magnetic phases and critical points of insulators and superconductors colloquium article: reviews of...
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Magnetic phases and critical points of insulators and superconductors
Colloquium article:Reviews of Modern Physics, 75, 913 (2003).
Reviews:http://onsager.physics.yale.edu/qafm.pdf
cond-mat/0203363
Talks online: Sachdev
What is a quantum phase transition ?Non-analyticity in ground state properties as a function of some control parameter
g
T Quantum-critical
Why study quantum phase transitions ?
ggc• Theory for a quantum system with strong correlations: describe phases on either side of gc by expanding in deviation from the quantum critical point. • Critical point is a novel state of matter without quasiparticle excitations
• Critical excitations control dynamics in the wide quantum-critical region at non-zero temperatures.
OutlineOutline
A. “Dimerized” Mott insulators with a spin gap Tuning quantum transitions by applied pressure
B. Spin gap state on the square latticeSpontaneous bond order
C. Tuning quantum transitions by a magnetic field1. Mott insulators
2. Cuprate superconductors
S=1/2 spins on coupled dimers
jiij
ij SSJH
10
JJ
Coupled Dimer AntiferromagnetM. P. Gelfand, R. R. P. Singh, and D. A. Huse, Phys. Rev. B 40, 10801-10809 (1989).N. Katoh and M. Imada, J. Phys. Soc. Jpn. 63, 4529 (1994).J. Tworzydlo, O. Y. Osman, C. N. A. van Duin, J. Zaanen, Phys. Rev. B 59, 115 (1999).M. Matsumoto, C. Yasuda, S. Todo, and H. Takayama, Phys. Rev. B 65, 014407 (2002).
close to 0 Weakly coupled dimers
2
1
Excitation: S=1 triplon (exciton, spin collective mode)
Energy dispersion away from antiferromagnetic wavevector
2 2 2 2
2x x y y
p
c p c p
spin gap
close to 0 Weakly coupled dimers
2
1
S=1/2 spinons are confined by a linear potential into a S=1 triplon
TlCuCl3
N. Cavadini, G. Heigold, W. Henggeler, A. Furrer, H.-U. Güdel, K. Krämer and H. Mutka, Phys. Rev. B 63 172414 (2001).
“triplon” or spin exciton
close to 1Square lattice antiferromagnetExperimental realization: 42CuOLa
Ground state has long-rangemagnetic (Neel or spin density wave) order
01 0 NS yx iii
Excitations: 2 spin waves (magnons)2 2 2 2
p x x y yc p c p
1c
Neel state
0S N
T=0
in cupratesPressure in TlCuCl3
Quantum paramagnet
0S
c = 0.52337(3) M.
Matsumoto, C. Yasuda, S. Todo, and H. Takayama, Phys. Rev. B 65, 014407 (2002)
b
c
PHCC – a two-dimensional antiferromagnet
PHCC = C4H12N2Cu2Cl6
a
cCu
ClC
N
M. B. Stone, I. A. Zaliznyak, D. H. Reich, and C. Broholm, Phys. Rev. B 64, 144405 (2001).
(
meV
)
Dispersion to “chains”Dispersion to “chains”
Not chains but planesNot chains but planes
M. B. Stone, I. A. Zaliznyak, D. H. Reich, and C. Broholm, Phys. Rev. B 64, 144405 (2001).
PHCC – a two-dimensional antiferromagnet
(
meV
)
Dispersion to “chains”Dispersion to “chains”
Not chains but planesNot chains but planes
(m
eV)
0
1 0
1
h
Triplon dispersion
M. B. Stone, I. A. Zaliznyak, D. H. Reich, and C. Broholm, Phys. Rev. B 64, 144405 (2001).
PHCC – a two-dimensional antiferromagnet
S. Sachdev and R.N. Bhatt, Phys. Rev. B 41, 9323 (1990).
Quantitative theory of experiments and simulations: method of bond operators
Operators algebra for all states on a single dimer
† 10
2s s
†
†
†
10
2
02
10
2
x x
y y
z z
t t
it t
t t
† †
†
†
1
, 1
,
s s t t
s s
t t
Canonical Bose operators with a hard
core constraint
† † †1
† † †1
1
21
2
S s t t s i t t
S s t t s i t t
Spin operators on both sites can be expressed in terms of bond operators
Quantitative theory of experiments and simulations: method of bond operators
S. Sachdev and R.N. Bhatt, Phys. Rev. B 41, 9323 (1990). A. V. Chubukov and Th. Jolicoeur, Phys. Rev. B 44, 12050 (1991).
†
Hamiltonian for coupled dimers
Solve c 1 ,
o
nstraint by s t t
† † †
2 2
Triplon
2
d
ispe
rs
io
n
:
t k k k k k kk
B kH A k t t t t t t
k A k B k
222 2 2
Transition to magnetically ordered state occurs when 0 and the
bosons condense, lea
ding to 0
x x x y y yc k
t t
K c k K
Quantitative theory of experiments and simulations: method of bond operators
S. Sachdev and R.N. Bhatt, Phys. Rev. B 41, 9323 (1990).
3-component antiferromagnetic order parameter
22 22 2 2 21
2 4!x c
ud xd cS
2 2
; 2 c
c pp c
Field theory for quantum criticality
For oscillations of about 0 lead to the
following structure in the dynamic structure factor ,c
S p
,S p Z p
Three triplon continuum
Triplon pole
Structure holds to all orders in u~3
3-component antiferromagnetic order parameter
22 22 2 2 21
2 4!x c
ud xd cS
Field theory for quantum criticality
0For oscillations of about 0 lead to the
following dynamic structure factor ,c z
zz
N
longitudinal S p
,zzS p
Two spin-wave continuum
Structure holds to all orders in u~3
220 2N p
Entangled states at of order c
1/c
Triplon quasiparticle
weight Z
~ cZ
A.V. Chubukov, S. Sachdev, and J.Ye, Phys. Rev. B 49, 11919 (1994)
Antiferromagnetic moment N0
0 ~ cN
1/c
Triplon energy gap ~ c
1/c
,S p
Critical coupling c
c p
(2 ) / 22 2 2~ c p
No quasiparticles --- dissipative critical continuum
Dynamic spectrum at the critical point
Field theory for quantum criticality
Field theory for quantum criticality
Quantum criticality described by strongly-coupled critical theory with universal dynamic response functions dependent on
Triplon scattering amplitude is determined by kBT alone, and not by the value of microscopic coupling u
S. Sachdev and J. Ye, Phys. Rev. Lett. 69, 2411 (1992).
Bk T
, BT T g k T
Can such a state with bond order be the ground state of a system with full square lattice symmetry ?
Can such a state with bond order be the ground state of a system with full square lattice symmetry ?
Need additional exchange interactions with full square lattice symmetry to move out of Neel state into
paramagnet e.g. a second neighbor exchange J2. This defines a dimensionless coupling g = J2 / J
Collinear spins and compact U(1) gauge theory
Key ingredient: Spin Berry PhasesKey ingredient: Spin Berry Phases
iSAe
A
Write down path integral for quantum spin fluctuations
Collinear spins and compact U(1) gauge theory
iSAe
A
Write down path integral for quantum spin fluctuations
Key ingredient: Spin Berry PhasesKey ingredient: Spin Berry Phases
a n
0n
an
aA
a
Neel order parameter;
1 on two square sublattices ;
oriented area of spherical triangle
formed by and an ar
~
, ,
a a a
a
a a
S
A
n
n n 0bitrary reference poi t n n
Discretize imaginary time: path integral is over fields on the sites of a
cubic lattice of points a
Collinear spins and compact U(1) gauge theory
,
11 exp
22
a a a a a aa aa
iZ d A
g
n n n n
Partition function on square lattice
Modulus of weights in partition function: those of a classical ferromagnet at “temperature” g
0Small ground state has Neel order with 0
Large paramagnetic ground state with 0
Berry phases lead to large cancellations between different
time histories need an effective action for
a
a
g N
g
n
n
at large aA g
a n
0n
an
aA
a a
Change in choice of n0 is like a “gauge transformation”
a a a aA A
(a is the oriented area of the spherical triangle formed by na and the two choices for n0 ).
0n
aA
The area of the triangle is uncertain modulo 4and the action is invariant under4a aA A
These principles strongly constrain the effective action for Aawhich provides description of the large g phase
,
2 2
2
with
This is compact QED in
1 1e
+1 dimensions with
static char
xp co
ges 1 on two sublattice
s2
~
s.
22
a a a a aaa
d
iZ dA A A A
e
e g
Simplest large g effective action for the Aa
N. Read and S. Sachdev, Phys. Rev. Lett. 62, 1694 (1989).S. Sachdev and R. Jalabert, Mod. Phys. Lett. B 4, 1043 (1990).
K. Park and S. Sachdev, Phys. Rev. B 65, 220405 (2002).
For S=1/2 and large e2 , low energy height configurations are in exact one-to-one correspondence with nearest-neighbor valence bond pairings of the sites square lattice
There is no roughening transition for three dimensional interfaces, which are smooth for all couplings There is a definite average height of the interface Ground state has bond order.
N. Read and S. Sachdev, Phys. Rev. Lett. 62, 1694 (1989).
Smooth interface with average height 3/8
0
1/2
1/4
3/4
0
1/2
1/4
3/4
0 1/4 0 1/4
W. Zheng and S. Sachdev, Phys. Rev. B 40, 2704 (1989)
Smooth interface with average height 5/8
1
1/2
1/4
3/4
1
1/2
1/4
3/4
1 1/4 1 1/4
W. Zheng and S. Sachdev, Phys. Rev. B 40, 2704 (1989)
Smooth interface with average height 7/8
1
1/2
5/4
3/4
1
1/2
5/4
3/4
1 5/4 1 5/4
W. Zheng and S. Sachdev, Phys. Rev. B 40, 2704 (1989)
Smooth interface with average height 1/8
0
1/2
1/4
-1/4
0
1/2
1/4
-1/4
0 1/4 0 1/4
W. Zheng and S. Sachdev, Phys. Rev. B 40, 2704 (1989)
“Disordered-flat” interface with average height 1/2
1/2
1/4
3/4 1/2
1/4
3/4
1/4 1/4
W. Zheng and S. Sachdev, Phys. Rev. B 40, 2704 (1989)
0 1 0 1
0 1 0 1
“Disordered-flat” interface with average height 3/4
1/23/4 1/23/4
W. Zheng and S. Sachdev, Phys. Rev. B 40, 2704 (1989)
1/ 4
5 / 4
1 1
1 1
1/ 4
5 / 4
1/ 4
5 / 4
1/ 4
5 / 4
1/4
-1/4 -1/4
W. Zheng and S. Sachdev, Phys. Rev. B 40, 2704 (1989)
1/ 2
-1/ 2
0 0
0 0
“Disordered-flat” interface with average height 0
1/4
1/4
1/ 2
-1/ 2
1/4
1/4
W. Zheng and S. Sachdev, Phys. Rev. B 40, 2704 (1989)
3/ 4
-1/ 4
0 0
0 0
“Disordered-flat” interface with average height 1/4
1/4
1/4
3/ 4
-1/ 4
1/4
1/2 1/2
Two possible bond-ordered paramagnets for S=1/2
There is a broken lattice symmetry, and the ground state is at least four-fold degenerate.
Distinct lines represent different values of on linksi jS S
N. Read and S. Sachdev, Phys. Rev. Lett. 62, 1694 (1989).
g0
,
a 1 on two square sublattices ;
Neel order parameter;
oriented area of spheri
11
cal trian
exp2
~
g
l
2a a a a a a
a aa
a a a
a
iZ d A
g
S
A
n n n n
n
0,
e
formed by and an arbitrary reference point , a a n n n
A. W. Sandvik, S. Daul, R. R. P. Singh, and D. J. Scalapino, Phys. Rev. Lett. 89, 247201 (2002)
Bond order in a frustrated S=1/2 XY magnet
2 x x y yi j i j i j k l i j k l
ij ijkl
H J S S S S K S S S S S S S S
g=
First large scale numerical study of the destruction of Neel order in a S=1/2 antiferromagnet with full square lattice symmetry
g0
,
a 1 on two square sublattices ;
Neel order parameter;
oriented area of spheri
11
cal trian
exp2
~
g
l
2a a a a a a
a aa
a a a
a
iZ d A
g
S
A
n n n n
n
0,
e
formed by and an arbitrary reference point , a a n n n
g0
S. Sachdev and R. Jalabert, Mod. Phys. Lett. B 4, 1043 (1990). K. Park and S. Sachdev, Phys. Rev. B 65, 220405 (2002).
g
Critical theory is not expressed in terms of order parameter of either phase, but instead contains spinons interacting the a non-compact U(1) gauge force
Phase diagram of S=1/2 square lattice antiferromagnet
or
Neel order Spontaneous bond order, confined spinons, and “triplon” excitations
T. Senthil, A. Vishwanath, L. Balents, S. Sachdev and M.P.A. Fisher, submitted to Science
Use a sequence of simpler models which can be analyzed by duality mappings
A. Non-compact QED with scalar matterB. Compact QED with scalar matter
C. N=1: Compact QED with scalar matter and Berry phases D. theory
E. Easy plane case for N=2N
Nature of quantum critical point
Use a sequence of simpler models which can be analyzed by duality mappings
A. Non-compact QED with scalar matterB. Compact QED with scalar matter
C. N=1: Compact QED with scalar matter and Berry phases D. theory
E. Easy plane case for N=2N
Nature of quantum critical point
A. N=1, non-compact U(1), no Berry phases
C. Dasgupta and B.I. Halperin, Phys. Rev. Lett. 47, 1556 (1981).
Use a sequence of simpler models which can be analyzed by duality mappings
A. Non-compact QED with scalar matterB. Compact QED with scalar matter
C. N=1: Compact QED with scalar matter and Berry phases D. theory
E. Easy plane case for N=2N
Nature of quantum critical point
Use a sequence of simpler models which can be analyzed by duality mappings
A. Non-compact QED with scalar matterB. Compact QED with scalar matter
C. N=1: Compact QED with scalar matter and Berry phases D. theory
E. Easy plane case for N=2N
Nature of quantum critical point
Use a sequence of simpler models which can be analyzed by duality mappings
A. Non-compact QED with scalar matterB. Compact QED with scalar matterC. N=1: Compact QED with scalar matter and Berry phases
D. theoryE. Easy plane case for N=2
N
Nature of quantum critical point
Use a sequence of simpler models which can be analyzed by duality mappings
A. Non-compact QED with scalar matterB. Compact QED with scalar matterC. N=1: Compact QED with scalar matter and Berry
phases D. theoryE. Easy plane case for N=2
N
Nature of quantum critical point
Use a sequence of simpler models which can be analyzed by duality mappings
A. Non-compact QED with scalar matterB. Compact QED with scalar matter
C. N=1: Compact QED with scalar matter and Berry phases D. theory
E. Easy plane case for N=2N
Nature of quantum critical point
Identical critical theories!
Use a sequence of simpler models which can be analyzed by duality mappings
A. Non-compact QED with scalar matterB. Compact QED with scalar matter
C. N=1: Compact QED with scalar matter and Berry phases D. theory
E. Easy plane case for N=2N
Nature of quantum critical point
Identical critical theories!
g
Critical theory is not expressed in terms of order parameter of either phase, but instead contains spinons interacting the a non-compact U(1) gauge force
Phase diagram of S=1/2 square lattice antiferromagnet
or
Neel order Spontaneous bond order, confined spinons, and “triplon” excitations
T. Senthil, A. Vishwanath, L. Balents, S. Sachdev and M.P.A. Fisher, submitted to Science
OutlineOutline
A. “Dimerized” Mott insulators with a spin gap Tuning quantum transitions by applied pressure
B. Spin gap state on the square latticeSpontaneous bond order
C. Tuning quantum transitions by a magnetic field1. Mott insulators
2. Cuprate superconductors
1c
Neel state
0S N
T=0
in cupratesPressure in TlCuCl3
Quantum paramagnet
0S
c = 0.52337(3) M.
Matsumoto, C. Yasuda, S. Todo, and H. Takayama, Phys. Rev. B 65, 014407 (2002)
Effect of a field on paramagnet
Energy of zero
momentum triplon states
H
0
Bose-Einstein condensation of
Sz=1 triplon
TlCuCl3
Ch. Rüegg, N. Cavadini, A. Furrer, H.-U. Güdel, K. Krämer, H. Mutka, A. Wildes, K. Habicht, and P. Vorderwisch, Nature 423, 62 (2003).
TlCuCl3
Ch. Rüegg, N. Cavadini, A. Furrer, H.-U. Güdel, K. Krämer, H. Mutka, A. Wildes, K. Habicht, and P. Vorderwisch, Nature 423, 62 (2003).
“Spin wave (phonon) above critical field
Phase diagram in a magnetic field
H
1/
Spin singlet state with a spin gap
Canted magnetic order
gBH =
H
1/
Spin singlet state with a spin gap
Canted magnetic order
1 Tesla = 0.116 meV
Related theory applies to double layer quantum Hall systems at =2
gBH =
2
Elastic scattering
intensity
0
I H
HI a
J
~c cH
Phase diagram in a magnetic field
TlCuCl3
M. Matsumoto, B. Normand, T.M. Rice,
and M. Sigrist, cond-mat/0309440.
Canted magnetic order
Spin gap paramagnet
Phase diagram in a strong magnetic field.
Magnetization =density of triplons
H
Spin gap
Canted magnetic order
At very large H, magnetization
saturates
1
Phase diagram in a strong magnetic field.
Magnetization =density of triplons
H
Spin gap
Canted magnetic order
M
1
1/2
Respulsive interactions between triplons can lead to
magnetization plateau at any rational fraction
ij zi zji j
J S S
Magnetization =density of triplons
H
Phase diagram in a strong magnetic field.
Spin gap
Canted magnetic order
M
1
1/2
Quantum transitions in and out of plateau are
Bose-Einstein condensations of “extra/missing”
triplons
Magnetization =density of triplons
H
Partial magnetization plateau observed in SrCu2(BO3)2 and NH4CuCl3
Phase diagram in a strong magnetic field.
Spin gap
Canted magnetic order
ky
•
kx
/a
/a0
Insulator
~0.12-0.140.055SC
0.020
J. M. Tranquada et al., Phys. Rev. B 54, 7489 (1996). G. Aeppli, T.E. Mason, S.M. Hayden, H.A. Mook, J. Kulda, Science 278, 1432
(1997). S. Wakimoto, G. Shirane et al., Phys. Rev. B 60, R769 (1999). Y.S. Lee, R. J. Birgeneau, M. A. Kastner et al., Phys. Rev. B 60, 3643 (1999)
S. Wakimoto, R.J. Birgeneau, Y.S. Lee, and G. Shirane, Phys. Rev. B 63, 172501 (2001).
(additional commensurability effects near =0.125)
T=0 phases of LSCO
Interplay of SDW and SC order in the cuprates
SC+SDWSDWNéel
• •• •
ky
kx
/a
/a0
Insulator
~0.12-0.140.055SC
0.020
J. M. Tranquada et al., Phys. Rev. B 54, 7489 (1996). G. Aeppli, T.E. Mason, S.M. Hayden, H.A. Mook, J. Kulda, Science 278, 1432
(1997). S. Wakimoto, G. Shirane et al., Phys. Rev. B 60, R769 (1999). Y.S. Lee, R. J. Birgeneau, M. A. Kastner et al., Phys. Rev. B 60, 3643 (1999)
S. Wakimoto, R.J. Birgeneau, Y.S. Lee, and G. Shirane, Phys. Rev. B 63, 172501 (2001).
(additional commensurability effects near =0.125)
T=0 phases of LSCO
SC+SDWSDWNéel
Interplay of SDW and SC order in the cuprates
••
•Superconductor with Tc,min =10 K•
ky
kx
/a
/a0
~0.12-0.140.055SC
0.020
J. M. Tranquada et al., Phys. Rev. B 54, 7489 (1996). G. Aeppli, T.E. Mason, S.M. Hayden, H.A. Mook, J. Kulda, Science 278, 1432
(1997). S. Wakimoto, G. Shirane et al., Phys. Rev. B 60, R769 (1999). Y.S. Lee, R. J. Birgeneau, M. A. Kastner et al., Phys. Rev. B 60, 3643 (1999)
S. Wakimoto, R.J. Birgeneau, Y.S. Lee, and G. Shirane, Phys. Rev. B 63, 172501 (2001).
(additional commensurability effects near =0.125)
T=0 phases of LSCO
SC+SDWSDWNéel
Interplay of SDW and SC order in the cuprates
Collinear magnetic (spin density wave) order
.Re ; order parameter is complex vector ji K rj e
����������������������������
S
, 0K ��������������
;
3 4, 0K ��������������
;
3 4, / 8K ��������������
;
Collinear spins ie n
••
•Superconductor with Tc,min =10 K•
ky
kx
/a
/a0
~0.12-0.140.055SC
0.020
T=0 phases of LSCO
SC+SDWSDWNéel
Use simplest assumption of a direct second-order quantum phase transition between SC and SC+SDW phases
Interplay of SDW and SC order in the cuprates
If does not exactly connect two nodal points,
critical theory is as in an insulator
K
Otherwise, new theory of coupled excitons and nodal quasiparticles
L. Balents, M.P.A. Fisher, C. Nayak, Int. J. Mod. Phys. B 12, 1033 (1998).
Magnetic transition in a d-wave superconductor
Coupling to the S=1/2 Bogoliubov quasiparticles of the d-wave superconductor
Trilinear “Yukawa” coupling
is prohibited unless ordering wavevector is fine-tuned.
2d rd
22 † is allowed
Scaling dimension of (1/ - 2) 0 irrelev t.an
d rd
2 22 2rd rd c V S
Similar terms present in action for SDW ordering in the insulator
Magnetic transition in a d-wave superconductor
••
•Superconductor with Tc,min =10 K•
ky
kx
/a
/a0
~0.12-0.140.055SC
0.020
T=0 phases of LSCO
SC+SDWSDWNéel
H
Follow intensity of elastic Bragg spots in a magnetic field
Use simplest assumption of a direct second-order quantum phase transition between SC and SC+SDW phases
Interplay of SDW and SC order in the cuprates
Recall, in an insulator intensity would increase ~ H2
Dominant effect of magnetic field: Abrikosov flux lattice
2 2
2
Spatially averaged superflow kinetic energy
3 ln c
sc
HHv
H H
1sv
r
r
1/ 2 22 2 2 22 2 21 2
0 2 2
T
b r
g gd r d c s S
2 22
2c d rd Sv
4
222
2GL rF d r iA
,
ln 0
GL b cFZ r D r e
Z r
r
S S
(extreme Type II superconductivity)Effect of magnetic field on SDW+SC to SC transition
Quantum theory for dynamic and critical spin fluctuations
Static Ginzburg-Landau theory for non-critical superconductivity
Triplon wavefunction in bare potential V0(x)
Energy
x0
Spin gap
Vortex cores
2
0
Bare triplon potential
V s r rv
D. P. Arovas, A. J. Berlinsky, C. Kallin, and S.-C. Zhang, Phys. Rev. Lett. 79, 2871 (1997) suggested nucleation of static magnetism (with =0) within vortex scores in a first-order transition. However,
given the small size of the vortex cores, the magnetism must become dynamic as in a spin gap state.
S. Sachdev, Phys. Rev. B 45, 389 (1992); N. Nagaosa and P. A. Lee, Phys. Rev. B 45, 966 (1992)
2
0
Wavefunction of lowest energy triplon
after including triplon interactions: V V g
r r r
E. Demler, S. Sachdev, and Y
. Zhang, . , 067202 (2001).
A.J. Bray and
repulsive interactions between excitons imply that triplons must be extended as 0.
Phys. Rev. Lett
Strongly relevant
87
M.A. Moore, . C , L7 65 (1982).
J.A. Hertz, A. Fleishman, and P.W. Anderson, . , 942 (1979).
J. Phys
Phys. Rev. Lett
15
43
Energy
x0
Spin gap
Vortex cores
2
0
Bare triplon potential
V s r rv
TlCuCl3
M. Matsumoto, B. Normand, T.M. Rice,
and M. Sigrist, cond-mat/0309440.
Canted magnetic order
Spin gap paramagnet
2 2
2
Spatially averaged superflow kinetic energy
3 ln c
sc
H Hv
H H
1sv
r
r
Phase diagram of SC and SDW order in a magnetic field
2eff
2
The suppression of SC order appears to the SDW order as a effective "doping" :
3 ln c
c
HHH C
H H
uniform
E. Demler, S. Sachdev, and Ying Zhang, Phys. Rev. Lett. 87, 067202 (2001).
E. Demler, S. Sachdev, and Ying Zhang, Phys. Rev. Lett. 87, 067202 (2001).
eff
( )~
ln 1/
c
c
c
H
H
Phase diagram of SC and SDW order in a magnetic field
eff
2
2
Elastic scattering intensity
, 0,
3 0, ln c
c
I H I
HHI a
H H
2- 4Neutron scattering of La Sr CuO at =0.1x x x
B. Lake, H. M. Rønnow, N. B. Christensen, G. Aeppli, K. Lefmann, D. F. McMorrow, P. Vorderwisch, P. Smeibidl, N. Mangkorntong, T. Sasagawa, M. Nohara, H. Takagi, T. E. Mason, Nature, 415, 299 (2002).
2
2
Solid line - fit ( ) nto : l c
c
HHI H a
H H
See also S. Katano, M. Sato, K. Yamada, T. Suzuki, and T. Fukase, Phys. Rev. B 62, R14677 (2000).
2
2
2
Solid line --- fit to :
is the only fitting parameter
Best fit value - = 2.4 with
3.01 l
= 6
n
0 T
0
c
c
c
I H HH
H
a
aI H
a H
Neutron scattering measurements of static spin correlations of the superconductor+spin-density-wave (SC+CM) in a magnetic field
H (Tesla)
2 4
B. Khaykovich, Y. S. Lee, S. Wakimoto,
K. J. Thomas, M. A. Kastner,
and R.J. Birge
Elastic neutron scatt
neau, B ,
014528 (2002)
ering off La C O
.
u y
Phys. Rev.
66
E. Demler, S. Sachdev, and Ying Zhang, Phys. Rev. Lett. 87, 067202 (2001).
Neutron scattering observation of SDW order enhanced by
superflow.
eff
( )~
ln 1/
c
c
c
H
H
Phase diagram of a superconductor in a magnetic field
2
2
1 triplon energy
30 ln c
c
S
HHH b
H H
Neutron scattering measurements of dynamic spin correlations of the superconductor (SC) in a magnetic field
B. Lake, G. Aeppli, K. N. Clausen, D. F. McMorrow, K. Lefmann, N. E. Hussey, N. Mangkorntong, M. Nohara, H. Takagi, T. E. Mason,
and A. Schröder, Science 291, 1759 (2001).
2- 4Neutron scattering off La Sr CuO ( 0.163, ) SC phase
Peaks at (0.5,0.5) (0.125,0)
and (0.5,0.5) (0,0.125)
dynamic SDW of period 8
red dat lo otsw temperatures in =0 ( ) and =7.5T blue d )s( otH H
Neutron scattering measurements of dynamic spin correlations of the superconductor (SC) in a magnetic field
B. Lake, G. Aeppli, K. N. Clausen, D. F. McMorrow, K. Lefmann, N. E. Hussey, N. Mangkorntong, M. Nohara, H. Takagi, T. E. Mason,
and A. Schröder, Science 291, 1759 (2001).
2- 4Neutron scattering off La Sr CuO ( 0.163, ) SC phase
Peaks at (0.5,0.5) (0.125,0)
and (0.5,0.5) (0,0.125)
dynamic SDW of period 8
red dat lo otsw temperatures in =0 ( ) and =7.5T blue d )s( otH H
Collinear magnetic (spin density wave) order
.Re ; order parameter is complex vector ji K rj e
����������������������������
S
3 4, 0K ��������������
;
3 4, / 8K ��������������
;
Collinear spins , and there is modulation
in the parameter at
wavevector 2
x
i
j j j a
e
Qbond order r
K
��������������
n
S S
E. Demler, S. Sachdev, and Ying Zhang, Phys. Rev. Lett. 87, 067202 (2001).
Neutron scattering observation of SDW order enhanced by
superflow.
eff
( )~
ln 1/
c
c
c
H
H
Phase diagram of a superconductor in a magnetic field
Prediction: SDW fluctuations enhanced by superflow and bond order pinned by vortex cores (no
spins in vortices). Should be observable in STM
K. Park and S. Sachdev Physical Review B 64, 184510 (2001); Y. Zhang, E. Demler and S. Sachdev, Physical Review B 66, 094501 (2002).
2
2
1 triplon energy
30 ln c
c
S
HHH b
H H
STM around vortices induced by a magnetic field in the superconducting state
J. E. Hoffman, E. W. Hudson, K. M. Lang, V. Madhavan, S. H. Pan, H. Eisaki, S. Uchida, and J. C. Davis, Science 295, 466 (2002).
-120 -80 -40 0 40 80 1200.0
0.5
1.0
1.5
2.0
2.5
3.0
Regular QPSR Vortex
Diffe
rential C
onducta
nce (
nS
)
Sample Bias (mV)
Local density of states
1Å spatial resolution image of integrated
LDOS of Bi2Sr2CaCu2O8+
( 1meV to 12 meV) at B=5 Tesla.
S.H. Pan et al. Phys. Rev. Lett. 85, 1536 (2000).
100Å
b7 pA
0 pA
Vortex-induced LDOS of Bi2Sr2CaCu2O8+ integrated from 1meV to 12meV
J. Hoffman E. W. Hudson, K. M. Lang, V. Madhavan, S. H. Pan, H. Eisaki, S. Uchida, and J. C. Davis, Science 295, 466 (2002).
Our interpretation: LDOS modulations are
signals of bond order of period 4 revealed in
vortex halo
See also: S. A. Kivelson, E. Fradkin, V. Oganesyan, I. P. Bindloss, J. M. Tranquada, A. Kapitulnik, and C. Howald, cond-
mat/0210683.
Conclusions
I. Introduction to magnetic quantum criticality in coupled dimer antiferromagnet.
II. Berry phases and bond order in square lattice antiferromagnets.
III. Theory of quantum phase transitions provides semi-quantitative predictions for neutron scattering measurements of spin-density-wave order in superconductors; theory also proposes a connection to STM experiments.
IV. Spontaneous bond order in spin gap state on the square lattice: possible connection to modulations observed in vortex halo.
Conclusions
I. Introduction to magnetic quantum criticality in coupled dimer antiferromagnet.
II. Berry phases and bond order in square lattice antiferromagnets.
III. Theory of quantum phase transitions provides semi-quantitative predictions for neutron scattering measurements of spin-density-wave order in superconductors; theory also proposes a connection to STM experiments.
IV. Spontaneous bond order in spin gap state on the square lattice: possible connection to modulations observed in vortex halo.