julien taieb - t-2 : lanlt2.lanl.gov › fiesta2014 › presentations › taieb.pdfjulien taieb for...
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![Page 1: Julien TAIEB - T-2 : LANLt2.lanl.gov › fiesta2014 › presentations › Taieb.pdfJulien TAIEB For the SOFIA Collaboration Fiesta workshop, Sept. 13th, 2014| PAGE 1. THE EXPERIMENTAL](https://reader033.vdocuments.us/reader033/viewer/2022060322/5f0d7ff17e708231d43aa9f1/html5/thumbnails/1.jpg)
Theoritician dreams /nightmares
come true
Julien TAIEB
For the SOFIA Collaboration
| PAGE 1Fiesta workshop, Sept. 13th, 2014
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THE EXPERIMENTAL TECHNIQUES
| PAGE 2
neutron• 1 or 2 FF detected
• Identified in A or Z
Pu, U, Th ...
Major difficulties
• (Thin) )Target usually radioactive
• Low detection efficiency
• Mass number only measured in most experiments
• Atomic number very hard to get
Despite 75 years of effort, there is no way to identify all FF
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THE FF MASS YIELDS MAJOR ACTINIDES
| PAGE 3
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THE NUCLEAR CHARGE MEASUREMENT ISSUE
| PAGE 4
Measurement of the nuclear charge of FF
• Full ID needed for applications and for underatanding of the process
• Mass number doesn’t mean much
• How to measure the Z ?
• Specific methods
• Chemical separation + Gamma spectroscopy
• X-ray identification
• General method : energy loss (DE)
• DE Z2
• Does work for the light FF
• No separation for the heavy FF
• Very low recoil velocity
• Strong fluctuation in mean charge state
• Only light fission fragments can be identified in Z and A
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THE FF MASS YIELDS MAJOR ACTINIDES
| PAGE 5Mass number A
Fis
sio
n y
ield
s (
%)
233U235U239Pu
Heavy peak seems to stay
Light peak seems to adjust
We would like to have a
deeper look at the heavy peak
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NEW EXPERIMENTAL APPROACH (K.H. SCHMIDT 96)
| PAGE 6
neutron
U, Th ...
direct kinematics
• Study the fission of
radioactive nuclides
• Two FF emitted in forward
direction : ∈𝑔𝑒𝑜𝑚
• Centre of mass boost:
easier identification of FF
• Nuclear charge measured
Actinide:
U, Th
Reverse kinematics
Stable target
![Page 7: Julien TAIEB - T-2 : LANLt2.lanl.gov › fiesta2014 › presentations › Taieb.pdfJulien TAIEB For the SOFIA Collaboration Fiesta workshop, Sept. 13th, 2014| PAGE 1. THE EXPERIMENTAL](https://reader033.vdocuments.us/reader033/viewer/2022060322/5f0d7ff17e708231d43aa9f1/html5/thumbnails/7.jpg)
FISSION IN REVERSE KINEMATICS AT GSI
| PAGE 7
Relativistic actinide U, Th ..
heavy target: Pb
E* distribution
The Giant Dipole
Resonances (GDR) are
populated
Fission induced by Coulomb excitation
Pb Pb11 MeV ± 3 MeV
<E*> =12.5, similar to 7 MeV neutron induced fission
fission
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THE SOFIA EFFORT
| PAGE 8
• Provide new data usable for :
• Current nuclear reactors operation
• Next generation nuclear reactor design
• simulation of accidental configurations
• Improve the understanding of the process
• Contribute to the qualification of theoretical codes
• Improve the r-process modelling
• Follow K.-H. Schmidt pioneering idea
• Improve precision
• Measure the mass number
• Get the number of emitted neutrons
• Get unprecedented mass and charge resolutions
• Study the fission of many actinides and preactinides
• 8 european labs involved
• 5 years of technical developments
• 5 million euros invested
• 1st experiment in august 2012
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| PAGE 9
GSI (DARMSTADT)
238U
1 A.GeV
C : SOFIA
Fission in reverse
kinematics, 650 A.MeV
Actinide secondary beams from fragmentation reactions of 238U
Injection fromUNILAC
R3B cave
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1ST SOFIA EXPERIMENT, 08/2012
| PAGE 10
For both fragments, we measure
Z and A
Z
N
Target : resolution < 1 (FWHM) over the full FF range
In addition:
• Number of emitted neutrons 𝝊 = Afiss– (A1 +A2)
• TKE
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| PAGE 11
The SOFIA set up
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THE SOFIA SET UP
all detectors developed for that experiment
Challenge : mass identification in the FF region
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| PAGE 15
Spectra
1) Chart of nuclide
2) Nuclear Charges
3) Masses
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CHART OF MEASURED FF
| PAGE 16𝑷𝒉𝑫 𝒕𝒉𝒆𝒔𝒊𝒔 ∶ 𝑱𝒖𝒍𝒊𝒆 𝑴𝒂𝒓𝒕𝒊𝒏
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NUCLEAR CHARGE SPECTRUM.
| PAGE 17
Num
ber
of counts
Rather good charge resolution
Visible odd-even staggering
ΔZ = 0,4 (FWHM)
𝑷𝒉𝑫 𝒕𝒉𝒆𝒔𝒊𝒔 ∶ 𝑱𝒖𝒍𝒊𝒆 𝑴𝒂𝒓𝒕𝒊𝒏
2𝟑𝟓𝑼 𝒄𝒐𝒖𝒍𝒆𝒙 𝒇𝒊𝒔𝒔𝒊𝒐𝒏
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MASS NUMBER SPECTRUM
| PAGE 18
A = 140 :
ΔA = 0,8 (FWHM)
A = 90 :
ΔA = 0,58 (FWHM)
Very good mass resolution for the light FF
Degrades for the heavy FF, still neighbouring
isotopes disantangled
Num
ber
of counts
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| PAGE 19
Fission yields
1) Element
2) Isotonic
3) Isotopic
4) Mass
5) Prompt Neutrons 𝜈
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238U, CHARGE YIELDS
| PAGE 20
𝜎𝑠𝑡𝑎𝑡 ≈ 2%
𝜎𝑠𝑡𝑎𝑡 ≈ 0.3 %𝝈𝒔𝒚𝒔𝒕 ≈ 𝟐%
𝑷𝒉𝑫 𝒕𝒉𝒆𝒔𝒊𝒔 ∶ 𝑬𝒓𝒊𝒄 𝑷𝒆𝒍𝒍𝒆𝒓𝒆𝒂𝒖
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235U, CHARGE YIELDS
| PAGE 21𝑷𝒉𝑫 𝒕𝒉𝒆𝒔𝒊𝒔 ∶ 𝑱𝒖𝒍𝒊𝒆 𝑴𝒂𝒓𝒕𝒊𝒏
𝜎𝑠𝑡𝑎𝑡 ≈ 0.5 %
𝜎𝑠𝑡𝑎𝑡 ≈ 4%
𝝈𝒔𝒚𝒔𝒕 ≈ 𝟏%
Most produced element moves from 52 to 54
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THE THORIUM CHAIN, K.-H. SCHMIDT ET AL VS SOFIA
| PAGE 22
𝑪𝒐𝒖𝒓𝒕𝒆𝒔𝒚 ∶ 𝑨𝒖𝒅𝒓𝒆𝒚 𝑪𝒉𝒂𝒕𝒊𝒍𝒍𝒐𝒏
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| PAGE 23
Fission yields
1) Element
2) Isotonic
3) Isotopic
4) Mass
5) Prompt Neutrons 𝜈
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ISOTONIC YIELDS: N = A – Z, FISSION OF 238U
| PAGE 24
N = 82
Odd-even staggering for the light and heavy FF
Proeminent peak at N=82
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ISOTONIC YIELDS: N = A – Z, FISSION OF 235U
| PAGE 25
N = 82
Odd-even staggering for the light and heavy FF
Proeminent peak at N=82
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| PAGE 26
Fission yields
1) Element
2) Isotonic
3) Isotopic
4) Mass
5) Prompt Neutrons 𝜈
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ISOTOPIC YIELDS (HEAVY FF)
| PAGE 27
Y (
%)
A
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ISOTOPIC YIELDS ; ZOOM Z = 49-50
| PAGE 28
Y (
N)
%Y
(N
) %
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FISSION MODES
Several paths toward the scission
50132𝑆𝑛
TKE (total kinetic energy)
Edef
Standard 1
Standard 2
PES
Super-Long
𝑪𝒐𝒖𝒓𝒕𝒆𝒔𝒚:𝑵𝒐𝒆𝒍 𝑫𝒖𝒃𝒓𝒂𝒚
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ISOTOPIC YIELDS; Z = 49-50
| PAGE 30
SL
SI
Y (
N)
%Y
(N
) %
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| PAGE 31
SL
Y (
N)
%
SL
scission
time
Edéformation decrease
E* increase
ISOTOPIC YIELDS; Z = 49-50
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| PAGE 32
Fission yields
1) Element
2) Isotonic
3) Isotopic
4) Mass
5) Prompt Neutrons 𝜈
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MASS YIELDS, COMPARISON TO THE EVALUATION
| PAGE 33
U 238 : E * = 13 MeV
U 239 : E * = 20 MeV
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| PAGE 34
Fission yields
1) Element
2) Isotonic
3) Isotopic
4) Mass
5) Prompt Neutrons 𝜈
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𝝊 VS Z , FISSION OF 235U
| PAGE 35
𝝊 = 235 – (A1 + A2)SL Mode : E* increases :
higher deformation
energy
SL 𝝊 = 3.7
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𝝊 VS A FOR Z = 49, , FISSION OF 235U
| PAGE 36A, Mass number
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𝝊 VS A FOR Z = 50, , FISSION OF 235U
| PAGE 37A, Mass number
𝟏𝟑𝟐𝑺𝒏
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| PAGE 38
Fission yields
1) Element
2) Isotonic
3) Isotopic
4) Mass
5) Prompt Neutrons 𝜈6) TKE
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TKE VS Z , FISSION OF 235U
| PAGE 39
Harder to extract that in
neutron induced fission
=> Hier uncertainty
𝑶𝒅𝒅 − 𝒆𝒗𝒆𝒏 𝒔𝒕𝒂𝒈𝒈𝒆𝒓𝒊𝒏𝒈 in TKE(Z) !
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TKE VS A FOR Z = 49, , FISSION OF 235U
| PAGE 40N, Neutron number
Uncertainty not evaluated yet
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TKE VS A FOR Z = 50, FISSION OF 235U
| PAGE 41A, Mass number
𝟏𝟑𝟐𝑺𝒏
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CONCLUSIONS
| PAGE 42
Nuclear charge resolution = 0,4 u FWHM
Mass resolution = 0,8 u FWHM for A = 140
Typical uncertainty on isotopic yields < 5 %
Big step forward w/ respect to previous knowledge
SOFIA1 provides new results :
Detailed information on fission modes
New data on the scission configurations
Total kinetic energy
Number of emitted neutrons
Fission of tens of nuclide studied in one experiment
All fission fragments identified unambiguously for the 1st time in low
energy fission
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| PAGE 43
𝑻𝒉𝒆 𝑺𝑶𝑭𝑰𝑨 𝒄𝒐𝒍𝒍𝒂𝒃𝒐𝒓𝒂𝒕𝒊𝒐𝒏
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PERSPECTIVES
| PAGE 44
L’238U : 1 noyau sur les 80 mesurés Intérêt aussi dans
les systématiques
SOFIA 2 en 2014
Futur 2 : FELISE @ FAIR Fission at ELISE : excitation électromagnétique par des
e- : E* mesurée
Futur 1 : R3B Aimant GLAD : 4,8 T.m. (ALADIN 2,2 T.m.)
CALIFA : Mesure des gammas
NEULAND : Mesure des neutrons (par fragment ?)
Répartition de l’énergie dans la fission
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SOUSTRACTION DE LA COMPOSANTE RÉSIDUELLE
| PAGE 45
La Sélection Z1+Z2 = 92 : n’élimine que les fissions de haute énergie
ou des PROTONS sont enlevés
Suppression de la composante ou seuls des NEUTRONS sont enlevés ?
Utilisation des fissions dans les matériaux légers (pas de fission e.m.)
K = facteur pour égaliser les
sections efficaces de fission
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SOUSTRACTION DE LA COMPOSANTE RÉSIDUELLE
| PAGE 46
La Sélection Z1+Z2 = 92 : n’élimine que les fissions de haute énergie
où des PROTONS sont enlevés
Suppression de la composante où seuls des NEUTRONS sont enlevés ?
Utilisation des fissions dans les matériaux légers (fissions nucléaires uniquement)
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MASSES - PIC/VALLÉE VS E*
| PAGE 47
E* ≈ 15 MeV
Consistant avec la valeur de 14 MeV attendue (calculs)
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FISSION E.M ET GDR
| PAGE 48
n
A (Ji,πi) A+1 (Jf,πf)
Jf =Ji +0.5 si neutron thermique
=Jf =Ji +0.5 + L , avec L = f(E neutron)
πf = πi si neutron thermique
= πi x(-1)L
A+1 (Ji,πi) A+1 (Jf,πf)
=GDR :
T = 1, L = 1, S = 0 Jf =Ji +1
πf = -πi
+
Fission induite par neutron
Fission induite par e.m.
Exemple : fission de l’U8 sur SOFIA :
U8 : GS = 0+ ; apres e.m. GDR : U8 : 1-
U7 : GS = 1/2+
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POLARISATION EN CHARGE
| PAGE 49
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SPECTRE D’EXCITATION À LA FISSION
| PAGE 50
E* ≈ 15 MeV
14 MeV en moyenne attendus
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| PAGE 51
Flux photons eq. Flux photons eq. x (GDR , GQR)
Probabilité fission.
E* a la fission
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12-Sep-14 52
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CHARGE POLARIZATION
| PAGE 53
UCD
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ACTIVE TARGET
| PAGE 54
e-e-
e-
e-
e-
1 cathode (Heavy Z)
+ 300 V
2 cm
U 238
FF 1
FF 2
Coulomb excitation
(photon exchange)
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MWPC : RÉSOLUTION EN POSITION
| PAGE 55
180 µm
FWHM
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RENDEMENTS ISOTOPIQUES ; ÉVOLUTION
| PAGE 56
Ecart valeurs moyennes consécutives
Largeur
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MUSIC : ANGLE RESOLUTION
| PAGE 57
CEA | 10 AVRIL 2012
≈ 60 µm FWHM
< 0,2 mrad FWHM Drift Time
ZAnode i-1 Anode i Anode i+1
Deviation to fit
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FISSION EN CINÉMATIQUE INVERSE RELATIVISTE
| PAGE 58
Noyau lourd fissionnant
relativiste
Pb
Excitation électromagnétiqueE* ≈11 MeV
• Etude de noyaux radioactifs
• Q = Z
• ∈𝑔𝑒𝑜𝑚 importante
Fission de l'238U en cinématique inverse n (≈6 MeV) + 237U
Peuplement
GDRPb Pb
fission
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| PAGE 59
The detectors
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CIBLE ACTIVE : FISSION DANS LES MATÉRIAUX
LOURDS
| PAGE 60
Fission in the cathodes
Anodes : provide ΔE
beam
FF1
FF2
Stack of ionisation chambers
AnodeCathode
(fission)
Anode
∆𝐸 𝐹𝐹1 + ∆𝐸 𝐹𝐹2 ≈∆𝐸 238𝑈
2
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MWPCs
| PAGE 61
Anodes +1200V
1) Création d’e-
d’ionisation
2) Avalanche d’e- autour
des fils d’anodes
3) Influence sur les pistes
de cathode
200 𝜇𝑚 requis en X
135 𝜇𝑚 mesures FWHM
Cathodes
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DISPOSITIF TEMPS DE VOL
| PAGE 62
Stop : contrainte de taille :
Dimensions : 90 * 60 cm2 (dispersion du dipôle)
Stop60 cm
90 cm
28 scintillateurs 56 PMTs
Haute énergie et base de vol courte (7.5 m) :
Nécessaire pour séparer A lourds : 40 ps FWHMAu GSI : 100 ps FWHM au mieux
A. Ebran et al.,
NIM A 728
(2013) 40-46
Bruyères-Le-Châtel
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Z2 VS Z1
| PAGE 63
Z1 + Z2 < 92
Fragmentation-Fission
Z2
Z1
Z1 + Z2 = ZCN =92
e.m induced fission
Z1 + Z2 = cste
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TWIN MUSIC : MULTI-SAMPLE IONISATION CHAMBER
| PAGE 64
e-e-e-
e-e-
e-
e-
e-
ΔE3 ΔE6 ΔE8
ΔEi : energy losses Z
ΔTi : drift time q
10 anodes
10 anodes
Upper view
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MUSIC : ANGLE RESOLUTION
| PAGE 65
CEA | 10 AVRIL 2012
≈ 65 µm FWHM
< 0,4 mrad FWHM
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TOF RESOLUTION
| PAGE 66
35 ps
FWHM
relativistic 124Sn
(heavy FF)
Num
ber
of counts