how do nuclei rotate?

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How do nuclei rotate? 1. The molecular picture

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How do nuclei rotate?. 1. The molecular picture. 3. 2. 1. The classical rotor. J. K. orbit. Axial rotor Classical motion of J. wobbling motion. Small E. Intermediate E. Large E. Triaxial rotor Classical motion of J. Euler angles. 5/30. Quantization. 3. Axial rotor. 2. - PowerPoint PPT Presentation

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Page 1: How do nuclei rotate?

How do nuclei rotate?

1. The molecular picture

Page 2: How do nuclei rotate?

The classical rotor

1

2

3

conserved : a.m. of valueabsolute

conserved 2

1

2

1 :energy

)( :inertia of moments

:momentumangular

axes principal 3,2,1 :locityangular ve

22

22

2,3

2,21

i

i

iii

nnnn

iii

i

JJ

JE

xxm

J

i

Page 3: How do nuclei rotate?

sphere momentumangular 22iJJ

2

1 spheroidenergy

2

i

iJE

Axial rotorClassical motion of J

21

orbit

K

J

Page 4: How do nuclei rotate?

Triaxial rotorClassical motion of J

Intermediate E Large E

Small E

wobblingmotion

Page 5: How do nuclei rotate?

Euler angles

5/30

Page 6: How do nuclei rotate?

Quantization

nspermutatio cyclic and ],[ :axes laboratory zyx JiJJ

nspermutatio cyclic and ],[ :axes fixedbody 321 JiJJ

zyxkJJ k ,, 0],[ 2

0],[ 3,2,1 0],[ 32 JJiJJ zi

)1( :numbers quantum 22 IIJMJ z

)1( :numbers quantum 223 IIJKJ

KMI ,,| :states

Page 7: How do nuclei rotate?

The molecular rotor

3NH

1

2

3 21 Axial rotor

3

23

1

23

2

2

1 JJJH

3

2

1

2)1(

2

1 KKIIE

0],[0],[0],[ 23 JHJHJH z

3

23

1

22

21

2

1 JJJH

Page 8: How do nuclei rotate?

KMI ,,| :seigenstate

function Wigner D iKIMK

iMIMK edeD )(),,(

orbitK

J

),,(8

12,,|,, :rotor ofn orientatiofor

amplitudey probabilit2/1

2

I

MKDI

KMI

Page 9: How do nuclei rotate?

Centrifugal stretching

....))1(()1( 2 IIBIAIEStiff bonds

Page 10: How do nuclei rotate?

1

2

3

OH2

Triaxial rotor

0],[2

13

3

23

2

22

1

21

JHJJJ

H

Small E

wobblingmotion

K

Kn KMIcnMI ,,|,,| ,

)2/1(2

)1(

1

nII

E W

2/1

32

3121

1

))((

I

W

10/30

Page 11: How do nuclei rotate?

.

.

Born-Oppenheimer Approximation

Electronic motion

Vibrations

Rotations eVrot410~

eVel 1~

CO

eVvib110~

Page 12: How do nuclei rotate?

rot

el

vib

Adiabatic approximation

vibRvibmm

mm

OC

OC || 2

elHHHelRV eenenn ||)(

),,()()( , rotrelnucel

rotvibel

Xx

EEEE

Page 13: How do nuclei rotate?

HCl

)1()()1(

)1()(

IBIEIE

JIIBIIE

Microwave absorptionspectrum

Page 14: How do nuclei rotate?

Band Spectrum

Page 15: How do nuclei rotate?

Indistinguishable Particles

.

.

2O

2

Upper particles Lower particles

Restriction of orientation

.2 with identical is 0

signature

2 ruleselection nI

elenuci

elenuc e )(2R

15/30

Page 16: How do nuclei rotate?

oddnI

e elenuci

elenucelenuc

211

)( 12

R

Page 17: How do nuclei rotate?

The nuclear rotor

Most nuclei have a deformed axial shape.

Unified Model (Bohr and Mottelson):

The nucleus rotates as a whole. (collective degrees of freedom)

The nucleons move independentlyinside the deformed potential (intrinsic degrees of freedom)

The nucleonic motion is much fasterthan the rotation (adiabatic approximation)

Page 18: How do nuclei rotate?

Nucleons are indistinguishable

),,(),,()( rotKrotin

rotin

x

EEE

2

)1( 2KIIEE in

The nucleus does not have an orientation degree of freedomwith respect to the symmetry axis.

03

2

K

Axial symmetryin

iKin e )(3R

K

2/1

2),,(

8

12

IMKD

I

Page 19: How do nuclei rotate?

symmetry

00

2/1

2

002

),,(8

12

rule selection signatureodd

evenI )(0

IMD

I

K R

)(2R

Page 20: How do nuclei rotate?

Dyin band medsuperdefor a from rays - 152

20/30

Page 21: How do nuclei rotate?

KKK )(2R

No signature selectionrule

Page 22: How do nuclei rotate?

2))1(()1(),( IIBIAIEKIE K

Page 23: How do nuclei rotate?

Electromagnetic Transitions

Emitted photon with multipolarity E1, E2, E2, ... or M1, M2, ...

Reduced transition probability

))((y probabilit n transitio thehas MEBET

2112221 ||),)((||);)((

2

MIMEMIIIMEBM

M

contains the information about nuclear structure.

Page 24: How do nuclei rotate?

Multipole moments of the nucleus ),)(( MEM

1),1( dipole electric rYqE vM

vv rYqE 2),2( quadrupole electric M

11

2/1

4

3),1( dipole magnetic sglgM slM

Page 25: How do nuclei rotate?

2121 ,0,0 KKKK

Reduced transition probabilities in the Unified Model

'|'

|

)''),((

)),((

rules Alaga

2221211

2221211

21

21

KIKKKI

KIKKKI

IIMEB

IIMEB

||),(||

| )),((2

2122

222121121

inKKKinK

KIKKKIIIMEB

M

|t Coefficien Gordan-Clebsh 221211 KIKKKI

Page 26: How do nuclei rotate?

20

2

2

2

45

)(

|202

|101

),2,2(

),1,1(

Q

Kgg

IKKI

IKKI

KIIKEB

KIIKMB RK

25/30

Page 27: How do nuclei rotate?

Limitations of the molecular picture

What is rotating? The nuclear surface

HCl

Nucleons are not on fixed positions.

rigid rotor

)( :inertia of moments 2,3

2,21

nnnn xxm

Page 28: How do nuclei rotate?

More like a liquid, but what kind of?

viscous

))((d

:inertia ofmoment body" rigid"

2,3

2,2rig1, nn xxm x

Ideal“irrotational flow” moment of inertia

1rig223

22

223

22

1irr )()(

)()(

RR

RR

Page 29: How do nuclei rotate?

rigid

irrotational

Page 30: How do nuclei rotate?

Breakdown of adiabatic approximation

Page 31: How do nuclei rotate?

Summary

• Molecules are the protoype of quantal rotors.• Electronic and vibrational motions are much faster than rotation.• Rotational bands consist of states with different angular momentum and the same intrinsic state

(elec., vib.).• Indistiguishability leads to restrictions in the possible values of the angular momentum.• Nuclei at low spin are are similar to molecules. The nuclear surface is rotating.• Unified model: intrinsic states correspond to the motion of nucleons in the deformed potential. • Nuclei are liquid-like. The flow pattern is dominated by quantal effects.• Microscopic theory needed for calculating them.