main sources: transport through andreev bound states in a graphene quantum dot travis dirks, taylor...

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Main sources: Transport through Andreev Bound States in a Graphene Quantum Dot Travis Dirks, Taylor L. Hughes, Siddhartha Lal, Bruno Uchoa, Yung-Fu Chen, Cesar Chialvo, Paul M. Goldbart, Nadya Mason Department of Physics and Frederick Seitz Materials Research Laboratory, University of Illinois at Urbana-Champaign, Urbana, IL 61801, USA Nature Physics 7, 386–390 (2011) doi:10.1038/nphys1911 Superconducting proximity effect through graphene from zero field to the Quantum Hall regime. Katsuyoshi Komatsu, Chuan Li, S. Autier-Laurent, H. Bouchiat and S. Gueron Laboratoire de Physique des Solides, Univ. Paris-Sud, CNRS, UMR 8502, F- 91405 Orsay Cedex, France. Phys. Rev. B 86, 115412 (2012) Quantum Hall Effect in Graphene with Superconducting Electrodes Peter Rickhaus, Markus Weiss,* Laurent Marot, and Christian Schnenberger Endre Tóvári, 2012. dec. 13. Superconducting proximity effect in graphene, Andreev reflection next to Quantum Hall edge states

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Page 1: Main sources: Transport through Andreev Bound States in a Graphene Quantum Dot Travis Dirks, Taylor L. Hughes, Siddhartha Lal, Bruno Uchoa, Yung-Fu Chen,

Main sources:Transport through Andreev Bound States in a Graphene Quantum DotTravis Dirks, Taylor L. Hughes, Siddhartha Lal, Bruno Uchoa, Yung-Fu Chen, Cesar Chialvo, Paul M. Goldbart, Nadya MasonDepartment of Physics and Frederick Seitz Materials Research Laboratory, University of Illinois at Urbana-Champaign, Urbana, IL 61801, USANature Physics 7, 386–390 (2011) doi:10.1038/nphys1911

Superconducting proximity effect through graphene from zero field to the Quantum Hall regime.Katsuyoshi Komatsu, Chuan Li, S. Autier-Laurent, H. Bouchiat and S. GueronLaboratoire de Physique des Solides, Univ. Paris-Sud, CNRS, UMR 8502, F-91405 Orsay Cedex, France.Phys. Rev. B 86, 115412 (2012)

Quantum Hall Effect in Graphene with Superconducting ElectrodesPeter Rickhaus, Markus Weiss,* Laurent Marot, and Christian SchonenbergerDepartment of Physics, University of Basel, Klingelbergstrasse 82, 4056 Basel, SwitzerlandNano Lett., 2012, 12 (4), pp 1942–1945, DOI: 10.1021/nl204415s

Endre Tóvári, 2012. dec. 13.

Superconducting proximity effect in graphene, Andreev reflection next to Quantum Hall edge states

Page 2: Main sources: Transport through Andreev Bound States in a Graphene Quantum Dot Travis Dirks, Taylor L. Hughes, Siddhartha Lal, Bruno Uchoa, Yung-Fu Chen,

Transport through Andreev Bound States in a Graphene Quantum Dot

Andreev reflection—where an electron in a normal metal backscatters off a superconductor into a hole—forms the basis of low energy transport through superconducting junctions. Andreev reflection in confined regions gives rise to discrete Andreev bound states (ABS)

http://www.physics.wayne.edu/~nadgorny/research3.html http://arxiv.org/pdf/1005.0443.pdf

Travis Dirks, Taylor L. Hughes, Siddhartha Lal, Bruno Uchoa, Yung-Fu Chen, Cesar Chialvo, Paul M. Goldbart, Nadya MasonDepartment of Physics and Frederick Seitz Materials Research Laboratory, University of Illinois at Urbana-Champaign, Urbana, IL 61801, USANature Physics 7, 386–390 (2011) doi:10.1038/nphys1911

Page 3: Main sources: Transport through Andreev Bound States in a Graphene Quantum Dot Travis Dirks, Taylor L. Hughes, Siddhartha Lal, Bruno Uchoa, Yung-Fu Chen,

Transport through Andreev Bound States in a Graphene Quantum Dot

The shift shows bulk p-doping by the backgate and contacts.Asymmetry shows doping by contacts:

1 layer

10 layers

Work function mismatch at end contacts charge transferLow graphene DOS metal dominance p-doping under end leads

http://arxiv.org/pdf/0802.2267v3.pdf http://arxiv.org/pdf/0804.2040v1.pdf

Page 4: Main sources: Transport through Andreev Bound States in a Graphene Quantum Dot Travis Dirks, Taylor L. Hughes, Siddhartha Lal, Bruno Uchoa, Yung-Fu Chen,

Work-function mismatch under SC probe: charge density pinned below the contact local n-doping confinement

The ABS form when the discrete QD levels are proximity coupled to the superconducting contact (Andreev refl. + Coulomb charging effects)

Transport through Andreev Bound States in a Graphene Quantum Dot

For Dirac particles, it is not the height but the slope of the barrier that results in the scattering and possible confinement of charge carriers. Klein tunneling through smooth barriers CAN lead to confinement.

Rtunnel~10x-100xR2p

Page 5: Main sources: Transport through Andreev Bound States in a Graphene Quantum Dot Travis Dirks, Taylor L. Hughes, Siddhartha Lal, Bruno Uchoa, Yung-Fu Chen,

Transport through Andreev Bound States in a Graphene Quantum Dot

Pb:2Δ=2.6 meV

0,26 K0,45 K0,67 K0,86 K1,25 K1,54 K

Subgap peak amplitude, T↑:Decreasing until 0,8 K, constant after

Quantum regime: Classical dot regime:2

BE k T e C 2Bk T E e C

If U>>Δeff:↑ and ↓ are widely split in energy, promoting pair-braking, QD is like a normal metal.ABS are formed from the discrete QD states due to Andreev reflections on the SC-QD interface

If U<<Δeff, the spin-up and spin-down states of the QD are nearly degenerate. Near the EF of the SC, they are occupied by paired electrons/holes, and the QD effectively becomes incorporated as part of the SC interface. The conductance is then BTK-like and thus suppressed inside the gap, as in SC-normal interfaces having large tunnel barriers.

Page 6: Main sources: Transport through Andreev Bound States in a Graphene Quantum Dot Travis Dirks, Taylor L. Hughes, Siddhartha Lal, Bruno Uchoa, Yung-Fu Chen,

Transport through Andreev Bound States in a Graphene Quantum Dot

Tunneling differential conductance map (logarithmic scale):

Subgap peaks from ABS

A phenomenological model that considers the effect of the SC proximity coupling on a singlepair of spin-split QD states:

. .

shift g

shift g

eff c c

H E V c c

h

U E V c c

c

221

4 2 22

ABSg eff shift gE V U E V U

If U=0: E-ABS > |Δeff| for every Vg. U>Uc needed for subgap conductance.

From 1 pair of spin-split QD states just one ABS will be inside the gap (E-).

Superposition of particle and hole states

Page 7: Main sources: Transport through Andreev Bound States in a Graphene Quantum Dot Travis Dirks, Taylor L. Hughes, Siddhartha Lal, Bruno Uchoa, Yung-Fu Chen,

Transport through Andreev Bound States in a Graphene Quantum Dot

A fit of the conductance data from the detailed transport calculations for a quantum dot with two levels, a finite charging energy, and with couplings to normal metal and superconducting leads.

solid(dashed) lines represent states which have dominant particle(hole) character (ABS: hybridized e+h states)

Essential parts:•QD confined via a pn-junction in graphene (+U Coulomb charging energy is large enough)•the low density of states in graphene•the large tunneling barrier

Normal (single-particle) QD states do not contribute to subgap features.

2 subgap peaks (E-) from ABS: originated from 2 QD states (in this range)

Page 8: Main sources: Transport through Andreev Bound States in a Graphene Quantum Dot Travis Dirks, Taylor L. Hughes, Siddhartha Lal, Bruno Uchoa, Yung-Fu Chen,

http://arxiv.org/pdf/1005.0443.pdf

Revealing the electronic structure of a carbon nanotube carrying asupercurrentNature Physics 6, 965 (2010)

Page 9: Main sources: Transport through Andreev Bound States in a Graphene Quantum Dot Travis Dirks, Taylor L. Hughes, Siddhartha Lal, Bruno Uchoa, Yung-Fu Chen,

Superconducting proximity effect through graphene from zero field to the Quantum Hall regime.

Critical current vs gate voltage in zero magnetic field

Proximity effect in the Integer Quantum Hall regime

Superconductor-graphene-superconductor:SGS junction

http://www.gdr-meso.phys.ens.fr/uploads/Aussois_2011/komatsu_GDR_forPDF.pdf

Superconducting proximity effect:

Katsuyoshi Komatsu, Chuan Li, S. Autier-Laurent, H. Bouchiat and S. GueronLaboratoire de Physique des Solides, Univ. Paris-Sud, CNRS, UMR 8502, F-91405 Orsay Cedex, France.Phys. Rev. B 86, 115412 (2012)

Page 10: Main sources: Transport through Andreev Bound States in a Graphene Quantum Dot Travis Dirks, Taylor L. Hughes, Siddhartha Lal, Bruno Uchoa, Yung-Fu Chen,

Superconducting proximity effect through graphene from zero field to the Quantum Hall regime.

Superconducting proximity effect:

Critical current sensitive to:•Phase coherence length (must be longer than sample)•Interface quality•Ic suppressed by temperature

Nb, 200mK

ReW, 55mK

Ic suppressed around CNP (Dirac point)

CNP=charge neutrality point, n(Vg)≈0

Page 11: Main sources: Transport through Andreev Bound States in a Graphene Quantum Dot Travis Dirks, Taylor L. Hughes, Siddhartha Lal, Bruno Uchoa, Yung-Fu Chen,

Superconducting proximity effect through graphene from zero field to the Quantum Hall regime.

Superconducting proximity effect:

Critical current sensitive to:•Phase coherence length (must be longer than sample)•Interface quality•Ic suppressed by temperature

200 mK55 mK

There is not a constant factor between ETh/eRN and Ic.

max 20 , c Th N ThI T E eR E D L

Page 12: Main sources: Transport through Andreev Bound States in a Graphene Quantum Dot Travis Dirks, Taylor L. Hughes, Siddhartha Lal, Bruno Uchoa, Yung-Fu Chen,

All pairs (e+h) contribute to the supercurrent with their phase.Specular reflection: not time-reversed trajectories, suppressed current.

Superconducting proximity effect through graphene from zero field to the Quantum Hall regime.

Superconducting proximity effect:

Critical current sensitive to:•Phase coherence length (must be longer than sample)•Interface quality•Ic suppressed by temperature

Page 13: Main sources: Transport through Andreev Bound States in a Graphene Quantum Dot Travis Dirks, Taylor L. Hughes, Siddhartha Lal, Bruno Uchoa, Yung-Fu Chen,

C. W. J. Beenakker: Colloquium: Andreev reflection and Klein tunneling in graphene, REVIEWS OF MODERN PHYSICS, VOL 80, OCT.–DEC. 2008http://www.gdr-meso.phys.ens.fr/uploads/Aussois_2011/komatsu_GDR_forPDF.pdf

Superconducting proximity effect through graphene from zero field to the Quantum Hall regime.

Doped graphene Near Dirac point

retroreflection specular reflection

Ky and ε are conserved, but the reflected hole is in the other band!

Deshpande et al., Phys. Rev. B 83, 155409 (2011)

Page 14: Main sources: Transport through Andreev Bound States in a Graphene Quantum Dot Travis Dirks, Taylor L. Hughes, Siddhartha Lal, Bruno Uchoa, Yung-Fu Chen,

http://www.gdr-meso.phys.ens.fr/uploads/Aussois_2011/komatsu_GDR_forPDF.pdf

Page 15: Main sources: Transport through Andreev Bound States in a Graphene Quantum Dot Travis Dirks, Taylor L. Hughes, Siddhartha Lal, Bruno Uchoa, Yung-Fu Chen,

http://www.gdr-meso.phys.ens.fr/uploads/Aussois_2011/komatsu_GDR_forPDF.pdf

Page 16: Main sources: Transport through Andreev Bound States in a Graphene Quantum Dot Travis Dirks, Taylor L. Hughes, Siddhartha Lal, Bruno Uchoa, Yung-Fu Chen,

Superconducting proximity effect through graphene from zero field to the Quantum Hall regime.

70 mK; 0-7,5 T (<Bc for ReW)Quantum Hall effect in a wide sample

en Bh filling factor

2eG

h

due to inhomogeneities and scattering in the wide sample (imagine 3 parallel sheets)

Page 17: Main sources: Transport through Andreev Bound States in a Graphene Quantum Dot Travis Dirks, Taylor L. Hughes, Siddhartha Lal, Bruno Uchoa, Yung-Fu Chen,

Superconducting proximity effect through graphene from zero field to the Quantum Hall regime.

ReW, 70 mK, Vg=-7..4V,B=7,5 T, no offset!

Vg

ReW, 55 mK, Vg=0,offset by 100 Ω

B

Sometimes a dip in dV/dI at zero bias, depending on gate and field. Dips (peaks) mean alternating constructive (destructive) interference of Andreev pairs - signature of proximity effect.

conduction via a few edge statessometimes the total round-trip dephasing doesn’t average to zero (tuning of interference), unlike at B=0 (puddles, crit. current suppressed)

Page 18: Main sources: Transport through Andreev Bound States in a Graphene Quantum Dot Travis Dirks, Taylor L. Hughes, Siddhartha Lal, Bruno Uchoa, Yung-Fu Chen,

Superconducting proximity effect through graphene from zero field to the Quantum Hall regime.

Zero field: reduced supercurrent near charge neutrality point, due to dephasing originating from specular reflection at charge puddles.

High field – Quantum Hall regime:

(ReW: high Hc superrconductor)

Aharonov-Bohm type effect in the edge state

• ballistic-like conduction via a few channels (edge states)• for some puddle configs (Vg) and fields the total

dephasing doesn’t average to zero• tuning of interference, and thus of the proximity effect

Page 19: Main sources: Transport through Andreev Bound States in a Graphene Quantum Dot Travis Dirks, Taylor L. Hughes, Siddhartha Lal, Bruno Uchoa, Yung-Fu Chen,

Quantum Hall Effect in Graphene with Superconducting ElectrodesPeter Rickhaus, Markus Weiss,* Laurent Marot, and Christian SchonenbergerDepartment of Physics, University of Basel, Klingelbergstrasse 82, 4056 Basel, SwitzerlandNano Lett., 2012, 12 (4), pp 1942–1945, DOI: 10.1021/nl204415s

Quantum Hall regime: •electron hitting the superconductor-graphene S-G interface : Andreev retroreflection (if in the same band)•Andreev edge state (e and h orbits) propagates along the interface,•perfect interface: doubling of conductance

Nb: upper critical field ~4 T at 4K

widequadratic

Page 20: Main sources: Transport through Andreev Bound States in a Graphene Quantum Dot Travis Dirks, Taylor L. Hughes, Siddhartha Lal, Bruno Uchoa, Yung-Fu Chen,

Quantum Hall Effect in Graphene with Superconducting Electrodes

2-terminal:•G is a mixture of σxx and σxy

•wide sample: W/L~70, σxx dominates•no flat plateaus visible•but G minima are (LL steps)

enhanced G due to superconductivity below Bc, plus QHE

Page 21: Main sources: Transport through Andreev Bound States in a Graphene Quantum Dot Travis Dirks, Taylor L. Hughes, Siddhartha Lal, Bruno Uchoa, Yung-Fu Chen,

quadratic

2-terminal conductance on quadratic samples:•clear plateaus, despite the mixing•corrected for contact resistance by mathing QH plateau at B>Bc2

Quantum Hall Effect in Graphene with Superconducting Electrodes

cuts at constant filling factor

Nb: upper critical field ~4 T at 4K

3.2T 4T

Page 22: Main sources: Transport through Andreev Bound States in a Graphene Quantum Dot Travis Dirks, Taylor L. Hughes, Siddhartha Lal, Bruno Uchoa, Yung-Fu Chen,

Quantum Hall Effect in Graphene with Superconducting Electrodes

3.2T 4T

• 1.1, 1.4 and 1.8 factor decrease between 3.2 T and 4 T for ν=2, 6, 10 (narrow field range: no LL overlap)

• the conductance increase is more pronounced when more QH edge states are involved (ν=6, 10 )

• upper limit: factor of 2 (ideal, fully transparent S-N interface)

Page 23: Main sources: Transport through Andreev Bound States in a Graphene Quantum Dot Travis Dirks, Taylor L. Hughes, Siddhartha Lal, Bruno Uchoa, Yung-Fu Chen,

Quantum Hall Effect in Graphene with Superconducting Electrodes

ideal, fully transparent S-N interface: 2G0

incoming electron edge state scatters into 2 Andreev edge-states (hybridized electron-hole states, with τ1, 1-τ1 probability)

after propagating along the S-N interface, the Andreev edge states scatter to an electron or a hole edge state at the opposite edge (τ2, 1-τ2)

quasi-classical picture

Landauer-Büttiker picture

EPL, 91 (2010) 17005, doi: 10.1209/0295-5075/91/17005

2e2/h

Weak disorder at S-2DEG interface, with 1 spin-degenerate edge state

Page 24: Main sources: Transport through Andreev Bound States in a Graphene Quantum Dot Travis Dirks, Taylor L. Hughes, Siddhartha Lal, Bruno Uchoa, Yung-Fu Chen,

Quantum Hall Effect in Graphene with Superconducting Electrodes

With only the E=0 Landau level populated (ν = 2):conductance of the S-G interface only depends on the angle θ between the valley polarizations of incoming and outgoing edge-state

Identical opposite edges, ν = 2:

(If the superconductor covers a single edge, ϴ= 0 and no current can enter the superconductor (without intervalley scattering, for ν = 2). )

Weak disorder at S-G interface, with 1 spin-degenerate edge state

Phys. Rev. Lett. 2007, 98, 157003

Andreev reflection can be used to detect the valley polarization of edge states

probably strong intervalley scattering

Deviations are due to intervalley scattering

N=0 Landau level’s edge states are valley-polarized: ideally cosϴ=-1, doubling of conductancemeasurement: 1.1x increase in SC statestrong intervalley scattering

N=1, 2 Landau levels’ edge states are valley degenerate (unlike N=0):less sensitive to disorder+further from edgesstronger conductance enhancement

For clean edges, conductance doubling would be expected for all LLs

Page 25: Main sources: Transport through Andreev Bound States in a Graphene Quantum Dot Travis Dirks, Taylor L. Hughes, Siddhartha Lal, Bruno Uchoa, Yung-Fu Chen,

Thank you for your attention!