in situ measurements of aerosol size distributions inside the … · 2016-03-29 · in situ...
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In situ measurements of aerosol size
distributions inside the Asian Summer
Monsoon Anticyclone
Ru-Shan Gao, Hagen Telg, Pengfei Yu, and Karen Rosenlof
NOAA Earth System Research Laboratory
Jianchun Bian, Zhixuan Bai, Dan Li, Yunjun Duan
Lageo, Institute of Atmospheric Physics, Chinese Academy of
Sciences
March 9, 2016
Asian Monsoon Workshop NCAR
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POPS description:
Size range: 140 – 3000 nm diameter (dry)
Sampling: 3 cm3 s-1
Weight: 1 kg
Communication:
8 size bins with O3,
CFH, COBALD (limited
by the iMet bandwidth)
POPS
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The Institute for Atmospheric Physics/Chinese Academy of Science Long Trek VII
UAS
- POPS integration and test flights in November 2015
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UAS implementation
The NOAA Pacific Marine Environment Laboratory (PMEL) Manta UAS
- POPS and ULR have been fully integrated
- Successful test flights in January 2015
- First field mission in April 2015 – Svalbard, Norway in collaboration with
PMEL
The University of Colorado Pilatus UAS
- POPS integration in February 2015
- Test flight in March 2015
- First field mission in April 2015 – Oliktok Point, AK in collaboration with Dept.
of Energy, University of Colorado, and Physical Sciences Division (PSD)
The Laboratory for Atmosphere and Cyclone (LACy, Reunion, France) R2 Drone
- POPS integration right now
- Test flight in this month
- First field mission in Indian Ocean
in collaboration with LACy
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POPS (optical particle counter) and miniSASP (sun photometer):
Aerosol optical density and hygroscopicity
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miniSASP (sun photometer
POPS (optical particle counter)
ECC ozone sensor
Total weight = 5.6 lbs.
2.1 m
Instrumented auto-homing glider (Skywalker X8)
Flight control by Black Swift Technologies
Autopilot Tablet UI Ground station
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COBALD
O3
CFH
POPS (Printed
Optical
Particle
Spectrometer)
iMet
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Aug 13, 2015: NCEP 100 mb hgt
Balloon measurements Balloon measurements
Kunming, China
Asian summer monsoon anticyclone
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Aug 14, 2015: NCEP 100 mb hgt
Balloon measurements
Kunming, China
Asian summer monsoon anticyclone
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Aug 17, 2015: NCEP 100 mb hgt
Asian summer monsoon anticyclone
Balloon measurements Balloon measurements
Kunming, China
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Ascent data, 200-m average
8006004002000
Aerosol concentration (# cm-3
)
Flt 3, 2015 08 17
12008004000
Aerosol concentration (# cm-3
)
Flt 2, 2015 08 14 Total 98 - 144 nm 144 - 179 nm 179 - 231 nm 231 - 360 nm CPT
30
25
20
15
10
5
Altitu
de
(km
)
10008006004002000
Aerosol concentration (# cm-3
)
Flt 1, 2015 08 13
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20
18
16
14
12
10
Altitud
e (
km
)
403020100 403020100
Particle concentration (# cm-3
)
403020100
252015105 252015105
455 nm backscatter ratio
252015105
Kunming PC CPT Houston PC Backscatter
13 August 2015 14 August 2015 17 August 2015
Ascent data, 200-m average
ATAL is a great UT air tracer in the LS
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Size distribution 2015 08 13
10-4
10-3
10-2
10-1
dN
/dlo
g(D
p)
1002 3 4 5 6 7 8 9
10002
Dp (nm)
15 - 17 km 17 - 19 km
Particles were likely formed in the UT
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Flt 2, 2015 08 14
T, O3, and WV
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20
19
18
17
16
15
Altitu
de
(km
)
161412108642
Aerosol concentration (# cm-3
)
01 August 1996 08 August 1996 Cold point
STRAT data
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20
19
18
17
16
15
Altitu
de
(km
)
14121086420
Aerosol concentration (# cm-3
)
03 August 2007 05 August 2007 06 August 2007 08 August 2007 09 August 2007 Cold point
TC4 data
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• In a general sense the ATAL is NOT unique!
- Brock et al., Science (1995)
• The air in the ASMA, similar to the air in the tropics,
is trapped and moving upward slowly.
• Condensables have sufficient time to form new
particles or condense on existing particles.
• Tropical aerosol layer too thin to be detected by
satellites?
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35
30
25
20
15
10
5
0
Altitud
e (
km
)
1086420
O3 (ppm)
Hilo Tsukuba Kunming
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36
34
32
30
28
26
24
Altitud
e (
km
)
1086
O3 (ppm)
Hilo Tsukuba Kunming
O3 is significantly higher above ~26 km
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19
18
17
16
Altitud
e (
km
)
0.80.60.40.20.0
O3 (ppm)
Hilo Tsukuba Kunming
O3 is significantly lower ~16-18 km
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Ascent
Mixing
Tropopause
Strat
air
Tropo
air
A crude mixing model:
• Ascent rate determined
by the local heating rate
and local thermal structure
• Particles = Trop. tracer
• O3 = Strat. tracer
• Mixing in strat can be
derived from these three.
(Arguably ascent is easier
to calculate than mixing) O3 poor, particle rich
O3 rich, particle poor
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Conclusions
1) ATAL appears to be robust feature
2) The particle enhancement has implications (additional
heating)
3) In the ASMA LS these particles are a good tracer of the
tropospheric air
- Size distributions suggest formation/growth in UT
- Tropospheric air is moving up into stratosphere
4) ATAL is similar to the tropical aerosol layer
5) Measureable mixing tracers: O3 and aerosol
6) A crude model may be useful for LS mixing rate
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