neutral atom nuclear edm experiments investigating radium lorenz willmann kvi, groningen ect*...
TRANSCRIPT
![Page 1: Neutral atom nuclear EDM Experiments Investigating Radium Lorenz Willmann KVI, Groningen ECT* Trento, June 21-25, 2004](https://reader036.vdocuments.us/reader036/viewer/2022062410/5697bf841a28abf838c86e0f/html5/thumbnails/1.jpg)
Neutral atom nuclear EDM Neutral atom nuclear EDM ExperimentsExperiments
Investigating Radium
Lorenz WillmannKVI, Groningen
ECT* Trento, June 21-25, 2004
![Page 2: Neutral atom nuclear EDM Experiments Investigating Radium Lorenz Willmann KVI, Groningen ECT* Trento, June 21-25, 2004](https://reader036.vdocuments.us/reader036/viewer/2022062410/5697bf841a28abf838c86e0f/html5/thumbnails/2.jpg)
Outline
• Nuclear edm searches in neutral atoms (199Hg)• Are there other systems
Schiff Moment in Hg, Xe, Rn, Ra, Pu, TlFDzuba, et al., PRA 66, 012111 (2002).
• Enhancements favours Ra:Nuclear StructureAtomic Structure
• Can we exploit natures offer?Road to edm with Radium
![Page 3: Neutral atom nuclear EDM Experiments Investigating Radium Lorenz Willmann KVI, Groningen ECT* Trento, June 21-25, 2004](https://reader036.vdocuments.us/reader036/viewer/2022062410/5697bf841a28abf838c86e0f/html5/thumbnails/3.jpg)
Violation of T-Symmetry
H= -(d E+µ B) I/Id - electric dipole momentµ - magnetic dipole momentI - Spin
Limit for nuclear EDM Hgd< 2.1 x 10–28 e cm
M. V. Romalis et al. Phys.Rev.Lett. 86, 2505 (2001)
Radium: Excellent candidateV. A. Dzuba et al. Phys. Rev.A61 062509(2000)
EDMs violate- Parity- Time Reversal
![Page 4: Neutral atom nuclear EDM Experiments Investigating Radium Lorenz Willmann KVI, Groningen ECT* Trento, June 21-25, 2004](https://reader036.vdocuments.us/reader036/viewer/2022062410/5697bf841a28abf838c86e0f/html5/thumbnails/4.jpg)
EDM SearchesEDM Searches
• point particles e,,• nucleons n• atoms Tl, Cs, Hg, Ra• Molecules PbO, YbF, TlF
Any object will do need guidance by theory
units 10-27 e cm
exp SM new physics
e (Tl) < 3 10-11 1 < 1.05 109 10-8 200 < 3.1 1011 10-7 1700 n < 63 10-4 60 Tl (odd p) < 105 Hg (odd n) < 0.21 various
What is the source for an EDM?
![Page 5: Neutral atom nuclear EDM Experiments Investigating Radium Lorenz Willmann KVI, Groningen ECT* Trento, June 21-25, 2004](https://reader036.vdocuments.us/reader036/viewer/2022062410/5697bf841a28abf838c86e0f/html5/thumbnails/5.jpg)
EDM Now and in the FutureEDM Now and in the Future
1.610-27•
Start TRIP
•199Hg
Radium potential
de (SM) < 10-37
![Page 6: Neutral atom nuclear EDM Experiments Investigating Radium Lorenz Willmann KVI, Groningen ECT* Trento, June 21-25, 2004](https://reader036.vdocuments.us/reader036/viewer/2022062410/5697bf841a28abf838c86e0f/html5/thumbnails/6.jpg)
Fortson GroupSeattle, Washington
d < 2.1 10-28 e cm
199Hg Experiment, M. Romalis
![Page 7: Neutral atom nuclear EDM Experiments Investigating Radium Lorenz Willmann KVI, Groningen ECT* Trento, June 21-25, 2004](https://reader036.vdocuments.us/reader036/viewer/2022062410/5697bf841a28abf838c86e0f/html5/thumbnails/7.jpg)
From M. Romalis
Fortson GroupSeattle, Washington
![Page 8: Neutral atom nuclear EDM Experiments Investigating Radium Lorenz Willmann KVI, Groningen ECT* Trento, June 21-25, 2004](https://reader036.vdocuments.us/reader036/viewer/2022062410/5697bf841a28abf838c86e0f/html5/thumbnails/8.jpg)
Measure EDMMeasure EDM
Prepare Ensemblein Spin State J
Apply Electric Field E
Determination of Ensemble Spin Average
d = Je h
2 m cElectric Dipole Moment:
Precession Frequency:
= d x E
d = 10-25 e cmE = 100 kV/cm = 1.5 *10-5 rad/s
![Page 9: Neutral atom nuclear EDM Experiments Investigating Radium Lorenz Willmann KVI, Groningen ECT* Trento, June 21-25, 2004](https://reader036.vdocuments.us/reader036/viewer/2022062410/5697bf841a28abf838c86e0f/html5/thumbnails/9.jpg)
SensitivitySensitivity
P Polarization Efficiency N Number of particles per secondT Measurements Time Spin Coherence Time
Paramenters
1
P N T/)1/2S =
![Page 10: Neutral atom nuclear EDM Experiments Investigating Radium Lorenz Willmann KVI, Groningen ECT* Trento, June 21-25, 2004](https://reader036.vdocuments.us/reader036/viewer/2022062410/5697bf841a28abf838c86e0f/html5/thumbnails/10.jpg)
TRITRIPP Radium Permanent Radium Permanent EElectric lectric DDipole ipole MMomentoment
Benefits of RadiumBenefits of Radium • near degeneracy of near degeneracy of 33PP11 and and 33DD22 ~~ 40 000 enhancement40 000 enhancement
• some nuclei strongly deformedsome nuclei strongly deformed spin > 1/2 spin > 1/2 nuclear enhancement nuclear enhancement
50~500 50~500
66
Ra also interesting for weak interaction effectsAnapole moment, weak charge
(Dzuba el al., PRA 6, 062509)
![Page 11: Neutral atom nuclear EDM Experiments Investigating Radium Lorenz Willmann KVI, Groningen ECT* Trento, June 21-25, 2004](https://reader036.vdocuments.us/reader036/viewer/2022062410/5697bf841a28abf838c86e0f/html5/thumbnails/11.jpg)
Enhancement of EDMEnhancement of EDM• Heavy Atoms
~ Z2 (RN/RA)
• Induced Dipol Moment Polarizability in nucleus as well as atomic shell
• Example: Tl ~ -585, Fr ~ 1150, Ra ~ 40.000
DA = + c.c. < nl | -de
(-1) E | n’(l+1) > < n’ (l+1) | -er | nl > Enl – En’(l+1)n’
![Page 12: Neutral atom nuclear EDM Experiments Investigating Radium Lorenz Willmann KVI, Groningen ECT* Trento, June 21-25, 2004](https://reader036.vdocuments.us/reader036/viewer/2022062410/5697bf841a28abf838c86e0f/html5/thumbnails/12.jpg)
Experimental AspectsExperimental Aspects• CellsCells
high densitymotional fields average to zero long coherence times
• BeamsBeams ultra high vacuum leakage current suppression higher electric fields coherence time limited by length of beam
• TrapsTraps ??no motional electric field, higher densitylong storage time long observation timesultra high vacuum high electric fields possiblesmall sample region homogeneity
• New SystemsNew SystemsNew production facilities for short lived isotopes
![Page 13: Neutral atom nuclear EDM Experiments Investigating Radium Lorenz Willmann KVI, Groningen ECT* Trento, June 21-25, 2004](https://reader036.vdocuments.us/reader036/viewer/2022062410/5697bf841a28abf838c86e0f/html5/thumbnails/13.jpg)
IonCatcher
RFQCooler
AtomTrap
Particle Physics Production
TargetMagneticSeparator
MeV meVkeV eV neVAGORcyclotron
TRIP - Trapped Radioactive Isotopes:-laboratories for fundamental Physics
Beyond the Standard Model
TeV PhysicsEDM/-decay
http://www.kvi.nl/~trimp/web/html/trimp.html
![Page 14: Neutral atom nuclear EDM Experiments Investigating Radium Lorenz Willmann KVI, Groningen ECT* Trento, June 21-25, 2004](https://reader036.vdocuments.us/reader036/viewer/2022062410/5697bf841a28abf838c86e0f/html5/thumbnails/14.jpg)
Cold Radionuclides WorkCold Radionuclides Work
• Ion traps have been successful Physics Program: mass measurementsnuclear spectroscopycorrelations in -decay
• Now to neutral atomsShort lived isotopes become available for ‘atomic physics’ experiments.
Na, Ne, Rb, Fr, Cs-isotopes, Ra, …
• Worldwide efforts like in Argonne National Lab, GANIL, GSI, Jyvaskylae, KEK, KVI, Stony Brook, TRIUMF …
![Page 15: Neutral atom nuclear EDM Experiments Investigating Radium Lorenz Willmann KVI, Groningen ECT* Trento, June 21-25, 2004](https://reader036.vdocuments.us/reader036/viewer/2022062410/5697bf841a28abf838c86e0f/html5/thumbnails/15.jpg)
Target
Gas filled Separator
QDQD
QD QD
208 Pbbeam
T1
TrapExperiments
DD DD
Isotope production @ TRIP KVI
• Separator commissioned with Na production • Ra at TRIP Facility in couple of month
![Page 16: Neutral atom nuclear EDM Experiments Investigating Radium Lorenz Willmann KVI, Groningen ECT* Trento, June 21-25, 2004](https://reader036.vdocuments.us/reader036/viewer/2022062410/5697bf841a28abf838c86e0f/html5/thumbnails/16.jpg)
AGOR CyclotronAGOR Cyclotron
Adaptating to New ChallengesAdaptating to New Challenges
• Heavy Ion BeamsHeavy Ion Beams e.g. e.g. 208208PbPb new sourcesnew sources
new injection channelnew injection channelvacuum improvementvacuum improvement
• High Power High Power (TRI(TRIP would appreciate 1 kW)P would appreciate 1 kW)
improved extractionimproved extractionbeam stopsbeam stopsbeam monitoringbeam monitoringradiation safetyradiation safety
Expect 10Expect 1077 213213Ra/kW beamRa/kW beam
AGOR
![Page 17: Neutral atom nuclear EDM Experiments Investigating Radium Lorenz Willmann KVI, Groningen ECT* Trento, June 21-25, 2004](https://reader036.vdocuments.us/reader036/viewer/2022062410/5697bf841a28abf838c86e0f/html5/thumbnails/17.jpg)
TRITRIPP
x-ra
y co
unts
[ar
b.]
x-ray energy [channels]
raw data raw data
fitted x-ray spectrafitted x-ray spectra
extracted Fr x-raysextracted Fr x-rays
A. Rogachevsky, H. Wilschut, S. Kopecky,V. Kravchuk, K. Jungmann + AGOR team
FirstFirst TRITRIPP TestsTests1515N N ++ 205205Tl Tl 213213RaRa + 7n + 7n
213213FrFr
C Tl C
NN
RaRa
Fr x-raysFr x-rays
Production Test Production Test 213213RaRa
Expected Production Rates~ 107/s with 1kW primary beam
![Page 18: Neutral atom nuclear EDM Experiments Investigating Radium Lorenz Willmann KVI, Groningen ECT* Trento, June 21-25, 2004](https://reader036.vdocuments.us/reader036/viewer/2022062410/5697bf841a28abf838c86e0f/html5/thumbnails/18.jpg)
Radium SpectroscopyRadium Spectroscopy
What do we know?
![Page 19: Neutral atom nuclear EDM Experiments Investigating Radium Lorenz Willmann KVI, Groningen ECT* Trento, June 21-25, 2004](https://reader036.vdocuments.us/reader036/viewer/2022062410/5697bf841a28abf838c86e0f/html5/thumbnails/19.jpg)
Radium Spectroscopy DataRadium Spectroscopy DataRadium Discharge analyzed with grating spectrometer
Ebbe Rasmussen, Z. Phys, 87, 607 , 1934; Z. Phys, 86, 24, 1933.
Resolution ~ 0.05 A, 99 lines, absolute accuracy
[A]
Corrections in deduces energy levels
1S0-1P1 1S0-3P1
H.N. Russel, Phys. Rev. 46, 989 (1934)
[A]
Similar to Barium identification as alkaline earth element
![Page 20: Neutral atom nuclear EDM Experiments Investigating Radium Lorenz Willmann KVI, Groningen ECT* Trento, June 21-25, 2004](https://reader036.vdocuments.us/reader036/viewer/2022062410/5697bf841a28abf838c86e0f/html5/thumbnails/20.jpg)
482.7 nm
714 nm
7s2 1S0
7s 7p 1P1
7s 7p 3P
7s 6d 1D2
7s 6d 3D1
23
2
1
0
1438 nm1488 nm
2.8 m
Transitions in RadiumTransitions in Radium
Collinear laser spectroscopy 1S0 – 1P1 transitionS.A. Ahmad, W. Klempt, R. Neugart, E.W. Otten, P.-G. Reinhard, G. Ulm K. Wendt and ISOLDE collaboration,Nuclear Physics A483, 244 (1988)
• Spectroscopy of P and D states• Lifetime measurement• Energy level spacing• Hyperfine structure
To do list:
According to NIST Database
![Page 21: Neutral atom nuclear EDM Experiments Investigating Radium Lorenz Willmann KVI, Groningen ECT* Trento, June 21-25, 2004](https://reader036.vdocuments.us/reader036/viewer/2022062410/5697bf841a28abf838c86e0f/html5/thumbnails/21.jpg)
Laser Cooling ChartLaser Cooling Chart
Efficient production of cold atoms: Magneto Optical Trap
Other Possibilities: Buffer Gas loading into magnetic trapJ. Doyle, Harvard; A. Richter, Konstanz
KVIRIMSTrace analysis
Next Species
Ba
Ra
![Page 22: Neutral atom nuclear EDM Experiments Investigating Radium Lorenz Willmann KVI, Groningen ECT* Trento, June 21-25, 2004](https://reader036.vdocuments.us/reader036/viewer/2022062410/5697bf841a28abf838c86e0f/html5/thumbnails/22.jpg)
Cooling and TrappingCooling and TrappingType Energies Scale
Slowing 1000 m/sZeeman, white light, chirped laser, bichromatic force 100 meV
MOT 100 m/s inhomogeneous B-Field
Optical Molasses 10 m/s, 1 K no B-Field
FORT > 1 mK no B-Field
Magnetic Trap 0.7 K/T/B inhomogeneous B-Field
Cryogenic Buffer 0.7 K/T/B inhomogeneous B-FieldGas Loading
Trap losses: background gas ~1 s @ 10-9 mbaroptical traps not closed cycling scheme
![Page 23: Neutral atom nuclear EDM Experiments Investigating Radium Lorenz Willmann KVI, Groningen ECT* Trento, June 21-25, 2004](https://reader036.vdocuments.us/reader036/viewer/2022062410/5697bf841a28abf838c86e0f/html5/thumbnails/23.jpg)
Preliminary Transition Rates as calculated by K. Pachucky (also by V. Dzuba et al.)
Trappist’s ViewTrappist’s View
3*104 s-1
2.2*108 s-1
7s2 1S0
7s 7p 1P1
7s 7p 3P
7s 6d 1D2
7s 6d 3D1
23
2
1
0
1*105 s-1
3*105
1.6*106 s-1
4*103 s-1
CoolingTransition
Repumping necessary
1.4*10-1 s-1
Weaker line, second stage cooling
Repumping
![Page 24: Neutral atom nuclear EDM Experiments Investigating Radium Lorenz Willmann KVI, Groningen ECT* Trento, June 21-25, 2004](https://reader036.vdocuments.us/reader036/viewer/2022062410/5697bf841a28abf838c86e0f/html5/thumbnails/24.jpg)
Preliminary Transition Rates as calculated by K. Pachucky (also by V. Dzuba et al.)
Trappist’s ViewTrappist’s View
3*104 s-1
2.2*108 s-1
7s2 1S0
7s 7p 1P1
7s 7p 3P
7s 6d 1D2
7s 6d 3D1
23
2
1
0
1*105 s-1
3*105
1.6*106 s-1
4*103 s-1
![Page 25: Neutral atom nuclear EDM Experiments Investigating Radium Lorenz Willmann KVI, Groningen ECT* Trento, June 21-25, 2004](https://reader036.vdocuments.us/reader036/viewer/2022062410/5697bf841a28abf838c86e0f/html5/thumbnails/25.jpg)
Trappist’s ViewTrappist’s View
7s 6d 3D1
23
2.2*108 s-1
7s2 1S0
7s 7p 1P1
7s 7p 3P
7s 6d 1D22
1
0
1.6*106 s-1
Consequences for Laser Cooling with 1S0-3P1
Smaller Enhancement of EDMLonger Lifetime of 3D2 in E-Field
Energy levels calculation3D-States are lower
J. Biron & K. Pachucky (priv. Comm.)
7s 6d 3D1
23
![Page 26: Neutral atom nuclear EDM Experiments Investigating Radium Lorenz Willmann KVI, Groningen ECT* Trento, June 21-25, 2004](https://reader036.vdocuments.us/reader036/viewer/2022062410/5697bf841a28abf838c86e0f/html5/thumbnails/26.jpg)
RadiumRadium Spectroscopy Spectroscopy
• Laser Cooling• Metastable Beam
BariumBarium
![Page 27: Neutral atom nuclear EDM Experiments Investigating Radium Lorenz Willmann KVI, Groningen ECT* Trento, June 21-25, 2004](https://reader036.vdocuments.us/reader036/viewer/2022062410/5697bf841a28abf838c86e0f/html5/thumbnails/27.jpg)
Heavy Alkaline Earth Element: BariumHeavy Alkaline Earth Element: Barium
– 8.4nsecIs=14mW/cm2
1 2
3
• Life time measurement• Hyperfine structure• Laser cooling of barium• Develop trapping strategy
791.3 nm
6s2 1S0
6s 6p 1P1
6s 5d 1D2
6s 6p 3P210
1130 nm
1499 nm
6s 5d 3D
3 m1108 nm
– 1.4 µsecIs=30µW/cm2
553.7 nm
Ideal testing ground:
No report yet on laser cooling and trapping!No report yet on laser cooling and trapping!
![Page 28: Neutral atom nuclear EDM Experiments Investigating Radium Lorenz Willmann KVI, Groningen ECT* Trento, June 21-25, 2004](https://reader036.vdocuments.us/reader036/viewer/2022062410/5697bf841a28abf838c86e0f/html5/thumbnails/28.jpg)
Verdi pumpat 532 nm
Collimator
Ba Oven500C
PD
M1
BS
Dye Laser
PowerStabilization
PMT
AOM
Optical fiber from 791.3 nm diode laser
553.7 nm
Coherent 699Single mode dye laser
B
/2
First StepsFirst Steps
![Page 29: Neutral atom nuclear EDM Experiments Investigating Radium Lorenz Willmann KVI, Groningen ECT* Trento, June 21-25, 2004](https://reader036.vdocuments.us/reader036/viewer/2022062410/5697bf841a28abf838c86e0f/html5/thumbnails/29.jpg)
138 B
a
137 B
a F
=5 /
213
7 Ba
F=
5 /2
138 B
a
135 B
a13
6 Ba
in Polarization plane
Polarization plane
Fluorescence at 553.7 nm from different Barium isotopesFluorescence at 553.7 nm from different Barium isotopesC
oun
ts [
kH
z]
PMT
PMT
Cou
nts
[k
Hz]
Frequency [MHz]
Frequency [MHz]
![Page 30: Neutral atom nuclear EDM Experiments Investigating Radium Lorenz Willmann KVI, Groningen ECT* Trento, June 21-25, 2004](https://reader036.vdocuments.us/reader036/viewer/2022062410/5697bf841a28abf838c86e0f/html5/thumbnails/30.jpg)
Lifetime Measurement: Hanle effectLifetime Measurement: Hanle effect
Life time of 1P1 state
Laser || B field
eff = h/(2 gJ B1/2)
eff = 8 nsec 0.5sec
138Ba 136Ba
138Ba 136Ba
Cou
nts
[k
Hz]
Cou
nts
[k
Hz]
Cou
nts
[k
Hz]
Cou
nts
[k
Hz]
Magnetic Field [G]
Magnetic Field [G]
Magnetic Field [G]
Magnetic Field [G]
![Page 31: Neutral atom nuclear EDM Experiments Investigating Radium Lorenz Willmann KVI, Groningen ECT* Trento, June 21-25, 2004](https://reader036.vdocuments.us/reader036/viewer/2022062410/5697bf841a28abf838c86e0f/html5/thumbnails/31.jpg)
0 100 200 300 400 5000
20
40
60
Grou
nd St
ate D
eplet
ion [%
]
Power [W]
553.7 nm
791.3 nm
6s2 1S0
6s 6p 1P1
6s 6p 3P1
6s 5d 3D
3 m
1.4 µsec
8.4 nsec
40%
60%
Creation of intense beam of meta-stable D-state atoms
321
Intercombination line Intercombination line 11SS00––33PP11
![Page 32: Neutral atom nuclear EDM Experiments Investigating Radium Lorenz Willmann KVI, Groningen ECT* Trento, June 21-25, 2004](https://reader036.vdocuments.us/reader036/viewer/2022062410/5697bf841a28abf838c86e0f/html5/thumbnails/32.jpg)
-0.010 -0.005 0.000 0.005-2
-1
0
1
2
Iodi
ne S
igna
l
k + 12636.6632 cm-1 [cm-1]
FM Saturated absorption spectroscopy of IFM Saturated absorption spectroscopy of I22
DiodeLaser791.3 nm
I2 Oven
(560ºC)
M1
M3BS
BSPD
Lock-InAmp
FeedbackControl
VCO
/4 AOM
To Beat note
Lock point
Reference Line P(52)(0-15) transition
f=f0+f1 Sin(wt)
w=90.5kHz
599 MHz away from 1S0–3P1 in 138Ba
(almost one line/5GHz from 500-900nm)
![Page 33: Neutral atom nuclear EDM Experiments Investigating Radium Lorenz Willmann KVI, Groningen ECT* Trento, June 21-25, 2004](https://reader036.vdocuments.us/reader036/viewer/2022062410/5697bf841a28abf838c86e0f/html5/thumbnails/33.jpg)
390 400 410 420 430 500 510 520 530 540
0.7
0.8
0.9
1.0
1.1 138Ba136Ba
Dep
leti
on
[%
]
Offset Frequency to I2 reference Line [MHz]
1S0–3P1 transition in an External Magnetic field
= gJ µ mJ B
IS = 138Ba–136Ba= 108.5 (3) MHz
2.3 MHz (FWHM)
• Decay rate• Branching into 3D States
![Page 34: Neutral atom nuclear EDM Experiments Investigating Radium Lorenz Willmann KVI, Groningen ECT* Trento, June 21-25, 2004](https://reader036.vdocuments.us/reader036/viewer/2022062410/5697bf841a28abf838c86e0f/html5/thumbnails/34.jpg)
Competitors
![Page 35: Neutral atom nuclear EDM Experiments Investigating Radium Lorenz Willmann KVI, Groningen ECT* Trento, June 21-25, 2004](https://reader036.vdocuments.us/reader036/viewer/2022062410/5697bf841a28abf838c86e0f/html5/thumbnails/35.jpg)
RadiumRadium
• Promising candidate for experimental EDM searches
• Production of 213Ra at KVI this year at new TRIP Facility
• Spectroscopy is indispensableLifetimes and Hyperfine Structure
• Development toward trapping with Barium• EDM and Parity violating effects are strong
Next year more about it