has been decreased by 0.16 keV, as
recommended by 1991Ry01. Other measurements 1996Wi27. I(α ) from 2007Ne01.
† From 1963Ba62, except where otherwise noted. Other measurements: 1958Wa16, 1953Ba29, 1949Ro08.
‡ α intensity per 100 α decays; Iα ' s are from 1963Ba62. The uncertainties on 4784.34α and 4601α are given as recommended by
1991Ry01.
§ HF(4784α )=1.0 gives r0(222Rn)=1.5397 3 .
# Absolute intensity per 100 decays.
γ (222Rn)
γγ : 1971Lo19. For calculated alpha decay l i fe t ime see 2005Sh42, 2006Xu04, 2007Pe30, 2009Ni06, 2009De32.
EㆠE(level) Comments
( 3 4 . 8 1 6 ) 6 3 5 . 4 7 Eγ : transition was not observed; its energy is from the level scheme.
Continued on next page (footnotes at end of table)
2 8 6 1
228
26Rn136–5 22
826Rn136–5NUCLEAR DATA SHEETS
226Ra αααα Decay (continued)
γ (222Rn) (continued)
Eγ† E(level) Iγ‡ Mult. α Comments
1 8 6 . 2 1 1 1 3 1 8 6 . 2 1 1 3 . 6 4 4 E2 0 . 6 9 3 Eγ : from 1993Di09 and 1977Zo01. Other measured energies: 186.0 1
(1969Li10), 185.97 5 (1971Lo19), 186.196 12 (1974AlZT), 185.8 2
(1975Ha31), 186.19 10 (1976De48), 186.19 16 (1982Ak03). Earlier
measurements: 1951Co15, 1960St20, 1964Ew04.
Iγ : absolute photon intensity per 100 226Ra α decays, as measured by
2001La14. Other absolute measurements: 3.50 5 (1983Ol01), 3.51 6
(1983Sc13), 3.29 3 (1983Co22), 3.59 6 (1991Li11).
Iγ=3.28 3 from intensity balance at the 186–keV level .
Other values: Iγ (186γ ) /Iγ (609γ of 214Bi in equilibrium)= 0.0858 5
(1993Di09), 0.0823 3 (1983Bu14), 0.092 10 (1982Ak03), 0.0907 14
(1982Fa10), 0.076 4 (1981We18), 0.0900 11 (1977Zo01), 0.087 15
(1975Ha31), 0.0820 12 (1970Mo28), 0.079 8 (1964Ew04). Iγ (609γ of 214Bi in equilibrium)=46.1% 5 is adopted in the Nuclear Data
Sheets for A=214. Other Iγ measurements: 1976De48, 1974AlZT,
1969Li10, 1969Wa27, 1969Gr33, 1967Ma51.
Mult. : from ce ratios measured by 1963Go21, 1955Ju14, 1954Ro05.
1973De50 α (K)=0.200 9 , α (L)=0.380 20 were deduced by 1973De50 from
I(K x ray)/I(186γ ) , I (L x ray)/I(186γ ) .
( 1 8 7 . 1 0 2 0 ) 6 3 5 . 4 7 Eγ : transition was not observed; its energy is from the level scheme.
I(γ+ce)(34.8γ )+I(γ+ce)(187.1γ )=0.0008 from the intensity balance at
the 635.47–keV level ; the intensity balance at the 448.37–keV
level yields I(γ+ce)(187.1γ )=0.0061 6–0.0065 3 . See the section on 222Rn adopted levels, gammas for the references where E1
transition probabil it ies and E1/E2 ratios were calculated and
discussed in terms of octupole deformations.
2 6 2 . 2 7 5 4 4 8 . 3 7 0 . 0 0 5 0 5 [ E2 ] 0 . 2 1 2 Iγ : from Iγ (262γ ) /Iγ (186γ )=0.0014 2 (1993Di09,1971Lo19). Other
measured ratios: 0.0029 (1960St20), 0.0025 (1956Ha71).
I(262γ )=0.0054 3 from I(4340α )=0.0065 3 and α (262γ )=0.212.
4 1 4 . 6 0 5 6 0 0 . 6 6 0 . 0 0 0 3 0 [ E1 ] 0 . 0 1 6 4 Iγ : from Iγ (414.6γ ) /Iγ (186γ )=0.000086 (1971Lo19). Other measured
ratio: 0.00021 (1960St20).
4 4 9 . 3 7 1 0 6 3 5 . 4 7 0 . 0 0 0 1 9 [ E1 ] 0 . 0 1 3 8 Iγ : from Iγ (449γ ) /Iγ (186γ )=5.5×10–5 (1971Lo19). Other measured
ratio: 9×10–5 (1960St20).
6 0 0 . 6 6 5 6 0 0 . 6 6 0 . 0 0 0 4 9 [ E1 ] 0 . 0 0 7 6 6 Iγ : from Iγ (600γ ) /Iγ (186γ )=0.00014 (1971Lo19). Other measured ratio:
0.00033 (1960St20).
† From 1971Lo19, except where noted otherwise. Other measurements: 1960St20, 1956Ha71.
‡ Absolute intensity per 100 decays.
0+ 0.0 1600 y
%α=100228
68Ra138
Qα=4870.6225
0+ 0.0 1.093.844784.34
2+ 186.211 0.32 ns 0.8576.164601
4+ 448.37 10.30.00654340
1– 600.66 4.40.00104191
3– 635.47 8.60.000274160
HFIαEα
Decay Scheme
Intensities: I(γ+ce) per 100
decays by this branch
186.
211
E2
6.1
6
262.
27 [
E2]
0.
0061
414.
60 [
E1]
0.
0003
0
600.
66 [
E1]
0.
0004
9
34.8
187.
10
449.
37 [
E1]
0.
0001
9
228
26Rn136
2 8 6 2
228
26Rn136–6 22
826Rn136–6NUCLEAR DATA SHEETS
(HI,xn γγγγ) 1999Co02,2000BuZY
232Th(136Xe,Xγ ) , E=833 MeV, multi–particle transfer reaction. Measured Eγ , Iγ , γγγ using GAMMASPHERE array of 73
HPGe detectors (1999Co02).
222Rn Levels
E(level) Jπ
0 . 0 † 0 +
1 8 6 . 3 9 † 2 0 2 +
4 4 8 . 9 † 3 4 +
6 0 0 . 8 ‡ 8 1 –
6 3 5 . 0 ‡ 3 3 –
7 6 8 . 5 † 4 ( 6 + )
7 9 7 . 8 ‡ 6 ( 5 – )
E(level) Jπ
1 0 4 9 . 2 ‡ 6 ( 7 – )
1 1 2 8 . 1 † 4 ( 8 + )
1 3 5 6 . 9 ‡ 6 ( 9 – )
1 5 1 3 . 0 † 5 ( 1 0 + )
1 7 0 8 . 2 ‡ 6 ( 1 1 – )
1 9 1 3 . 4 ? † 6 ( 1 2 + )
2 0 8 9 . 1 ‡ 8 ( 1 3 – )
E(level) Jπ
2 3 1 7 . 2 ? † 8 ( 1 4 + )
2 4 8 5 . 3 ? ‡ 8 ( 1 5 – )
2 7 2 7 . 7 ? † 9 ( 1 6 + )
2 8 8 1 . 9 ? ‡ 1 0 ( 1 7 – )
3 2 8 5 . 9 ? ‡ 1 1 ( 1 9 – )
3 6 9 6 . 1 ? ‡ 1 2 ( 2 1 – )
† (A): g.s . band.
‡ (B): Octupole vibrational band.
γ (222Rn)
Eγ E(level) Iγ Mult. I(γ+ce) Comments
1 6 3 . 0 † 5 7 9 7 . 8
1 7 5 . 6 † 5 2 0 8 9 . 1
1 8 6 . 4 2 1 8 6 . 3 9 1 0 0 1 5 E2 1 6 9 2 5
1 9 5 . 4 5 1 7 0 8 . 2 2 2 1 4 E1 2 4 1 5
2 2 8 . 8 5 1 3 5 6 . 9 2 3 1 3 E1 2 4 1 4
2 5 1 . 4 † 5 1 0 4 9 . 2
2 6 2 . 5 2 4 4 8 . 9 1 3 4 2 0 E2 1 6 2 1 0
2 8 0 . 6 5 1 0 4 9 . 2 2 5 7 E1 2 6 7
3 0 7 . 7 5 1 3 5 6 . 9 3 1 1 3 E2 3 5 1 5
3 1 9 . 6 2 7 6 8 . 5 1 1 8 2 6 E2 1 3 2 2 9
3 4 8 . 9 † 5 7 9 7 . 8
3 5 1 . 2 5 1 7 0 8 . 2 4 6 1 4 E2 5 0 1 5
3 5 9 . 6 2 1 1 2 8 . 1 7 5 1 4 E2 8 1 1 5
3 8 0 . 9 5 2 0 8 9 . 1 1 5 8 E2 1 6 9
3 8 4 . 9 2 1 5 1 3 . 0 4 0 1 1 E2 4 3 1 1
3 9 6 . 3 † 5 2 4 8 5 . 3 ?
3 9 6 . 6 † 5 2 8 8 1 . 9 ?
4 0 0 . 4 † 5 1 9 1 3 . 4 ?
4 0 3 . 8 † 5 2 3 1 7 . 2 ?
4 0 4 . 0 † 5 3 2 8 5 . 9 ?
4 1 0 . 2 † 5 3 6 9 6 . 1 ?
4 1 0 . 5 † 5 2 7 2 7 . 7 ?
4 1 4 . 6 6 0 0 . 8 Eγ : Not seen in 1999Co02 but taken from adopted gammas.
4 4 8 . 6 † 5 6 3 5 . 0
6 0 0 . 7 6 0 0 . 8 Eγ : Not seen in 1999Co02 but taken from adopted gammas.
† Placement of transition in the level scheme is uncertain.
2 8 6 3
228
27Fr135
228
27Fr135NUCLEAR DATA SHEETS
Adopted Levels
Q(β–)=2028 22 ; S(n)=5000 22 ; S(p)=5412 22 ; Q(α )=5826 24 2003Au03,2011AuZZ.
222Fr Levels
E(level) Jπ T1/2 Comments
0 . 0 2 – 1 4 . 2 m i n 3 %β–=100.
μ=0.63 1 ; Q=0.51 4 (2005St24,1985Co24).
Jπ : 1978Ek02 measured spin (atomic–beam magnetic resonance, 1978Ek02). Log f t values for β–
transitions to 0+ and 4+ states give π=–.
Isotopic shift=–26262 MHZ 3 (1985Co24).
See 2005Dz02 for isotopic shift calculations.
See 1987Co19 for deduced change in the mean square charge radius relative to 212Fr from their
measured isomeric shift , and for calculated deformation parameter from the electric quadrupole
moment.
T1/2: from 1973AfZV (14.2 min 3 ) , 1976VaZC (14.2 min). Other measurement: 1950Hy20 (14.8 min).
Branching: only β– decay was observed. Calculation of probabil ity for 14C emission (1985Po11).
%α<1 was estimated by 1950Hy20 from α systematics. No α decay has been observed.
4 0 2 2 Level populated by 226Ac α decay.
E(level) : from Eα=5399 5 , measured in 226Ac α decay and Q(α ) (226Ac)=5536 21 (2003Au03,2011AuZZ).
226Ac αααα Decay
Parent 226Ac: E=0.0; Jπ=(1); T1/2=29.37 h 12 ; Q(g.s. )=5536 21 ; %α decay=6×10–3 2 .
222Fr Levels
E(level) Jπ T1/2
0 . 0 2 – 1 4 . 2 m i n 3
4 0 2 2
α radiations
Eα E(level) Iα† HF Comments
5 3 9 9 5 4 0 1 0 0 5 1 1 9 Eα : measurement by 1975VaZD. Other measurement: 1964Mc21.
Iα : only one α group was observed.
HF: r0(222Fr)=1.538 6 , T1/2(226Ac)=29.37 h 12 , measured by 1987Mi10 and Q(α ) (226Ac)=5536 21
from 2003Au03, 2011AuZZ are used in calculations.
† For α intensity per 100 decays, multiply by 6×10–5 2 .
2 8 6 4
228
28Ra134–1 22
828Ra134–1NUCLEAR DATA SHEETS
Adopted Levels, Gammas
Q(β–)=–2300 7 ; S(n)=6714 6 ; S(p)=6246 6 ; Q(α )=6679 4 2003Au03,2011AuZZ.
For calculations of level energies by various methods, some including deformations of order higher than β (2) , and
for discussions on level structure see 2006Sa53, 2005Za02, 2003Sh02, 2001Za04 2001Za09, 1998Bu18, 1998Ra05,
1997Bu07, 1997Bu28, 1995De13, 1987En05, 1986Da03, 1985Na07, 1983Pi04, 1983Ia01, 1980Sh07, 1970Ne08.
For theoretical calculations of equil ibrium deformations and deformation energies see 1994Cw01, 1991Sk01, 1988So08,
1986Bo19, 1986Le05, 1984Na22, 1983Ro14, 1982Le19, 1982Du16 and 1981Gy03.
Exotic nuclear shapes, including superdeformation, hyperdeformation and octupole shapes, were calculated and
discussed by 1994Cw01, 1992Ch20, 1992SkZZ, 1989De11, 1989Eg02, 1988Ba48, 1988Ro05, 1988So08, 1987Na10, 1987Ro08,
1986Bo19, 1986Ch23, 1984Na22.
For calculations of electric–dipole moment, and for discussions on the strong octupole effects and octupole
deformation, as well as higher order of deformations, see 2004Ad15, 2003Ad32, 1991Eg01, 1991Bu10, 1989De11,
1986Le05.
See 1988Ro02 for the E1, E3 transition probabil it ies and the 0+, 1– energy splitting.
See 1986Le05, 1993Yo02 for calculations of B(E1)/B(E2) transition probabil it ies from the Kπ=0– band.
For calculations of 14C emission probabil ity, partial half–lives and branchings by using various models, see
1984Po08, 1985Po11, 1985Sh01, 1986De32, 1986Gr20, 1986Ir01, 1986Ka46, 1986La01, 1986Pi11, 1986Po15, 1986Ru11,
1987Bl04, 1987Gu04, 1987Iv01, 1987Po08, 1987Sh04, 1988Ba01, 1988Bl11, 1988Iv02, 1988Sh29, 1988Ta25, 1989Bu06,
1989Ci03, 1989Ma21, 1989Sh37, 1990Ba20, 1990Bu09, 1990Hu07, 1990Ka15, 1990Sh01, 1991Bu01, 1992Gu10, 1993Bu05,
1993De38, 1993Go18, 1993Gr15, 1993Gu11, 1993Ka21, 1993Si26, 1994Bu07, 1994De38, 1995Si05, 1998Ro11, 2002Sa55,
2004Re22, 2004Ba64, 2005Ku32, 2006Xu15, 2009QI07, 2009RO16, 2010Ni13, 2008Ni12.
See 2001Ch02 for calculation of yrast band energies.
Weighted mean of intrinsic electric dipole moment/intrinsic electric quadrupole moment=4.02 11 extracted from
B(E1)/B(E2) (2007Co08).
222Ra Levels
The Kπ=0+ g.s. band and the Kπ=0– band at 242.11 keV have been interpreted as octupole parity–doublet bands. This
nucleus falls sl ightly to the left of middle of the region of octupole deformation defined by the spin systematics
for octupole shapes (1990Ja11).
Cross Reference (XREF) Flags
A 226Th α Decay
B 222Fr β– Decay
C 232Th(136Xe,Xγ )
E(level) Jπ XREF T1/2 Comments
0 . 0 † 0 + ABC 3 8 . 0 s 5 %α=100; %14C=3.0×10–8 10 .
T1/2: from measured values of 38.0 s (1948St42),37.5 s 5 (1956As38), 39 s 4
(1958To25). Other measurement: 1982Bo04.
14C branching from measured values of I(14C)/I(α )= 3.7×10–10 6 (1985Pr01),
3.1×10–10 10 (1985Ho21), and 2.3×10–10 3 (1991Hu02). 1991Hu02 searched also
for any 14C branching to the 3– state in 208Pb at 2614 keV and deduced an
upper l imit of 2×10–10% for its branch.
The isotope shift relative to 214Ra was measured by 1988Ah02; the change in the
nuclear mean square charge radius and the change in the quadrupole
deformation parameter were deduced as Δ<r2>=–0.198, and Δ<β2>1/2=0.191. See
also 1987We03, 1985Ne09.
1 1 1 . 1 2 † 2 2 + ABC 0 . 5 2 n s 4 T1/2: by (α ) (ce 111γ ) (t) in 226Th α decay.
2 4 2 . 1 1 ‡ 2 1 – ABC < 1 . 2 n s T1/2: by (α ) (242γ ) (t) in 226Th α decay.
3 0 1 . 3 9 † 4 4 + ABC < 1 . 4 n s T1/2: by (α ) (190γ ) (t) in 226Th α decay.
3 1 7 . 2 9 ‡ 5 3 – ABC The nuclear electric dipole moment was deduced by 1992Ru01 as 0.036 6 fm from
the branching ratio for E1, E2 transitions deexciting the level . The electric
quadrupole moment of 6.74 b 28 for both the g.s. and the Kπ=0– band was
assumed.
4 7 3 . 7 6 ‡ 8 ( 5 – ) ABC
5 5 0 . 3 † 4 ( 6 + ) C
7 0 3 . 2 ‡ 4 ( 7 – ) C
8 4 3 . 3 † 4 ( 8 + ) C
9 1 4 . 0 § 3 ( 0 + ) A Jπ : gammas to 2+, 1– states; no γ to 0+, 3–, 4+; analogy to the 0+, 916–keV
level in 224Ra.
9 9 2 . 4 ‡ 5 ( 9 – ) C
1 0 2 4 . 9 § 2 2 + AB Jπ : gammas to 0+ and 4+ levels.
1 1 7 0 . 9 2 ( 3 – , 4 + ) B Jπ : γ ' s to 3–, (5–) states; log f t=8.1 3 for β branch from 2– 222Fr.
1 1 7 1 . 6 3 1 + , 1 – , 2 + B Jπ : γ to 0+.
1 1 7 3 . 3 † 5 ( 1 0 + ) C
1 2 2 5 . 2 2 1 + , 1 – , 2 + B Jπ : γ to 0+.
Continued on next page (footnotes at end of table)
2 8 6 5
228
28Ra134–2 22
828Ra134–2NUCLEAR DATA SHEETS
Adopted Levels, Gammas (continued)
222Ra Levels (continued)
E(level) Jπ XREF Comments
1 2 6 5 . 0 3 ( 2 + , 3 ) B Jπ : γ ' s to 2+, 4+; log f t=7.2 for β branch from 2– 222Fr.
1 3 1 0 . 2 3 B
1 3 3 0 . 8 ‡ 6 ( 1 1 – ) C
1 3 6 0 . 6 3 B
1 3 7 5 . 7 3 B
1 4 0 2 . 6 2 ( 3 – ) B Jπ : γ ' s to the 1–, 3– states of the K=0 octupole–vibrational band and to the 2+, 4+ states of
the g.s. band.
1 4 3 2 . 6 3 1 , 2 , 3 – B Jπ : γ ' s to 1–, 2– states; log f t=7.2 for the β branch from 2– 222Fr.
1 4 3 9 . 9 2 ( 3 – ) B Jπ : γ transitions to 1– and (5–) states.
1 4 9 9 . 5 3 1 – , 2 , 3 – B Jπ : γ transitions to 1–, 3– states.
1 5 3 7 . 2 † 6 ( 1 2 + ) C
1 5 5 6 . 1 4 2 + B Jπ : γ transitions to 0+ and 4+ states.
1 6 1 9 . 6 4 B
1 6 4 4 . 9 3 2 + , 3 – B Jπ : γ transitions to 1– and 4+ states.
1 7 1 0 . 3 ‡ 6 ( 1 3 – ) C
1 7 5 4 . 4 6 3 – B Jπ : γ transitions to 2+, 4+, (5–) states; log f t=6.3 for the β feeding from 2– 222Fr.
1 8 2 1 . 5 5 1 , 2 , 3 B Jπ : log f t=6.7 for the β branch from 2– 222Fr.
1 8 4 1 . 2 5 1 , 2 , 3 Jπ : log f t=5.8 for the β branch from 2– 222Fr. If Jπ (1645 level)=3–, then Jπ (1841)≠1+.
1 9 3 3 . 2 † 7 ( 1 4 + ) C
2 1 2 5 . 3 ‡ 7 ( 1 5 – ) C
2 3 5 8 . 7 † 8 ( 1 6 + ) C
2 5 7 0 . 1 ‡ 8 ( 1 7 – ) C
2 8 1 1 . 0 † 1 0 ( 1 8 + ) C
3 0 4 0 . 9 ‡ 1 0 ( 1 9 – ) C
3 2 8 7 . 7 † 1 1 ( 2 0 + ) C
† (A): K=0 g.s. band.
‡ (B): K=0 octupole vibrational band.
§ (C): K=0 band.
γ (222Ra)
E(level) Eㆇ Iγ§ Mult.# α I(γ+ce) Comments
1 1 1 . 1 2 1 1 1 . 2 2 2 8 1 2 E2 6 . 2 6 2 0 5 9 1 B(E2)(W.u.)=111 9 .
2 4 2 . 1 1 1 3 1 . 0 0 2 3 2 . 1 1 6 [ E1 ] 0 . 2 5 4 B(E1)(W.u.)>1.5×10–5.
2 4 2 . 1 1 2 1 0 0 5 E1 0 . 0 5 8 0 B(E1)(W.u.)>7.4×10–6.
Mult. : from ce work in 226Th α decay.
3 0 1 . 3 9 1 9 0 . 7 2 1 0 0 1 9 E2 0 . 7 1 6 1 7 1 3 2 B(E2)(W.u.)>12.
3 1 7 . 2 9 7 5 . 1 3 2 0 . 0 1 7 4
2 0 6 . 1 7 5 1 0 0 1 0 E1 0 . 0 8 4 7 Mult. : from ce work in 226Th α decay.
4 7 3 . 7 6 1 7 2 . 3 7 2
5 5 0 . 3 2 4 8 . 4 2 8 6 1 7 E2 1 1 0 2 1
7 0 3 . 2 1 5 3 . 1 5 7 2 2 3 E1 8 4 2 7
2 2 9 . 3 5 1 3 4 E2 1 8 5
8 4 3 . 3 1 4 0 . 1 2 6 6 1 2 E1 8 0 1 4
2 9 2 . 9 2 6 1 5 E2 7 2 6
9 1 4 . 0 6 7 1 . 9 3 1 0 0 1 1
8 0 2 . 7 5 2 1 8
9 9 2 . 4 1 4 9 . 3 5 5 0 8 E1 5 8 1 0
2 8 9 . 0 5 4 4 5 E2 5 2 6
1 0 2 4 . 9 7 0 7 . 5 2 1 0 0 5
7 2 3 . 4 4 3 . 4 5
7 8 2 . 8 2 9 8 9
9 1 3 . 7 4 1 7 3
1 0 2 5 . 0 4 6 . 7 1 2
1 1 7 0 . 9 6 9 6 . 9 2 2 8 . 7 5
8 5 3 . 8 2 1 0 0 7
8 6 9 . 6 2 8 1 2 5
1 1 7 1 . 6 9 2 9 . 5 2 1 5 2
1 0 6 0 . 3 2 1 0 0 8
1 1 7 1 . 7 2 5 3 6
Continued on next page (footnotes at end of table)
2 8 6 6
228
28Ra134–3 22
828Ra134–3NUCLEAR DATA SHEETS
Adopted Levels, Gammas (continued)
γ (222Ra) (continued)
E(level) Eㆇ Iγ§ Mult.# I(γ+ce)
1 1 7 3 . 3 1 8 0 . 9 2 5 7 1 3 E1 6 4 1 5
3 3 0 . 1 2 4 3 4 E2 4 9 5
1 2 2 5 . 2 9 8 2 . 9 2 9 7 1 9
1 1 1 4 . 3 2 1 0 0 1 9
1 2 2 5 . 2 2 3 8 7
1 2 6 5 . 0 9 6 3 . 6 2 2 6 4
1 1 5 3 . 9 2 1 0 0 1 0
1 3 1 0 . 2 1 0 6 8 . 1 2
1 3 3 0 . 8 1 5 7 . 4 5 2 7 4 E1 3 1 4
3 3 8 . 3 5 4 2 4 E2 4 6 6
1 3 6 0 . 6 1 0 4 3 . 6 2 1 0 0 1 3
1 2 4 9 . 1 2 6 0 1 1
1 3 7 5 . 7 1 1 3 3 . 6 2
1 4 0 2 . 6 2 3 1 . 7 2 1 5 . 2 1 6
3 7 7 . 6 2 2 4 2
1 0 8 5 . 2 2 9 2 1 2
1 1 0 1 . 1 2 1 0 0 1 0
1 1 6 0 . 5 2 1 4 . 4 1 4
1 2 9 1 . 6 2 9 . 6 1 6
1 4 3 2 . 6 1 1 9 0 . 4 3 8 . 5 1 5
1 3 2 1 . 6 2 1 0 0 8
1 4 3 9 . 9 2 6 9 . 0 2 1 3 3
4 1 5 . 0 2 1 1 2
9 6 6 . 2 2 2 3 5
1 1 2 2 . 4 2 4 0 7
1 1 3 8 . 5 2 1 0 0 1 0
1 1 9 8 . 0 2 3 0 5
1 4 9 9 . 5 4 7 4 . 5 3 1 0 0 1 0
1 1 8 2 . 1 3 8 7 1 0
1 2 5 7 . 5 3 3 3 7
1 3 8 8 . 5 3 7 6 1 0
1 5 3 7 . 2 2 0 6 . 2 5 2 7 5 E1 3 0 6
E(level) Eㆇ Iγ§ Mult.# I(γ+ce)
1 5 3 7 . 2 3 6 3 . 9 5 4 2 4 E2 4 6 4
1 5 5 6 . 1 1 2 3 8 . 6 3 1 0 0 1 3
1 2 5 4 . 4 4 2 6 3
1 4 4 5 . 2 4 6 9 1 1
1 5 5 6 . 5 4 5 9 1 1
1 6 1 9 . 6 1 3 7 7 . 4 3 1 0 0 1 5
1 5 0 8 . 7 4 2 4 7
1 6 4 4 . 9 6 1 9 . 9 2 3 1 4
1 3 2 7 . 6 2 1 0 0 9
1 3 4 3 . 3 3 1 0 . 4 1 7
1 4 0 2 . 5 4 2 7 3
1 5 3 4 . 1 4 1 7 3
1 7 1 0 . 3 1 7 3 . 1 5 2 8 4 E1 3 2 5
3 7 9 . 6 5 3 4 3 E2 3 6 4
1 7 5 4 . 4 3 5 1 . 7 2 5 2 1 2
1 2 8 1 . 0 3 3 4 7
1 4 3 6 . 4 3 1 0 0 7
1 4 5 3 . 4 3 4 5 1 0
1 6 4 3 . 9 3 4 4 1 2
1 8 2 1 . 5 1 5 7 9 . 4 4
1 8 4 1 . 2 1 9 6 . 3 2 1 0 0 1 3
1 5 9 9 . 6 4 1 6 5
1 9 3 3 . 2 3 9 6 . 0 5 3 0 4 E2 3 2 4
2 1 2 5 . 3 1 9 2 . 1 5 2 3 1 0 E1 2 5 1 1
4 1 5 . 0 5 3 4 4 E2 3 5 4
2 3 5 8 . 7 4 2 5 . 5 5 2 4 4 E2 2 5 4
2 5 7 0 . 1 2 1 1 . 4 5
4 4 4 . 8 5 3 2 6 E2 3 4 6
2 8 1 1 . 0 4 5 2 . 3 5 1 7 4 E2 1 7 4
3 0 4 0 . 9 4 7 0 . 8 5 1 5 4 E2 1 6 4
3 2 8 7 . 7 4 7 6 . 7 5 1 0 4 E2 1 1 4
† From 232Th(136Xe,Xγ ) dataset. Those not observed in this dataset are taken from decay datasets.
‡ From 226Th α decay and 222Fr β– decay. The uncertainties of γ ' s deexciting the levels above 1 MeV have been increased because
of a poor energy f it to the level scheme; therefore, the Eγ values have been rounded off here. See 222Fr β– decay section for
the experimental values l isted by the authors.
§ Relative photon intensity deexciting each level .
# From GAMMASPHERE data (1999Co02). Multipolarities inside the square brackets are from the ce work in 226Tl α decay.
A
A
A
(A) K=0 g.s. band
(B) K=0 octupolevibrational band
(C) K=0 band
0.00+
111.122+
301.394+
550.3(6+)
843.3(8+)
1173.3(10+)
1537.2(12+)
1933.2(14+)
2358.7(16+)
2811.0(18+)
3287.7(20+)
111
191
248
293
330
364
396
426
452
477
242.111-
317.293-
473.76(5-)
703.2(7-)
992.4(9-)
1330.8(11-)
1710.3(13-)
2125.3(15-)
2570.1(17-)
3040.9(19-)
229
289
338
380
415
445
471
914.0(0+)
1024.92+
1025
803
914
723
222
88Ra134
2 8 6 7
228
28Ra134–4 22
828Ra134–4NUCLEAR DATA SHEETS
2 8 6 8
228
28Ra134–5 22
828Ra134–5NUCLEAR DATA SHEETS
222Fr ββββ– Decay 1992Ru01
Parent 222Fr: E=0.0; Jπ=2–; T1/2=14.2 min 3 ; Q(g.s. )=2032 21 ; %β– decay=100.
222Fr–%β– decay: Relative photon intensities were normalized by 1992Ru01 to Iγ (324.2γ from 222Ra)=2.77 8 per 100
222Ra decays. This value was measured absolutely by 1969Pe17, and it has been adopted by the evaluator. However,
1992Ru01 did not provide their measured Iγ (324γ ) relative to the Iγ ' s given here. From the γ–transition
intensities shown on the decay scheme of 1992Ru01, Iγ normalization=0.49 6 ; an assumption of any β feeding to the
g.s . to be negligible yields Iγ normalization=0.51 6 ; by requiring that the log f1ut for a β feeding to the g.s.
is >8.5, Iβ is calculated to be <7%. Iβ (g.s . )=3% 3 yields Iγ normalization=0.50 6 .
The 222Fr β– decay scheme is presented as constructed by 1992Ru01 based on their β–gated γγ–coincidence
measurements. The decay scheme was built upon the previously known levels which were established up to the
1170–keV level .
222Ra Levels
E(level) Jπ T1/2
0 . 0 0 + 3 8 . 0 s 5
1 1 1 . 1 2 2 2 +
2 4 2 . 1 1 2 1 –
3 0 1 . 3 9 4 4 +
3 1 7 . 2 9 5 3 –
4 7 3 . 7 6 8 ( 5 – )
1 0 2 4 . 9 2 2 +
1 1 7 0 . 9 2 ( 3 – , 4 + )
E(level) Jπ
1 1 7 1 . 6 3 1 + , 1 – , 2 +
1 2 2 5 . 2 2 1 + , 1 – , 2 +
1 2 6 5 . 0 3 ( 2 + , 3 )
1 3 1 0 . 2 3
1 3 6 0 . 6 3
1 3 7 5 . 7 3
1 4 0 2 . 6 2 ( 3 – )
1 4 3 2 . 6 3 1 , 2 , 3 –
E(level) Jπ
1 4 3 9 . 9 2 ( 3 – )
1 4 9 9 . 5 3 1 – , 2 , 3 –
1 5 5 6 . 1 4 2 +
1 6 1 9 . 6 4
1 6 4 4 . 9 3 2 + , 3 –
1 7 5 4 . 4 6 3 –
1 8 2 1 . 5 5 1 , 2 , 3
1 8 4 1 . 2 5 1 , 2 , 3
β– radiations
See 1975We23 for singles β spectrum measurements. The spectrum shows a f lat tail of low intensity and extended to
much higher energy than the main portion of the data. After subtraction of this tail (which was assumed due to α
particles from 222Ra), an F–K analysis gives Eβ (max)=1780 20 for the endpoint which does not agree with the Eβ–
(to 111.12 level) .
Eβ– E(level) Iβ–† Log f t
( 1 9 1 2 1 ) 1 8 4 1 . 2 0 . 1 0 6 5 . 8
( 2 1 1 2 1 ) 1 8 2 1 . 5 0 . 0 1 6 4 6 . 7
( 2 7 8 2 1 ) 1 7 5 4 . 4 0 . 1 0 3 1 6 6 . 3
( 3 8 7 2 1 ) 1 6 4 4 . 9 0 . 1 2 6 6 . 7
( 4 1 2 2 1 ) 1 6 1 9 . 6 0 . 0 4 9 8 7 . 2
( 4 7 6 2 1 ) 1 5 5 6 . 1 0 . 0 6 9 1 0 7 . 2
( 5 3 3 2 1 ) 1 4 9 9 . 5 0 . 1 1 7 1 6 7 . 2
( 5 9 2 2 1 ) 1 4 3 9 . 9 0 . 3 4 5 6 . 9
( 5 9 9 2 1 ) 1 4 3 2 . 6 0 . 1 4 7 2 1 7 . 2
( 6 2 9 2 1 ) 1 4 0 2 . 6 0 . 6 5 1 0 6 . 7
( 6 5 6 2 1 ) 1 3 7 5 . 7 0 . 0 3 7 6 8 . 0
( 6 7 1 2 1 ) 1 3 6 0 . 6 0 . 0 5 2 9 7 . 9
Eβ– E(level) Iβ–† Log f t
( 7 2 2 2 1 ) 1 3 1 0 . 2 0 . 0 2 2 5 8 . 3
( 7 6 7 2 1 ) 1 2 6 5 . 0 0 . 3 4 5 7 . 2
( 8 0 7 2 1 ) 1 2 2 5 . 2 0 . 0 8 7 1 5 7 . 9
( 8 6 0 2 1 ) 1 1 7 1 . 6 0 . 7 8 1 1 7 . 1
( 8 6 1 2 1 ) 1 1 7 0 . 9 0 . 0 7 4 8 . 1
( 1 0 0 7 2 1 ) 1 0 2 4 . 9 0 . 8 5 1 2 7 . 3
( 1 7 1 5 2 1 ) 3 1 7 . 2 9 5 4 9 6 . 3
( 1 7 3 1 2 1 ) 3 0 1 . 3 9 0 . 3 7 6 9 . 4 1 u
( 1 7 9 0 2 1 ) 2 4 2 . 1 1 1 . 7 4 7 . 9
( 1 9 2 1 2 1 ) 1 1 1 . 1 2 3 8 1 2 6 . 2
( 2 0 3 2 ‡ 2 1 ) 0 . 0 3 3 ≥ 8 . 5 1 u
† From intensity balance at each level .
‡ Existence of this branch is questionable.
γ (222Ra)
βγ , βγγ : see 1992Ru01.
X r a y s ( Ra ) :
E I ( x r a y ) / I ( 2 0 6 γ )
1 9 8 5Go 0 5 1 9 8 5Go 0 5 c a l c u l a t e d
– – – – – – – – – – – – – – – – – – – – – – – – – – –
8 8 . 5 0 . 1 4 3 2 0 0 . 1 1 1 1 6 Kα x r a y
1 0 0 . 0 0 . 0 2 7 5 3 5 0 . 0 3 2 5 Kβ x r a y
Eγ† E(level) Iγ‡# Mult.§ α
x 5 4 . 1 4 2 0 . 0 3 0 5
7 5 . 1 3 2 3 1 7 . 2 9 0 . 0 1 7 4 [ E2 ] 3 7 . 5
1 1 1 . 1 1 1 1 1 1 . 1 2 2 6 . 2 2 6 E2 6 . 2 6
1 3 0 . 9 8 1 2 4 2 . 1 1 1 . 2 5 1 2 ( E1 ) 0 . 2 5 4
1 7 2 . 3 7 2 4 7 3 . 7 6 0 . 1 2 1 [ E1 ] 0 . 1 3 0
Continued on next page (footnotes at end of table)
2 8 6 9
228
28Ra134–6 22
828Ra134–6NUCLEAR DATA SHEETS
222Fr ββββ– Decay 1992Ru01 (continued)
γ (222Ra) (continued)
Eγ† E(level) Iγ‡# Mult.§ α Comments
1 9 0 . 2 4 2 3 0 1 . 3 9 1 . 1 9 1 E2 0 . 7 1 6
1 9 6 . 3 1 4 1 8 4 1 . 2 0 . 0 8 1 [ D , E2 ] 1 . 3 1 2
2 0 6 . 1 7 5 3 1 7 . 2 9 1 0 0 1 0 E1 0 . 0 8 4 7 Eγ=206.18 2 (1992Ru01), 206.10 4 (1985Go05); 206.23 5 from 226Th α decay.
x 2 1 8 . 6 6 4 0 . 1 2 1
x 2 2 1 . 3 6 2 0 . 5 2 5
x 2 2 4 . 1 0 2 0 . 1 9 2
2 3 1 . 6 7 4 1 4 0 2 . 6 0 . 0 7 6 8 [ D , E2 ] 0 . 8 7 α : α (E1)=0.0643, α (M1)=1.53, α (E2)=0.356.
2 4 2 . 1 1 1 2 4 2 . 1 1 3 . 9 4 E1 0 . 0 5 8 0
2 6 8 . 9 9 4 1 4 3 9 . 9 0 . 0 4 0 8 0 . 5 3 4 8 α : α (E1)=0.0454, α (M1)=1.01, α (E2)=0.217.
3 5 1 . 7 5 4 1 7 5 4 . 4 0 . 0 3 7 8 [M1 , E2 ] 0 . 2 9 1 9 α (M1)=0.484, α (E2)=0.0973.
3 7 7 . 6 4 4 1 4 0 2 . 6 0 . 1 2 1 [ E1 ] 0 . 0 2 1 3
4 1 5 . 0 5 4 1 4 3 9 . 9 0 . 0 3 2 6 [ E1 ] 0 . 0 0 0 3 0
x 4 5 5 . 3 7 7 0 . 0 1 8 4
4 7 4 . 4 5 9 1 4 9 9 . 5 0 . 0 7 9 8
6 1 9 . 9 5 4 1 6 4 4 . 9 0 . 0 7 2 8
6 9 6 . 8 8 5 1 1 7 0 . 9 0 . 0 4 6 8
7 0 7 . 5 4 3 1 0 2 4 . 9 0 . 8 9 4 [ E1 ] 0 . 0 0 6 0 2
7 2 3 . 4 5 4 1 0 2 4 . 9 0 . 0 3 0 4 [ E2 ] 0 . 0 1 7 3
7 8 2 . 7 7 3 1 0 2 4 . 9 0 . 8 7 8 [ E1 ] 0 . 0 0 4 9 9
x 8 3 1 . 5 8 5 0 . 0 3 6 5
x 8 4 6 . 7 2 8 0 . 0 7 0 1 4
8 5 3 . 7 8 8 1 1 7 0 . 9 0 . 1 6 1
8 6 9 . 6 2 1 1 7 0 . 9 0 . 1 3 4
9 1 3 . 6 9 5 1 0 2 4 . 9 0 . 1 5 2
9 2 9 . 4 7 8 1 1 7 1 . 6 0 . 1 4 2
9 6 3 . 6 1 6 1 2 6 5 . 0 0 . 1 4 2
9 6 6 . 2 4 9 1 4 3 9 . 9 0 . 0 7 0 1 4
9 8 2 . 9 0 8 1 2 2 5 . 2 0 . 0 7 2 1 4
1 0 2 5 . 0 2 8 1 0 2 4 . 9 0 . 0 6 0 1 0
1 0 4 3 . 6 0 9 1 3 6 0 . 6 0 . 0 6 5 8
1 0 6 0 . 3 3 5 1 1 7 1 . 6 0 . 9 2 7
1 0 6 8 . 0 8 8 1 3 1 0 . 2 0 . 0 4 3 8
1 0 8 5 . 2 0 5 1 4 0 2 . 6 0 . 4 6 6
1 1 0 1 . 0 9 5 1 4 0 2 . 6 0 . 5 0 5
1 1 1 4 . 2 6 8 1 2 2 5 . 2 0 . 0 7 4 1 4
1 1 2 2 . 4 1 9 1 4 3 9 . 9 0 . 1 2 2
1 1 3 3 . 6 1 8 1 3 7 5 . 7 0 . 0 7 4 8
1 1 3 8 . 4 7 5 1 4 3 9 . 9 0 . 3 0 3
1 1 5 3 . 8 7 5 1 2 6 5 . 0 0 . 5 4 5
x 1 1 5 6 . 7 5 9 0 . 0 4 4 9
1 1 6 0 . 5 2 8 1 4 0 2 . 6 0 . 0 7 2 7
1 1 7 1 . 6 9 8 1 1 7 1 . 6 0 . 4 9 5
1 1 8 2 . 0 5 8 1 4 9 9 . 5 0 . 0 6 9 8
1 1 9 0 . 4 1 1 4 3 2 . 6 0 . 0 2 3 4
1 1 9 7 . 9 9 8 1 4 3 9 . 9 0 . 0 8 9 1 5
1 2 2 5 . 2 4 8 1 2 2 5 . 2 0 . 0 2 8 5
1 2 3 8 . 6 0 8 1 5 5 6 . 1 0 . 0 5 4 7
1 2 4 9 . 1 1 1 3 6 0 . 6 0 . 0 3 9 7
1 2 5 4 . 4 2 1 5 5 6 . 1 0 . 0 1 4 3
1 2 5 7 . 5 1 1 4 9 9 . 5 0 . 0 2 6 5
1 2 8 0 . 9 9 9 1 7 5 4 . 4 0 . 0 2 4 5
1 2 9 1 . 6 1 8 1 4 0 2 . 6 0 . 0 4 8 8
x 1 2 9 5 . 6 1 0 . 0 2 8 5
1 3 2 1 . 6 5 6 1 4 3 2 . 6 0 . 2 7 2
Eγ† E(level) Iγ‡#
1 3 2 7 . 5 8 6 1 6 4 4 . 9 0 . 2 3 2
1 3 4 3 . 3 1 1 6 4 4 . 9 0 . 0 2 4 4
1 3 7 7 . 4 1 1 6 1 9 . 6 0 . 0 8 0 9
1 3 8 8 . 5 1 1 4 9 9 . 5 0 . 0 6 0 8
1 4 0 2 . 5 2 1 6 4 4 . 9 0 . 0 6 2 7
1 4 3 6 . 4 1 1 7 5 4 . 4 0 . 0 7 1 7
1 4 4 5 . 2 2 1 5 5 6 . 1 0 . 0 3 7 6
1 4 5 3 . 4 1 1 7 5 4 . 4 0 . 0 3 2 6
x 1 5 0 2 . 3 1 0 . 0 5 0 9
1 5 0 8 . 7 2 1 6 1 9 . 6 0 . 0 1 9 4
1 5 3 4 . 1 2 1 6 4 4 . 9 0 . 0 3 9 7
1 5 5 6 . 5 2 1 5 5 6 . 1 0 . 0 3 2 6
1 5 7 9 . 4 2 1 8 2 1 . 5 0 . 0 3 2 6
1 5 9 9 . 6 2 1 8 4 1 . 2 0 . 0 1 3 4
1 6 4 3 . 9 1 1 7 5 4 . 4 0 . 0 3 1 8
† From 1992Ru01, except where noted. Other measurement: 1985Go05.
‡ Relative photon intensities, measured by 1992Ru01.
§ From 226Th α decay. The multipolarities in square brackets are from the level scheme.
# For absolute intensity per 100 decays, multiply by 0.50 6 .
x γ ray not placed in level scheme.
28
70
228
28 Ra
13
4 –7
228
28 Ra
13
4 –7
NU
CL
EA
R D
AT
A S
HE
ET
S
2
22F
r β βββ– D
ec
ay
19
92
Ru
01
(co
ntin
ue
d)
2– 0.0 14.2 min
%β–=100
228
27Fr135
Q–=203221
0+ 0.0 38.0 s≥8.51u3
2+ 111.126.238
1– 242.117.91.7
4+ 301.399.41u0.37
3– 317.296.354
(5–) 473.76
2+ 1024.97.30.85
(3–,4+) 1170.98.10.07
1+,1–,2+ 1171.67.10.78
1+,1–,2+ 1225.27.90.087
(2+,3) 1265.07.20.34
1310.28.30.022
1360.67.90.052
1375.78.00.037
(3–) 1402.66.70.65
1,2,3– 1432.67.20.147
(3–) 1439.96.90.34
1–,2,3– 1499.57.20.117
2+ 1556.17.20.069
1619.67.20.049
2+,3– 1644.96.70.12
3– 1754.46.30.103
1,2,3 1821.56.70.016
1,2,3 1841.25.80.10
Log f tIβ–
Decay Scheme
Intensities: I(γ+ce) per 100 decays by this branch
111.
11 E
2 9
5
130.
98 (
E1)
0.
78
242.
11 E
1 2
.1
190.
24 E
2 1
.02
75.1
3 [E
2]
0.33
206.
17 E
1 5
4172.
37 [
E1]
0.
068
707.
54 [
E1]
0.
45
723.
45 [
E2]
0.
015
782.
77 [
E1]
0.
44
913.
69
0.07
5
1025
.02
0.0
30696.
88
0.02
3
853.
78
0.08
0
869.
6 0
.065
929.
47
0.07
0
1060
.33
0.4
6
1171
.69
0.2
5
982.
90
0.03
6
1114
.26
0.0
37
1225
.24
0.0
14
963.
61
0.07
0
1153
.87
0.2
7
1068
.08
0.0
22
1043
.60
0.0
32
1249
.1
0.02
0
1133
.61
0.0
37
231.
67 [
D,E
2]
0.07
377.
64 [
E1]
0.
061
1085
.20
0.2
3
1101
.09
0.2
5
1160
.52
0.0
36
1291
.61
0.0
24
1190
.4
0.01
15
1321
.65
0.1
35
268.
99
0.03
1
415.
05 [
E1]
0.
016
966.
24
0.03
5
1122
.41
0.0
60
1138
.47
0.1
50
1197
.99
0.0
45
474.
45
0.04
0
1182
.05
0.0
34
1257
.5
0.01
3
1388
.5
0.03
0
1238
.60
0.0
27
1254
.4
0.00
70
1445
.2
0.01
9
1556
.5
0.01
6
1377
.4
0.04
0
1508
.7
0.00
95
619.
95
0.03
6
1327
.58
0.1
15
1343
.3
0.01
20
1402
.5
0.03
1
1534
.1
0.02
0
351.
75 [
M1,
E2]
0.
024
1280
.99
0.0
12
1436
.4
0.03
6
1453
.4
0.01
6
1643
.9
0.01
5
1579
.4
0.01
6
196.
31 [
D,E
2]
0.09
1599
.6
0.00
65
228
28Ra134
2 8 7 1
228
28Ra134–8 22
828Ra134–8NUCLEAR DATA SHEETS
226Th αααα Decay
Parent 226Th: E=0.0; Jπ=0+; T1/2=30.57 min 10 ; Q(g.s. )=6450.9 22 ; %α decay=100.
222Ra Levels
α γ ( t ) :
( 6 2 3 4 α ) ( c e 1 1 1 γ ) ( t ) T 1 / 2 ( 1 1 1 l e v e l ) = 0 . 5 2 n s 4 5
( α ) ( 2 4 0 γ ) ( t ) T 1 / 2 ( 2 4 2 l e v e l ) < 1 . 2 n s
( α ) ( 1 9 0 γ ) ( t ) T 1 / 2 ( 3 0 1 l e v e l ) < 1 . 4 n s
E(level) Jπ T1/2
0 . 0 0 + 3 8 . 0 s 5
1 1 1 . 1 2 2 2 + 0 . 5 2 n s 4
2 4 2 . 1 1 2 1 – < 1 . 2 n s
3 0 1 . 3 9 4 4 + < 1 . 4 n s
3 1 7 . 2 9 5 3 –
4 7 3 . 7 6 8 ( 5 – )
9 1 4 . 0 3 ( 0 + )
1 0 2 4 . 9 2 2 +
α radiations
See 1986Ch36, 1980Ka41, 1979Po23 for theoretical calculations of α–decay probabil it ies.
See 2010Wa31, 2009Wa01, 2009De32, 2009Ni06 and 2006Xu08 for calculation of branching ratio and half–lives. 2007Pe30,
2006Xu04, 2005Sh42, 2003Ba64, 2002Ba60, 2002Du16 for calculations of half–lives See 2005Bu38,199de51, 1996De19 for
calculation of alpha decay width.
Eα† E(level) Iα‡@ HF§ Comments
( 5 3 3 3 # 6 ) 1 0 2 4 . 9 0 . 0 0 0 1 7 4 4 . 0 1 0
( 5 4 4 2 # 6 ) 9 1 4 . 0 0 . 0 0 0 3 4 4 8 . 2 1 0
( 5 8 7 4 # 6 ) 4 7 3 . 7 6 0 . 0 0 0 2 3 2 2 . 2 × 1 0 3 2
6 0 2 8 5 3 1 7 . 2 9 0 . 2 0 6 9 1 3 . 9 7 Iα : 0.22% was measured by 1975VaZD.
6 0 4 0 5 3 0 1 . 3 9 0 . 1 8 7 1 1 1 8 . 1 1 1 Iα : 0.2% was measured by 1975VaZD.
6 0 9 9 5 2 4 2 . 1 1 1 . 2 6 5 5 . 0 2 Iα : the measured values are 1.7% (1956As38), 1.2% (1963Le17), 1.3% 2
(1975VaZD).
6 2 3 4 5 1 1 1 . 1 2 2 2 . 8 2 1 . 0 8 2 Iα : measurement of 1969Pe17. Other measured values: 19.0% 15 (1956As38),
20% (1961Ru06), 23.0% 23 (1975VaZD). 23.1% 16 from level scheme.
6 3 3 6 . 8 1 0 0 . 0 7 5 . 5 3 1 . 0 Iα : from sum of Iα ' s . Iα=75.3% 3 is recommended by 1991Ry01. The measured
intensities are 79% (1956As38), 78% (1961Ru06), 75% 8 (1975VaZD).
Iα=75.2 16 from Iγ ' s .
† The energies of α ' s to the g.s. and to the 111–keV level are given as recommended by 1991Ry01 from Eα measurements of 1956As38
and 1975VaZD. The energies measured by 1956As38 are increased 4.6 keV, the Eα (0) and Eα (111 level) measured by 1975VaZD are
decreased 0.4 keV and 6.1 keV, respectively, by 1991Ry01 because of changes in calibration energies. All other Eα ' s are
calculated by the evaluator from Eα (g.s . ) and E(level) .
‡ Deduced from level scheme, except for Iα (to g.s. ) and Iα (to 111 level) , as indicated.
§ HF(α to g.s. )=1.0 gives r0(222Ra)=1.5382 5 . T1/2(226Th)=30.57 min 10 , measured by 1987Mi10, and Q(α ) (226Th)=6450.9 22 of
1993Au05, 2011AuZZ are used in calculations. See 1990Bu30 for a semiclassical calculation of nuclear radius and for systematics
of T1/2(α ) and r0 values. See also 1977Ba70.
# α has not been observed.
@ Absolute intensity per 100 decays.
γ (222Ra)
γγ : see 1976Ku08, 1956As38.
αγ : see 1963Le17, 1969Pe17, 1969Br10.
αγ (θ ) : see 1971He19, 1954St02.
Eγ† E(level) Iγ‡& Mult. α
( 7 5 . 1 3 § 2 ) 3 1 7 . 2 9 3 . 2 × 1 0 – 5 # 8 [ E2 ] 3 7 . 5
Continued on next page (footnotes at end of table)
2 8 7 2
228
28Ra134–9 22
828Ra134–9NUCLEAR DATA SHEETS
226Th αααα Decay (continued)
γ (222Ra) (continued)
Eγ† E(level) Iγ‡& Mult. α Comments
1 1 1 . 1 2 3 1 1 1 . 1 2 3 . 2 9 2 0 E2 6 . 2 6 Iγ : 3.3% 2 was measured by 1969Pe17.
Mult. : Ice measurements: L12:L3:M23:N=
17.0 22 :11.6 19 :9.5 17 :3.2 7 (1967LoZZ); α (L2)=2.4 4 ,
α (L)=4.1 5 (1974Va28). Ice 's given here were normalized to
Ice(K)(230γ of 226Ac decay)=5.45. For absolute Ice 's per 100 α
decays, they should be multiplied by 0.269 18 .
α : 6.24 25 was deduced by 1969Pe17 from αγ data.
1 3 1 . 0 2 5 2 4 2 . 1 1 0 . 2 7 8 1 3 ( E1 ) 0 . 2 5 4 Mult. : no ce l ines were observed (1969Br10).
1 7 2 . 3 3 4 7 3 . 7 6 0 . 0 0 0 2 0 2 [ E1 ] 0 . 1 3 0 Transition was observed only in γγ–coincidence spectra.
1 9 0 . 3 0 5 3 0 1 . 3 9 0 . 1 0 9 6 E2 0 . 7 1 6 Mult. : from ce data of 1976Ku08 (measured ce intensities were not
given). Only E2 multipolarity yields an intensity balance at
the 301.42–keV level .
2 0 6 . 2 3 5 3 1 7 . 2 9 0 . 1 8 9 8 E1 0 . 0 8 4 7 Mult. : from ce data of 1976Ku08 (measured ce intensities were not
given). Only E1 multipolarity is consisted with the intensity
balance at the 317.35 level .
2 4 2 . 1 2 5 2 4 2 . 1 1 0 . 8 6 6 4 0 E1 0 . 0 5 8 0 Mult. : α (K)exp≈0.06 (estimated by the evaluator from the (α ) (ce)
spectrum shown by 1969Br10).
6 7 1 . 9 3 9 1 4 . 0 0 . 0 0 0 2 8 3
7 0 7 . 5 5 1 0 2 4 . 9 0 . 0 0 0 0 6@ 2
7 2 3 . 4 § 4 1 0 2 4 . 9 0 . 0 0 0 0 0 2 # 1
7 8 3 . 0 5 1 0 2 4 . 9 0 . 0 0 0 0 9@ 3
8 0 2 . 7 5 9 1 4 . 0 0 . 0 0 0 0 6 2
9 1 3 . 7 § 4 1 0 2 4 . 9 0 . 0 0 0 0 1 0 # 4
1 0 2 5 . 0 § 4 1 0 2 4 . 9 0 . 0 0 0 0 0 4 # 2
† From 1976Ku08. Other measurements: 1974Va28, 1969Br10, 1956Sm88, 1956As38.
‡ From 1976Ku08. Relative photon intensities were normalized by 1976Ku08 to I(324γ of 222Ra α decay)=2.77% (taken from 1969Pe17)
to obtain intensities per 100 α decays.
§ This γ was not observed in 226Th α decay; its energy is the adopted value from 222Fr β– decay.
# From relative branching deexciting the level , as measured in 222Fr β– decay.
@ Iγ (783γ ) /Iγ (707γ )=0.98 9 was measured in 222Fr β– decay.
& Absolute intensity per 100 decays.
0+ 0.0 30.57 min
%α=100229
60Th136
Qα=6450.922
0+ 0.0 38.0 s 1.075.56336.8
2+ 111.12 0.52 ns 1.0822.86234
1– 242.11 <1.2 ns 5.01.266099
4+ 301.39 <1.4 ns 18.10.1876040
3– 317.29 13.90.2066028
(5–) 473.76 2.2×1030.00023
(0+) 914.0 8.20.00034
2+ 1024.9 4.00.00017
HFIαEα
Decay Scheme
Intensities: I(γ+ce) per 100 decays by
this branch
111.
12 E
2 2
3.9
131.
02 (
E1)
0.
349
242.
12 E
1 0
.92
190.
30 E
2 0
.187
75.1
3 [E
2]
0.00
12
206.
23 E
1 0
.205
172.
3 [E
1]
0.00
0226
671.
9 0
.000
28
802.
7 0
.000
06
707.
5 0
.000
06
723.
4 0
.000
002
783.
0 0
.000
09
913.
7 0
.000
010
1025
.0
0.00
0004
228
28Ra134
2 8 7 3
228
28Ra134–10 22
828Ra134–10NUCLEAR DATA SHEETS
232Th(136Xe,X γγγγ) 1999Co02
E=833 MeV. Measured Eγ , Iγ , γγγ using GAMMASPHERE array of 73 HP Ge detectors (1999Co02). Others (same group):
1998Bu17, 1997Co08, 1997Co14.
Weighted mean of intrinsic electric dipole moment/intrinsic electric quadrupole moment=4.02 11 extracted from
B(E1)/B(E2) (2007Co08).
222Ra Levels
E(level) Jπ
0 . 0 † 0 +
1 1 1 . 2 0 † 2 0 2 +
2 4 2 . 2 ‡ 8 1 –
3 0 1 . 9 † 3 4 +
3 1 7 . 3 ‡ 1 1 3 –
4 7 4 . 0 ‡ 5 ( 5 – )
5 5 0 . 3 † 4 ( 6 + )
E(level) Jπ
7 0 3 . 2 ‡ 4 ( 7 – )
8 4 3 . 3 † 4 ( 8 + )
9 9 2 . 4 ‡ 5 ( 9 – )
1 1 7 3 . 3 † 5 ( 1 0 + )
1 3 3 0 . 8 ‡ 6 ( 1 1 – )
1 5 3 7 . 2 † 6 ( 1 2 + )
1 7 1 0 . 3 ‡ 6 ( 1 3 – )
E(level) Jπ
1 9 3 3 . 2 † 7 ( 1 4 + )
2 1 2 5 . 3 ‡ 7 ( 1 5 – )
2 3 5 8 . 7 † 8 ( 1 6 + )
2 5 7 0 . 1 ‡ 8 ( 1 7 – )
2 8 1 1 . 0 † 1 0 ( 1 8 + )
3 0 4 0 . 9 ‡ 1 0 ( 1 9 – )
3 2 8 7 . 7 † 1 1 ( 2 0 + )
† (A): g.s . Band.
‡ (B): Octupole–vibrational Band.
γ (222Ra)
Eγ E(level) Iγ Mult. I(γ+ce)
1 1 1 . 2 2 1 1 1 . 2 0 2 8 1 2 E2 2 0 5 9 1
1 3 1 . 0 2 † 2 4 2 . 2
1 4 0 . 1 2 8 4 3 . 3 6 6 1 2 E1 8 0 1 4
1 4 9 . 3 5 9 9 2 . 4 5 0 8 E1 5 8 1 0
1 5 3 . 1 5 7 0 3 . 2 7 2 2 3 E1 8 4 2 7
1 5 7 . 4 5 1 3 3 0 . 8 2 7 4 E1 3 1 4
1 7 2 . 2 5 4 7 4 . 0
1 7 3 . 1 5 1 7 1 0 . 3 2 8 4 E1 3 2 5
1 8 0 . 9 2 1 1 7 3 . 3 5 7 1 3 E1 6 4 1 5
1 9 0 . 7 2 3 0 1 . 9 1 0 0 1 9 E2 1 7 1 3 2
1 9 2 . 1 5 2 1 2 5 . 3 2 3 1 0 E1 2 5 1 1
2 0 6 . 1 5 † 3 1 7 . 3
2 0 6 . 2 5 1 5 3 7 . 2 2 7 5 E1 3 0 6
2 1 1 . 4 5 2 5 7 0 . 1
2 2 9 . 3 5 7 0 3 . 2 1 3 4 E2 1 8 5
Eγ E(level) Iγ Mult. I(γ+ce)
2 4 2 . 1 2 † 2 4 2 . 2
2 4 8 . 4 2 5 5 0 . 3 8 6 1 7 E2 1 1 0 2 1
2 8 9 . 0 5 9 9 2 . 4 4 4 5 E2 5 2 6
2 9 2 . 9 2 8 4 3 . 3 6 1 5 E2 7 2 6
3 3 0 . 1 2 1 1 7 3 . 3 4 3 4 E2 4 9 5
3 3 8 . 3 5 1 3 3 0 . 8 4 2 4 E2 4 6 6
3 6 3 . 9 5 1 5 3 7 . 2 4 2 4 E2 4 6 4
3 7 9 . 6 5 1 7 1 0 . 3 3 4 3 E2 3 6 4
3 9 6 . 0 5 1 9 3 3 . 2 3 0 4 E2 3 2 4
4 1 5 . 0 5 2 1 2 5 . 3 3 4 4 E2 3 5 4
4 2 5 . 5 5 2 3 5 8 . 7 2 4 4 E2 2 5 4
4 4 4 . 8 5 2 5 7 0 . 1 3 2 6 E2 3 4 6
4 5 2 . 3 5 2 8 1 1 . 0 1 7 4 E2 1 7 4
4 7 0 . 8 5 3 0 4 0 . 9 1 5 4 E2 1 6 4
4 7 6 . 7 5 3 2 8 7 . 7 1 0 4 E2 1 1 4
† Not observed by 1999Co02 but taken from adopted gammas.
2 8 7 4
228
29Ac133
228
29Ac133NUCLEAR DATA SHEETS
Adopted Levels
Q(β–)=–582 13 ; S(n)=5970 50 ; S(p)=3631 7 ; Q(α )=7137.4 20 2003Au03,2011AuZZ.
222Ac Levels
E(level) Jπ T1/2 Comments
0 . 0 1 – 5 . 0 s 5 %α=99 1 ; %ε+%β+=1 1 .
Possible ε branching was estimated by 1966Wa23 as 1 to 2% from Iα (7.13–MeV a) of 218Rn shown in 222Ac α spectrum by 1964Mc21.
Jπ : favored α decay (HF=2.6) to 1– g.s. of 218Fr.
T1/2: from measured values of 5.5 s 5 (1952Me13) and 4.2 s 5 (1958To25). Other measurement: 5 s 1
(1972Es03).
Assignment: daughter 226Pa (1952Me13,1964Mc21,1968Ha14).
See 2004Ho12 for predictions of cluster decay.
0 . 0 + x 6 3 s 3 %α≥88; %IT≤10; 0.7≤%ε+%β+≤2 (1972Es03).
%IT was deduced by 1972Es03 from ratio of Iα ' s of 5–s 222Ac and 63–s 222Ac.
%ε+%β+ was deduced by 1972Es03 from the intensities of α ' s from 218Rn, 214Po and 63–s 222Ac.
E(level) : x=E(level in 218Fr fed by 7000α of 63–s isomer)–(14 21 ) , deduced from Eα=7013 2 and
7000 20 of 5.0–s and 63–s state α decay, respectively.
T1/2: from measured values of 66 s 3 (1972Es03), 62 s 5 (1973Mo07), 60 s 4 (1982Bo04).
Assignment: Pb(18O,pxn) excit (1972Es03); parent of 218Fr (7870α ) , parent of 214At (8810α ) , parent
of 218Rn (7130α ) , parent of 5–s 222Ac (1972Es03).
On the basis of measured production cross–section ratio, 1972Es03 suggested that the 63–s isomeric
state has higher spin than the spin of 5.0–s g.s.
4 1 1 4 Level seen in 226Pa α decay.
1 3 7 1 4 Level seen in 226Pa α decay.
226Pa αααα Decay
Parent 226Pa: E=0.0; Jπ=?; T1/2=1.8 min 2 ; Q(g.s. )=6987 10 ; %α decay=74 5 .
For a review of α decay from oriented nuclei , see 1992Wo14.
222Ac Levels
E(level) Jπ
0 . 0 1 –
4 1 1 4
1 3 7 1 4
α radiations
Eα† E(level) Iα‡# HF§
6 7 2 9 1 0 1 3 7 1 9 1 1 4
6 8 2 4 1 0 4 1 4 6 4 . 7 7
6 8 6 4 1 0 0 . 0 5 2 6 . 0 9
† Measured by 1964Mc21. Original energies have been increased by 6 keV because of a change in the calibration energy of the 227Pa
α from 6460 to 6465.8 3 , recommended by 1991Ry01. Other measurements: 1951Me10, 1968Ha14, 1988Hu08.
‡ From 1964Mc21.
§ r0(222Ac)=1.536 4 is used in calculations.
# For α intensity per 100 decays, multiply by 0.74 5 .
2 8 7 5
229
20Th132–1 22
920Th132–1NUCLEAR DATA SHEETS
Adopted Levels, Gammas
Q(β–)=–4910 SY ; S(n)=7806 15 ; S(p)=4610 50 ; Q(α )=8127 5 2003Au03,2011AuZZ.
Estimated: ΔQ(β–)=70 (2003Au03,2011AuZZ).
See 1982Du16, 1982Le19, 1983Ro14, 1984Na22, 1988So08, 1989Eg02 for calculations of equil ibrium deformations and
discussions of deformation parameters.
See 1987Na10, 1985Na07, 1984Fr06 and 1984Na08 for studies on the shapes of the rotating nuclei .
See 2010Gu18 for microscopic description of nuclear shape evolution from spherical to octupole–deformation.
See 2009Qi07 for predictions of 14C cluster decay using universal decay law.
See 1991Bu10 for theoretical calculations of intrinsic–dipole moments by including β (2) – β (8) deformations which
were taken from 1988So08. Using the ground–state deformation parameters of 1984Na22, the macroscopic dipole moment
was calculated by 1986Do03. See also 2004Ad15, 2003Ad32.
Theoretical values of the reduced dipole and quadrupole transition probabil it ies were calculated, and their ratios
were compared with experimental ratios by 1995De13, 1993Dz01, 1988Ot02, 1987Ka37, 1987Na10, 1986Le05.
The level energies of the g.s. band up to the 26+ state and of the octupole–vibrational band up to the 25– state
were calculated by 1995De13 by considering higher order of deformations. See 1995De13 for calculations,
discussions and comparison with experiments. See also 1988Na08, 1988Ot02, 2005Za02, 2003Sh02, 2001Za04, 2001Za09,
1999Jo17.
The changes in calculated binding energies due to varying the 26 pole deformation parameters were studied by
1986Ch23.
Possible decay by 26Ne emission was studied and partial half–li fe relative to α decay half–li fe was calculated by
1990Sh01.
222Th Levels
The Kπ=0+ g.s. band and the Kπ=0– band at 467.0 keV have been interpreted as octupole parity–doublet bands. This
nucleus l ies in the left part of the octupole deformation defined by the spin systematics for octupole shapes
(1990Ja11).
Cross Reference (XREF) Flags
A 226U α Decay
B (HI,xnγ )
E(level) Jπ† XREF T1/2‡ Comments
0 . 0 § 0 + AB 2 . 8 ms 3 %α=100.
Branching: only α decay has been observed.
%ε<1.3×10–8 from log f t>5.9 for an ε branch to g.s.
T1/2: from 1970Va13. Other measurements: 4 ms 1 (1970To07), 2.6 ms 6 (1990AnZU), 2.2
ms 2 (1991AnZZ).
1 8 3 . 3 § 2 + AB 2 4 0 p s 2 0
4 3 9 . 8 § 4 + B 4 6 p s 6
4 6 7 . 0 # 3 – B
6 5 1 . 0 # 5 – B
7 5 0 . 0 § 6 + B ≤ 4 5 p s
9 2 3 . 5 # 7 – B
1 0 9 3 . 5 § 8 + B
1 2 5 5 . 3 # 9 – B
1 4 6 1 . 1 § 1 0 + B
1 6 2 2 . 6 # 1 1 – B
1 8 5 0 . 7 § 1 2 + B
2 0 1 5 . 5 # 1 3 – B
2 2 5 9 . 7 § 1 4 + B
2 4 3 1 . 9 # 1 5 – B
2 6 8 7 . 8 § 1 6 + B
2 8 7 3 . 0 # 1 7 – B
3 1 3 3 . 5 § 1 8 + B
3 3 4 0 . 7 # 1 9 – B
3 5 9 6 . 0 § 2 0 + B
3 8 3 5 . 5 # 2 1 – B
4 0 7 7 . 6 § 2 2 + B
4 3 4 9 . 5 # 2 3 – B
4 5 7 7 . 9 § 2 4 + B
4 8 8 2 . 5 ? # ( 2 5 – ) B
5 0 9 7 . 9 ? § ( 2 6 + ) B
† All excited state properties are from (HI,xnγ ) reaction data. Jπ are based upon γ multipolarities and fits to rotational bands.
‡ The excited state half–lives were measured by 1985Bo32. See (HI,xnγ ) reaction section.
§ (A): Kπ=0+ g.s. band.
# (B): Kπ=0– octupole–vibrational band.
2 8 7 6
229
20Th132–2 22
920Th132–2NUCLEAR DATA SHEETS
Adopted Levels, Gammas (continued)
γ (222Th)
E(level) Eγ† Mult.‡ α I(γ+ce)§ Comments
1 8 3 . 3 1 8 3 . 3 E2 0 . 9 3 1 B(E2)(W.u.)=74 7 .
4 3 9 . 8 2 5 6 . 5 E2 0 . 2 8 3 B(E2)(W.u.)=108 15 .
4 6 7 . 0 2 8 3 . 7
6 5 1 . 0 2 1 1 . 2 E1 0 . 0 8 3 6
7 5 0 . 0 9 9 . 1 ( E1 ) 0 . 1 2 2 7 1 . 6 B(E1)(W.u.)≥0.0015.
3 1 0 . 2 E2 0 . 1 5 5 1 0 0 B(E2)(W.u.)≥27.
9 2 3 . 5 1 7 3 . 3 E1 0 . 1 3 4 1 0 0
2 7 2 . 5 ( E2 ) 0 . 2 3 2 8 . 7
1 0 9 3 . 5 1 7 0 . 4 E1 0 . 1 4 0 1 0 0
3 4 3 . 5 E2 0 . 1 1 5 2 6 . 3
1 2 5 5 . 3 1 6 1 . 2 E1 0 . 1 6 0 1 0 0
3 3 1 . 8 E2 0 . 1 2 7 3 1 . 8
1 4 6 1 . 1 2 0 6 . 4 E1 0 . 0 8 8 1 0 0
3 6 7 . 6 E2 0 . 0 9 5 1 8 . 3
1 6 2 2 . 6 1 6 0 . 9 ( E1 ) 0 . 1 6 0 1 0 0
3 6 7 . 3 E2 0 . 0 9 5 4 3 . 1
1 8 5 0 . 7 2 2 8 . 5 E1 0 . 0 7 0 0 1 0 0
3 8 9 . 6 E2 0 . 0 8 1 3 2 6 . 5
2 0 1 5 . 5 1 6 4 . 6 E1 0 . 1 5 2 1 0 0
3 9 2 . 9 E2 0 . 0 7 9 5 4 7 . 5
2 2 5 9 . 7 2 4 4 . 3 E1 0 . 0 5 9 7 1 0 0
4 0 9 . 0 E2 0 . 0 7 1 5 1 5 . 3
2 4 3 1 . 9 1 7 2 . 0 ( E1 ) 0 . 1 3 7 1 0 0
4 1 6 . 4 E2 0 . 0 6 8 3 7 3 . 8
2 6 8 7 . 8 2 5 6 . 1 E1 0 . 0 5 3 6 1 0 0
4 2 8 . 1 E2 0 . 0 6 3 6 6 0
2 8 7 3 . 0 1 8 5 . 0 ( E1 ) 0 . 1 1 5 1 0 0
4 4 1 . 1 E2 0 . 0 5 8 9 8 3 . 5
3 1 3 3 . 5 2 6 0 . 2 1 0 0
4 4 5 . 7 2 8 . 2
3 3 4 0 . 7 2 0 7 . 5 1 0 0
4 6 7 . 7 5 4 . 0
3 5 9 6 . 0 2 5 5 1 0 0
4 6 2 . 5 E2 0 . 0 5 2 4 4 0 . 0
3 8 3 5 . 5 2 3 9 . 2 1 0 0
4 9 4 . 8 3 3 . 3
4 0 7 7 . 6 2 4 3 1 0 0
4 8 1 . 6 6 5 . 0
4 3 4 9 . 5 2 7 3
5 1 4
4 5 7 7 . 9 2 2 8 ≈ 1 1 0
5 0 0 . 3 1 0 0
4 8 8 2 . 5 ? 3 0 4 #
5 3 3 . 3
5 0 9 7 . 9 ? 2 1 7 #
5 2 0 . 0
† From (HI,xnγ ) data.
‡ All γ properties are from (HI,xnγ ) reaction data.
§ Relative transition intensity deexciting each level .
# Placement of transition in the level scheme is uncertain.
(A) Kπ=0+ g.s. band
(B) Kπ=0- octupole-vibrational band
0.00+
183.32+
439.84+
750.06+
1093.58+
1461.110+
1850.712+
2259.714+
2687.816+
3133.518+
3596.020+
4077.622+
4577.924+
5097.9(26+)
183
256
310
344
368
390
409
428
446
462
482
500
520
467.03-
651.05-
923.57-
1255.39-
1622.611-
2015.513-
2431.915-
2873.017-
3340.719-
3835.521-
4349.523-
4882.5(25-)
272
332
367
393
416
441
468
495
514
533
222
90Th132
2 8 7 7
229
20Th132–3 22
920Th132–3NUCLEAR DATA SHEETS
2 8 7 8
229
20Th132–4 22
920Th132–4NUCLEAR DATA SHEETS
226U αααα Decay
Parent 226U: E=0.0; Jπ=0+; T1/2=0.35 s 15 ; Q(g.s. )=7715 14 ; %α decay=100.
T1/2(226U)=0.20 s 5 was measured by 1990An22,0.5 s 2 by 1973Vi10, 0.281 s 9 by 2000He17, 0.260 s 20 by 2001Ku07,
0.260 s 10 by 1999Gr28.
See 2009Ni06, 2009Ro06, 2008Sa40, 2007Pe30, for calculations of alpha decay half–lives.
%α (226U)=100 is adopted in 1996Ak02. From the gross β– decay calculations of 1973Ta30, the ε decay branch is
estimated to be %ε<0.05.
1997Mo25 calculated the partial half–li fe of 226U β+ decay as >100 s.
Q(α ) (226U)=7701 4 is recommended by 2003Au03, 2011AUZZ.
222Th Levels
E(level) Jπ
0 . 0 † 0 +
1 8 3 . 3 † 2 +
† (A): K=0+ g.s. band.
α radiations
Eα† E(level) Iᆧ HF‡
7 3 8 7 7 1 8 3 . 3 1 5 5 1 . 4 8
7 5 6 6 4 0 . 0 8 5 1 1 1 . 0
† Measurement by 2001Ku07. Others: 1999Gr28, 2000He17.
‡ r0(222Th)=1.628 23 is used in calculations. The calculated radius parameters by
using various half–lives are r0=1.506 23 for T1/2=0.5 s 2 , r0=1.548 20 for T1/2=0.20
s 5 , and r0=1.543 22 for T1/2=0.22 8 (the weighted average of 0.5 s 2 and 0.20 s 2 ) .
§ Absolute intensity per 100 decays.
(HI,xn γγγγ)
208Pb(18O,4nγ ) , 208Pb(17O,3nγ ) pulsed beams, E≈95 MeV (1983Wa20).
208Pb(18O,4nγ ) , E=88–96 MeV (1985Bo32).
208Pb(18O,4nγ ) , E=95 MeV (1987KoZF).
208Pb(18O,4nγ ) E=94 MeV (1988ScZN,1988HaZJ).
208Pb(18O,4n) E=95 MeV (1996Bu53,1997Jo15).
208Pb(18O,4n) E=95 MeV (1995Sm06).
γγ , γ (θ ) : 1983Wa20, 1985Bo32.
From the experimental B(E1)/B(E2) ratios which were calculated from the γ intensities, the octupole deformation of
0.25 was inferred by 1986Sc18. Numerous theoretical calculations have been done for the deformation parameters of
the ground state and high–spin states. See the adopted levels for the references. See 1996Bu53 and 1997Jo15 for
study of yrast transition upto 12+ using using sacred array for conversion electron spectroscopy. See also
1997Ju03, 1996Bu26.
1995Sm06 observed shape transition at spin (24+). These results are consistent with the theoretical predictions of
1987Na10.
222Th Levels
E(level) Jπ‡ T1/2†
0 . 0 § 0 +
1 8 3 . 3 § 2 + 2 4 0 p s 2 0
4 3 9 . 8 § 4 + 4 6 p s 6
4 6 7 . 0 # 3 –
6 5 1 . 0 # 5 –
7 5 0 . 0 § 6 + ≤ 4 5 p s
9 2 3 . 5 # 7 –
1 0 9 3 . 5 § 8 +
1 2 5 5 . 3 # 9 –
E(level) Jπ‡
1 4 6 1 . 1 § 1 0 +
1 6 2 2 . 6 # 1 1 –
1 8 5 0 . 7 § 1 2 +
2 0 1 5 . 5 # 1 3 –
2 2 5 9 . 7 § 1 4 +
2 4 3 1 . 9 # 1 5 –
2 6 8 7 . 8 § 1 6 +
2 8 7 3 . 0 # 1 7 –
3 1 3 3 . 5 § 1 8 +
E(level) Jπ‡
3 3 4 0 . 7 # 1 9 –
3 5 9 6 . 0 § 2 0 +
3 8 3 5 . 5 # 2 1 –
4 0 7 7 . 6 § 2 2 +
4 3 4 9 . 5 # 2 3 –
4 5 7 7 . 9 § 2 4 +
4 8 8 2 . 5 ? # ( 2 5 – )
5 0 9 7 . 9 ? § ( 2 6 + )
† Measured by 1985Bo32 by recoil shadow method.
‡ From 1983Wa20, 1985Bo32 and 1988HaZJ.
§ (A): K=0 g.s. band.
# (B): K=0 octupole vibrational band.
2 8 7 9
229
20Th132–5 22
920Th132–5NUCLEAR DATA SHEETS
(HI,xn γγγγ) (continued)
γ (222Th)
Eγ† E(level) Mult.§ α I(γ+ce)‡
9 9 . 1 7 5 0 . 0 ( E1 ) 0 . 1 2 2 3 3 . 0
x 1 3 1 . 2 # E1 0 . 2 6 1 7@ 1
x 1 4 4 . 9 # E1 0 . 2 0 6 7@ 1
1 6 0 . 9 1 6 2 2 . 6 E1 0 . 1 6 0 2 9
1 6 1 . 2 1 2 5 5 . 3 E1 0 . 1 6 0 5 0
1 6 4 . 6 2 0 1 5 . 5 E1 0 . 1 5 2 2 2 . 1
1 7 0 . 4 1 0 9 3 . 5 E1 0 . 1 4 0 5 9 . 4
1 7 2 . 0 2 4 3 1 . 9 ( E1 ) 0 . 1 3 7 1 4 . 5
1 7 3 . 3 9 2 3 . 5 E1 0 . 1 3 4 6 8 . 6
1 8 3 . 3 1 8 3 . 3 E2 0 . 9 3 1 1 0 0
1 8 5 . 0 2 8 7 3 . 0 ( E1 ) 0 . 1 1 5 7 . 9
x 1 9 9 . 6 # E1 0 . 0 9 6 4@ 1
2 0 6 . 4 1 4 6 1 . 1 E1 0 . 0 8 8 4 7
2 0 7 . 5 3 3 4 0 . 7 [ E1 ] 0 . 0 8 7 5
2 1 1 . 2 6 5 1 . 0 E1 0 . 0 8 3 6 6 5 . 7
2 1 7 a 5 0 9 7 . 9 ?
2 2 8 4 5 7 7 . 9 [ E1 ] 0 . 0 7 0 0 ≈ 1
2 2 8 . 5 1 8 5 0 . 7 E1 0 . 0 7 0 0 2 3
x 2 3 1 . 8 # E1 0 . 0 6 7 4 4@ 1
2 3 9 . 2 3 8 3 5 . 5 [ E1 ] 0 . 0 6 2 7 3
2 4 3 4 0 7 7 . 6 [ E1 ] 0 . 0 6 0 4 2
2 4 4 . 3 2 2 5 9 . 7 E1 0 . 0 5 9 7 1 7
x 2 5 1 . 0 # E2 0 . 3 0 4 2 3@ 2
2 5 5 3 5 9 6 . 0 [ E1 ] 0 . 0 5 4 1 4
2 5 6 . 1 2 6 8 7 . 8 E1 0 . 0 5 3 6 1 0
2 5 6 . 5 4 3 9 . 8 E2 0 . 2 8 3 1 1 8
2 6 0 . 2 3 1 3 3 . 5 [ E1 ] 0 . 0 5 1 7 7 . 8
2 7 2 . 5 9 2 3 . 5 ( E2 ) 0 . 2 3 2 6 . 0
Eγ† E(level) Mult.§ α I(γ+ce)‡
2 7 3 4 3 4 9 . 5 [ E1 ] 0 . 0 4 6 4 ≈ 1
2 8 3 . 7 4 6 7 . 0 5 . 0
x 2 9 5 . 5 # 5@ 1
3 0 4 a 4 8 8 2 . 5 ?
3 1 0 . 2 7 5 0 . 0 E2 0 . 1 5 5 4 6 . 1
x 3 2 1 . 9 # E2 0 . 1 3 9 6@ 1
3 3 1 . 8 1 2 5 5 . 3 E2 0 . 1 2 7 1 5 . 9
3 4 3 . 5 1 0 9 3 . 5 E2 0 . 1 1 5 1 5 . 6
3 6 7 . 3 1 6 2 2 . 6 E2 0 . 0 9 5 1 2 . 5
3 6 7 . 6 1 4 6 1 . 1 E2 0 . 0 9 5 8 . 6
3 8 9 . 6 1 8 5 0 . 7 E2 0 . 0 8 1 3 6 . 1
3 9 2 . 9 2 0 1 5 . 5 E2 0 . 0 7 9 5 1 0 . 5
4 0 9 . 0 2 2 5 9 . 7 E2 0 . 0 7 1 5 2 . 6
4 1 6 . 4 2 4 3 1 . 9 E2 0 . 0 6 8 3 1 0 . 7
x 4 2 3 . 3 # E2 0 . 0 6 5 4 8@ 1
4 2 8 . 1 2 6 8 7 . 8 E2 0 . 0 6 3 6 6 . 0
4 4 1 . 1 2 8 7 3 . 0 E2 0 . 0 5 8 9 6 . 6
4 4 5 . 7 3 1 3 3 . 5 [ E2 ] 0 . 0 5 7 4 2 . 2
4 6 2 . 5 3 5 9 6 . 0 E2 0 . 0 5 2 4 1 . 6
4 6 7 . 7 3 3 4 0 . 7 [ E2 ] 0 . 0 5 1 0 2 . 7
4 8 1 . 6 4 0 7 7 . 6 [ E2 ] 0 . 0 4 7 4 1 . 3
x 4 8 5 . 8 # E2 0 . 0 4 6 5 3@ 1
4 9 4 . 8 3 8 3 5 . 5 [ E2 ] 0 . 0 4 4 5 1 . 1
5 0 0 . 3 4 5 7 7 . 9 [ E2 ] 0 . 0 4 3 1 0 . 9
5 1 4 4 3 4 9 . 5 [ E2 ] 0 . 0 4 0 4
5 2 0 . 0 5 0 9 7 . 9 ? [ E2 ] 0 . 0 3 9 3 0 . 7
5 3 3 . 3 4 8 8 2 . 5 ? [ E2 ] 0 . 0 3 7 1 0 . 8
† Excellent agreement among the energies measured by 1983Wa20, 1985Bo32 and 1988HaZJ. Eγ ' s of 1988HaZJ are given, except for
those transitions not placed on the level scheme. See also 1984Bu38 and 1987KoZF.
‡ Relative transition intensities, as shown by 1988HaZJ on their level scheme, are given, except where noted. The intensities are
normalized to I(γ+ce)(183.3γ )=100.
§ From ce work of 1985Bo32 and γ (θ ) measurements of 1983Wa20. Multipolarities in square brackets are from the level scheme.
# From 1985Bo32. In the authors ' later work, 1988HaZJ, although some additional γ ' s with lower intensities were placed on the
level scheme, these unplaced γ ' s are not mentioned. It is not clear whether or not their assignments to the 222Th level scheme
should be considered questionable.
@ From 1985Bo32.
a Placement of transition in the level scheme is uncertain.
x γ ray not placed in level scheme.
2 8 8 0
229
21Pa131
229
21Pa131NUCLEAR DATA SHEETS
Adopted Levels
Q(β–)=–2180 SY ; S(n)=6340 SY ; S(p)=2110 SY ; Q(α )=8850 SY 2003Au03,2011AuZZ.
Estimated ΔQ(β–)=120 ΔS(n)=90, ΔS(p)=70,ΔQ(α )=50 (2003Au03,2011AuZZ).
Assignment: 209Bi(16O,3n), 206Pb(19F,3n), excit (1970Bo13); 184W(40Ar,Pn) E=165–202 MeV, excit (1979Sc09); parent of
218Ac (9210α ) (1970Bo13,1979Sc09); parent of 214Fr (8430α ) (1979Sc09). See 1999Bo52 for production cross–section
measurements.
222Pa Levels
E(level) T1/2 Comments
0 . 0 2 . 9 ms + 6 – 4 %α=100.
Branching: only α decay was observed.
%ε+%β+≈4×10–4 from gross β– decay calculations (1973Ta30).
See 1985Po14 for calculation of heavy–ion emission probabil it ies.
T1/2: from 1979Sc09. Other measurement: 5.7 ms 5 (1970Bo13).
0 + x †
6 0 + x † 3 0
† Level was observed in 226Np α decay.
226Np αααα Decay
Parent 226Np: E=0.0; Jπ=?; T1/2=35 ms 10 ; Q(g.s. )=8200 50 ; %α decay=100.
226Np–%α decay: Only α decay of 226Np was observed.
Q(α ) (226Np)=8205 20+E(level in 222Pa populated by the 8060α ) . 2003Au03, 2011AuZZ give Q(α ) (226Np)=8200 50 .
T1/2(226Np)=31 ms 8 , measured by 1990Ni05.
222Pa Levels
E(level)
0 . 0 + x
6 0 + x 3 0
α radiations
Eα† E(level) Iα‡# HF§
8 0 0 0 2 0 6 0 + x 5 0 1 5 1 . 9 9
8 0 6 0 2 0 0 . 0 + x 5 0 1 5 2 . 9 1 3
† Measurement by 1993AnZS. Only one α group at 8044 20 was observed by 1990Ni05.
‡ α intensity per 100 α decay, measured by 1993AnZS.
§ r0(222Pa)=1.53 2 is used in calculations.
# Absolute intensity per 100 decays.
2 8 8 1
229
22U130
229
22U130NUCLEAR DATA SHEETS
Adopted Levels
S(n)=8360 SY ; S(p)=3370 SY ; Q(α )=9500 SY 2003Au03,2011AuZZ.
Estimated ΔS(n)=140, ΔS(p)=110, ΔQ(α )=100 (2003Au03,2011AuZZ).
calculation of ground state alpha decay half–li fe: 2001Mo07, 2007Pe30, 2009Ni06.
Assignment: natural W(40Ar,xn) E=180 MeV; products were separated from the primary beam by the velocity f i lter;
parent of 214Ra (7.16–MeV α ) (1983Hi12).
see 1988So08, 1984Na22 and 1982Le19 for calculation of nuclear–potential minimum and equilibrium deformations.
222U Levels
E(level) Jπ T1/2 Comments
0 . 0 0 + 1 . 0 μ s + 1 2 – 4 %α=100.
%ε+%β+<1×10–6 from gross β– decay calculations (1973Ta30).
Only α decay was observed.
T1/2: from 1983Hi12. α peak observed at 12.08 MeV was interpreted as the superposition of 222U and 218Th (T1/2=122 ns) decays. The half–li fe of 1.0 μs was calculated from correlated
7.16–MeV (of granddaughter 214Ra) and 12.08–MeV α–peak rates. The r0(218Th) parameter
deduced from HF(α to g.s. from 222U)=1.0 by using Q(α ) (222U)=9500 100 , Iα (to g.s. )=80% 20
and T1/2(α )=1.0 μs +10–4 is consistent with the local systematics.
2 8 8 2
NUCLEAR DATA SHEETS
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2 8 8 3
NUCLEAR DATA SHEETS
REFERENCES FOR A= 2 2 2 ( CONT I NUED )
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1 9 7 6Ku 0 8 W . K u r c e w i c z , N . K a f f r e l l , N . T r a u t m a n n , A . P l o c h o c k i , J . Z y l i c z , K . S t r y c z n i e w i c z , I . Y u t l a n d o v – N u c l . P h y s . A 2 7 0 , 1 7 5
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1 9 7 6Va ZC V . M . V a k h t e l , T . V y l o v , N . A . G o l o v k o v , V . M . G o r o z h a n k i n , B . S . D z h e l e p o v , R . B . I v a n o v , M . A . M i k h a i l o v a , V . G . C h u m i n –
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1 9 8 0Ka 4 1 S.G.Kadmensky, S.D.Kurgalin – Izv.Akad.Nauk SSSR, Ser.Fiz. 44, 1955 (1980)
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1 9 8 3Bu 1 4 D.D.Burgess, R.J.Tervo – Nucl.Instrum.Methods 214, 431 (1983)
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1 9 8 4Bu 3 8 J . D . B u r r o w s , P . A . B u t l e r , K . A . C o n n e l l , G . D . J o n e s , A . N . J a m e s , A . M . Y . E l – L a w i n d y , T . P . M o r r i s o n , J . S i m p s o n , R . W a d s w o r t h
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Phys.Rev.Lett. 53, 2060 (1984)
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1 9 8 5C o 2 4 A . C o c , C . T h i b a u l t , F . T o u c h a r d , H . T . D u o n g , P . J u n c a r , S . L i b e r m a n , J . P i n a r d , J . L e r m e , J . L . V i a l l e , S . B u t t g e n b a c h ,
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1 9 8 5Go 0 5 N . A . G o l v k o v , B . S . D z h e l e p o v , R . B . I v a n o v , M . A . M i k h a i l o v a – I z v . A k a d . N a u k S S S R , S e r . F i z . 4 9 , 2 1 ( 1 9 8 5 ) ;
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1 9 8 6Da 0 3 H.J.Daley, B.R.Barrett – Nucl.Phys. A449, 256 (1986)
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1 9 8 6Ru 1 1 V . A . R u b c h e n y a , V . P . E i s m o n t , S . G . Y a v s h i t s – I z v . A k a d . N a u k S S S R , S e r . F i z . 5 0 , 1 0 1 6 ( 1 9 8 6 ) ; B u l l . A c a d . S c i . U S S R ,
Phys.Ser. 50, No.5, 184 (1986)
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2 8 8 4
NUCLEAR DATA SHEETS
REFERENCES FOR A= 2 2 2 ( CONT I NUED )
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1 9 8 7C o 1 9 A . C o c , C . T h i b a u l t , F . T o u c h a r d , H . T . D u o n g , P . J u n c a r , S . L i b e r m a n , J . P i n a r d , M . C a r r e , J . L e r m e , J . L . V i a l l e ,
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1 9 8 7Ko ZF T.Kohno, Y.Gono, Ch.Briancon, F.A.Beck, and the Chateau de Cristal Collaboration – RIKEN–86, p.17 (1987)
1 9 8 7Mi 1 0 G.J.Miller, J.C.McGeorge, I .Anthony, R.O.Owens – Phys.Rev. C36, 420 (1987)
1 9 8 7Na 1 0 W.Nazarewicz, G.A.Leander, J.Dudek – Nucl.Phys. A467, 437 (1987)
1 9 8 7 P o 0 8 D.N.Poenaru, M.Ivascu, D.Mazilu, I .H.Plonski – Rev.Roum.Phys. 32, 283 (1987)
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1 9 8 7We 0 3 K . W e n d t , S . A . A h m a d , W . K l e m p t , R . N e u g a r t , E . W . O t t e n , H . H . S t r o k e , a n d t h e I S O L D E C o l l a b o r a t i o n – Z . P h y s . D 4 , 2 2 7
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1 9 8 8Ah 0 2 S . A . A h m a d , W . K l e m p t , R . N e u g a r t , E . W . O t t e n , P . – G . R e i n h a r d , G . U l m , K . W e n d t , a n d t h e I S O L D E C o l l a b o r a t i o n – N u c l . P h y s .
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1 9 8 8Ba 0 1 F.Barranco, R.A.Broglia, G.F.Bertsch – Phys.Rev.Lett. 60, 507 (1988)
1 9 8 8Ba 4 8 F.Barranco, E.Vigezzi , R.A.Broglia, G.F.Bertsch – Phys.Rev. C38, 1523 (1988)
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1 9 8 8Na 0 8 E . G . N a d z h a k o v , I . N . M i k h a i l o v – I z v . A k a d . N a u k S S S R , S e r . F i z . 5 2 , 1 1 1 ( 1 9 8 8 ) ; B u l l . A c a d . S c i . U S S R , P h y s . S e r . 5 2 , N o . 1 ,
104 (1988)
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1 9 8 9Bu 0 9 D . G . B u r k e , H . F o l g e r , H . G a b e l m a n n , E . H a g e b o , P . H i l l , P . H o f f , O . J o n s s o n , N . K a f f r e l l , W . K u r c e w i c z , G . L o v h o i d e n , K . N y b o ,
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1 9 8 9 P o 0 3 R . J . P o y n t e r , P . A . B u t l e r , G . D . J o n e s , R . J . T a n n e r , C . A . W h i t e , J . R . H u g h e s , S . M . M u l l i n s , R . W a d s w o r t h , D . L . W a t s o n ,
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1 9 9 0An ZU A.N.Andreev , D .D .Bogdanov , A .V .Eremin , A .P .Kabachenko , O .N .Malyshev , G .M.Ter–Akopyan , V . I .Chep ig in – J INR–P7–90–232
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1 9 9 0Bu 0 9 B.Buck, A.C.Merchant – J.Phys.(London) G16, L85 (1990)
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1 9 9 0N i 0 5 V . N i n o v , F . P . H e s s b e r g e r , P . A r m b r u s t e r , S . H o f m a n n , G . M u n z e n b e r g , M . L e i n o , Y . F u j i t a , D . A c k e r m a n n , W . M o r a w e k ,
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1 9 9 1An Z Z A . N . A n d r e e v , D . D . B o g d a n o v , A . V . E r e m i n , A . P . K a b a c h e n k o , O . N . M a l y s h e v , G . M . T e r – A k o p y a n , V . I . C h e p i g i n – P r o g r a m a n d
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1 9 9 1Bu 1 0 P.A.Butler, W.Nazarewicz – Nucl.Phys. A533, 249 (1991)
1 9 9 1Eg 0 1 J.L.Egido, L.M.Robledo – Nucl.Phys. A524, 65 (1991)
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2 8 8 5
NUCLEAR DATA SHEETS
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1 9 9 2De 4 4 D.S.Delion, A.Insolia, R.J.Liotta – Phys.Rev. C46, 1346 (1992)
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1 9 9 2 S k Z Z J . S k a l s k i , P . – H . H e e n e n , P . B o n c h e , H . F l o c a r d , J . M e y e r – P r o c . I n t . C o n f . N u c l e a r S t r u c t u r e a t H i g h A n g u l a r M o m e n t u m ,
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1 9 9 3An ZS A . N . A n d r e y e v , D . D . B o g d a n o v , V . I . C h e p i g i n , M . F l o r e k , A . P . K a b a c h e n k o , O . N . M a l y s h e v , S . S h a r o , G . M . T e r – A k o p i a n ,
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1 9 9 3Au 0 5 G.Audi, A.H.Wapstra – Nucl.Phys. A565, 1 (1993)
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1 9 9 3De 3 8 D.S.Delion, A.Insolia, R.J.Liotta – J.Phys.(London) G19, L189 (1993)
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2 8 8 6
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