impurity and vortex-core states in superconducting spin ...nqs2017.ws/slides/sympo/9th/...ruo 4 •...
TRANSCRIPT
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Impurity and vortex-core states in superconducting spin-
helical Dirac fermions
Hiroki IsobeMassachusetts Institute of Technology
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Acknowledgment
Liang Fu Michał Papaj
HI, M. Papaj, and L. Fu (to appear)
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Outline
2D topological surface states in proximity to s-wave superconductivity will host Majorana zero modes.
• We look into impurity bound states and vortex core states in detail.
• Is there a way to distinguish Majorana zero modes from another zero energy localized modes?
Results: • Impurity bound states can also be zero-energy localized
modes. • However, they are different in: spatial distribution, spin
configuration…
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Search for Majorana zero modes
• Majorana condition 𝛾𝛾0 = 𝛾𝛾0†
• Localized at an ℎ𝑐𝑐/2𝑒𝑒 vortex in a 𝑝𝑝 + 𝑖𝑖𝑝𝑝 superconductor • It necessarily lies at zero energy in superconductors.
• Non-Abelian statistics and application to quantum computation
M. Sato and Y. Ando, Reports Prog. Phys. 80, 076501 (2017).
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Search for Majorana zero modes
However, a Majorana zero mode is not the only one localized midgap modes in superconductors.
Midgap states includes:• Vortex-core states (Caroli-de Gennes-Matricon, 1964)
• Include Majorana zero modes
• Impurity bound states (Yu, 1965; Shiba, 1968; Rusinov, 1969)
• Kondo impurity resonance, etc.
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Midgap states in superconductors
For conventional s-wave superconductors:
• Impurity bound states – Yu-Shiba-Rusinov states
• Vortex-core states – Caroli-de Gennes-Matricon statesA. V. Balatsky, I. Vekhter, and J.-X. Zhu, Rev. Mod. Phys. 78, 373 (2006).
C. Caroli, P. G. De Gennes, and J. Matricon, Phys. Lett. 9, 307 (1964).
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Realization of topological superconductivity
Majorana zero modes in 2D superconductors:• Intrinsic (p+ip)-superconductor
Sr2RuO4
• 3D Topological insulator surface states + s-wave SC• Proximity effect• Intrinsic realizationCuxBi2Se3, Sn1-xInxTe, FeTe1-xSex
• 2D electron gas with Rashba + s-wave SC + Zeeman
See reviews, e.g., Alicea (2012), Sato and Ando (2017)
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Superconductivity proximity effect
2D superconductor on top of 3D topological insulator
L. Fu and C. L. Kane, Phys. Rev. Lett. 100, 096407 (2008).
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FeSe1-xTex: Normal state
DFT calculations• Band inversion along Γ − 𝑍𝑍 line• Topological “metal”• Single Dirac cone on 001 surface
Z. Wang, P. Zhang, G. Xu, L. K. Zeng, H. Miao, X. Xu, T. Qian, H. Weng, P. Richard, A. V. Fedorov, H. Ding, X. Dai, and Z. Fang, Phys. Rev. B 92, 115119 (2015).
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FeSe1-xTex: Superconducting state
DFT calculations• Energy spectrum along a vortex line (like a Majorana chain)• Self-doping by excess Fe atoms Fe1+ySe0.5Te0.5 (TSC: 0.03<y<0.06)
G. Xu, B. Lian, P. Tang, X.-L. Qi, and S.-C. Zhang, Phys. Rev. Lett. 117, 047001 (2016).
Topological
Γ
Z
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FeSe1-xTex: ARPES
FeTe0.55Se0.45 (Tc=14.5K)• Spin-helical surface Dirac cone
P. Zhang, K. Yaji, T. Hashimoto, Y. Ota, T. Kondo, K. Okazaki, Z. Wang, J. Wen, G. D. Gu, H. Ding, and S. Shin, arXiv:1706.05163.
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FeSe1-xTex: ARPES
FeTe0.55Se0.45 (Tc=14.5K)• s-wave superconducting gap on the surface
P. Zhang, K. Yaji, T. Hashimoto, Y. Ota, T. Kondo, K. Okazaki, Z. Wang, J. Wen, G. D. Gu, H. Ding, and S. Shin, arXiv:1706.05163.
2.4K
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FeSe1-xTex: STM/S (impurity)
Pristine Fe(Te,Se) (Tc=14.5K)At an interstitial iron impurity (excess iron atom)
Highest Tc without IFIs
J.-X. Yin et al., Nat. Phys. 11, 543 (2015).
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FeSe1-xTex: STM/S (impurity)
J.-X. Yin, Z. Wu, J.-H. Wang, Z.-Y. Ye, J. Gong, X.-Y. Hou, L. Shan, A. Li, X.-J. Liang, X.-X. Wu, J. Li, C.-S. Ting, Z.-Q. Wang, J.-P. Hu, P.-H. Hor, H. Ding, and S. H. Pan, Nat. Phys. 11, 543 (2015).
Possibilities for midgap states:• Majorana zero modes• Impurity bound states (magnetic or
non-magnetic)• Pair of spectral peaks, symmetric around
zero energy• Zeeman split under magnetic field
• Kondo resonance• Not at zero energy• Zeeman split
• d-wave pairing state with an impurity at unitary limit
• Four-fold pattern in real space
along c-axis
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FeSe1-xTex: STM/S (vortex)
FeTe0.55Se0.45 (T=0.55K, Tc=14.5K)• Vortex lattice under magnetic field along the c-axis (4T)
D. Wang et al., arXiv:1706.06074.
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Model
• Spin-helical Dirac fermion + s-wave superconductivity (2D)
• Coherence length
• Symmetry• Time reversal• Particle-hole
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Vortex core states
Apply magnetic fieldQuantized vortex (𝑙𝑙: vorticity)
• Around the vortex core, the wave function acquires the phase. (𝜈𝜈: angular momentum)
[ for a conventional s-wave superconductor]
Majorana zero mode (𝑙𝑙 = 1, 𝜈𝜈 = 0)
References:I. M. Khaymovich, N. B. Kopnin, A. S. Mel’nikov, and I. A. Shereshevskii, Phys. Rev. B 79, 224506 (2009).D. L. Bergman and K. Le Hur, Phys. Rev. B 79, 184520 (2009).M. Cheng, R. M. Lutchyn, V. Galitski, and S. Das Sarma, Phys. Rev. B 82, 094504 (2010)
mod 2𝜋𝜋
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Vortex core states
Apply magnetic fieldQuantized vortex (𝑙𝑙: vorticity)
• Around the vortex core, the wave function acquires the phase. (𝜈𝜈: angular momentum)
[ for a conventional s-wave superconductor]
Majorana zero mode (𝑙𝑙 = 1, 𝜈𝜈 = 0)
References:I. M. Khaymovich, N. B. Kopnin, A. S. Mel’nikov, and I. A. Shereshevskii, Phys. Rev. B 79, 224506 (2009).D. L. Bergman and K. Le Hur, Phys. Rev. B 79, 184520 (2009).M. Cheng, R. M. Lutchyn, V. Galitski, and S. Das Sarma, Phys. Rev. B 82, 094504 (2010)
mod 2𝜋𝜋
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Vortex core states
Midgap states at a vortex:
Majorana zero mode
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Impurity bound state
Impurity potential• 𝑈𝑈: scalar potential• 𝑆𝑆: classical spin
Bound state energy: pole of T-matrix
Equivalently, from the Bogoliubov-de Gennes equation
Is there a zero energy state?
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Magnetic impurity
Impurity potential• 𝑈𝑈 = 0, 𝐽𝐽𝑆𝑆 ≠ 0
Energy spectrum of midgap states• Pairs of states at any 𝐽𝐽𝑆𝑆• Accidental crossing at a certain 𝐽𝐽𝑆𝑆
Energy spectrum at large 𝜇𝜇
• Same form as one for conventional s-wave superconductors
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Magnetic + scalar impurity
Impurity potentialAssume only the spin-up level is on resonance: 𝑈𝑈 = 𝐽𝐽𝑆𝑆(= 𝑔𝑔).• Zero energy states exist in the strong coupling limit.
(There also exist pair states with negative energy.)
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Magnetic + scalar impurity
Impurity potentialAssume only the spin-up level is on resonance: 𝑈𝑈 = 𝐽𝐽𝑆𝑆(= 𝑔𝑔).• Zero energy states exist in the strong coupling limit.
Large 𝜇𝜇
(There also exist pair states with negative energy.)
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Magnetic + scalar impurity
Impurity potentialAssume only the spin-up level is on resonance: 𝑈𝑈 = 𝐽𝐽𝑆𝑆(= 𝑔𝑔).• Zero energy states exist in the strong coupling limit.
𝜇𝜇 = 0
(There also exist pair states with negative energy.)
• Momentum cutoff Λ(≫ Δ0/𝑣𝑣)• Valid for large 𝑔𝑔
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Magnetic + scalar impurity
Impurity potentialAssume only the spin-up level is on resonance: 𝑈𝑈 = 𝐽𝐽𝑆𝑆(= 𝑔𝑔).• Zero energy states exist in the strong coupling limit.
Intermediate 𝜇𝜇
(There also exist pair states with negative energy.)
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Difference from Majorana zero modes
Further differences will be found if we look at wave functions.
Impurity bound states Majorana zero modes
Localized at … Impurity Vortex (magnetic flux)
Locked at zero energy? No Yes
Appear in pairs? Yes No
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Wave function
Solve the Bogoliubov-de Gennes equation: Pientka et al. (2013)
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Wave function
: modified Bessel function
Only spin-up components
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Wave function
Only electron components
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Wave function
Two length scales:• Coherence length 𝜉𝜉 = 𝑣𝑣/Δ0 (decay)• Fermi wavelength 𝜆𝜆𝐹𝐹 = 2𝜋𝜋/𝑘𝑘𝐹𝐹 (oscillations)
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Local density of states (LDOS)
STM measurement
Spin-averaged LDOS• Oscillation for large doping
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Local density of states (LDOS)
STM measurement
Spin-resolved LDOS• At large doping:
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Spin accumulation
Response to external magnetic field
Insensitive to external magnetic field
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Difference from Majorana zero modes
Impurity bound states Majorana zero modes
Localized at … Impurity Vortex (magnetic flux)
Locked at zero energy? No Yes
Appear in pairs? Yes, but may be degenerate. No
Oscillation of LDOS?
(spin-averaged) Yes/No (depending on 𝜇𝜇) No
(spin-resolved) Yes Yes
Energy shift under B field? Yes/No (B field direction) No
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Summary
• Differences in measureable quantities.• Clues for experimental detection of Majorana zero modes.
Impurity bound states Majorana zero modes
Localized at … Impurity Vortex (magnetic flux)
Locked at zero energy? No Yes
Appear in pairs? Yes, but may be degenerate. No
Oscillation of LDOS?
(spin-averaged) Yes/No (depending on 𝜇𝜇) No
(spin-resolved) Yes Yes
Energy shift under B field? Yes/No (B field direction) No