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Exploring EDM enhancements in quadrupole-octupole interacting boson model Alexander Volya Florida State University

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Page 1: Exploring EDM enhancements in quadrupole-octupole ...€¦ · • Physics beyond standard model. system EDM limit SM e (electron) 10-27 10-40 n (neutron) 3.0x10-26 10-32 225 Ra 1.4x10-23

Exploring EDM enhancements in quadrupole-octupole interacting

boson model

Alexander Volya Florida State University

Page 2: Exploring EDM enhancements in quadrupole-octupole ...€¦ · • Physics beyond standard model. system EDM limit SM e (electron) 10-27 10-40 n (neutron) 3.0x10-26 10-32 225 Ra 1.4x10-23

Dipole-moment and violation of P and T-symmetries

spin

spin

d dT-reversal

spin

spin

d dP-reversal

Observation of the dipole moment is an indication of parity and time-reversal violation

Limit on EDM in electron Experiment 10-27 e cmStandard model » 10-38 e cmPhysics beyond SM » 10-28 e cm

Page 3: Exploring EDM enhancements in quadrupole-octupole ...€¦ · • Physics beyond standard model. system EDM limit SM e (electron) 10-27 10-40 n (neutron) 3.0x10-26 10-32 225 Ra 1.4x10-23

Why is this interesting?

• Sensitive test of CP violation in the standard model • Baryon asymmetry in the universe. • Physics beyond standard model.

system EDM limit SM

e (electron) 10-27 10-40

n (neutron) 3.0x10-26 10-32

225Ra 1.4x10-23 10-33

199Hg 7.4x10-30 10-33

T. E. Chupp, P. Fierlinger, M. J. Ramsey-Musolf, and J. T. Singh, Electric dipole moments of atoms, molecules, nuclei, and particles, Rev. Mod. Phys. 91, 015001 (2019).

Page 4: Exploring EDM enhancements in quadrupole-octupole ...€¦ · • Physics beyond standard model. system EDM limit SM e (electron) 10-27 10-40 n (neutron) 3.0x10-26 10-32 225 Ra 1.4x10-23

Schiff Moment• The nuclear dipole moment causes

polarization of the electron cloud so that the total atomic dipole moment for point particles vanishes!

• For a finite size nucleus the screening is not complete. The net result is determined by the vector called the Schiff moment

R. A. Sen'kov, N. Auerbach, V. V. Flambaum, and V. G. Zelevinsky, Phys. Rev. A 77, 014101 (2008).

Page 5: Exploring EDM enhancements in quadrupole-octupole ...€¦ · • Physics beyond standard model. system EDM limit SM e (electron) 10-27 10-40 n (neutron) 3.0x10-26 10-32 225 Ra 1.4x10-23

PT mixing NN-interaction

O. P. Sushkov, V. V. Flambaum, and I. B. Khriplovich, Feasibility of Investigation of P-Odd and T-Odd Nuclear-Forces in Atomic and Molecular Experiments, Z. Eksp. Theor. Fiz. 87, 1521-1540 (1984).

Page 6: Exploring EDM enhancements in quadrupole-octupole ...€¦ · • Physics beyond standard model. system EDM limit SM e (electron) 10-27 10-40 n (neutron) 3.0x10-26 10-32 225 Ra 1.4x10-23

Parity conservation

PT mixing in a parity-doublet

Small parity violating interaction W

Perturbed ground state

Non-zero Schiff moment

Page 7: Exploring EDM enhancements in quadrupole-octupole ...€¦ · • Physics beyond standard model. system EDM limit SM e (electron) 10-27 10-40 n (neutron) 3.0x10-26 10-32 225 Ra 1.4x10-23

Single-particle parity-doublet

No enhancement in close-lying states!

O. P. Sushkov, V. V. Flambaum, and I. B. Khriplovich, Feasibility of Investigation of P-Odd and T-Odd Nuclear-Forces in Atomic and Molecular Experiments, Z. Eksp. Theor. Fiz. 87, 1521-1540 (1984).

Page 8: Exploring EDM enhancements in quadrupole-octupole ...€¦ · • Physics beyond standard model. system EDM limit SM e (electron) 10-27 10-40 n (neutron) 3.0x10-26 10-32 225 Ra 1.4x10-23

199Hg example

5.8 MeV

1/2+

1/2-

Page 9: Exploring EDM enhancements in quadrupole-octupole ...€¦ · • Physics beyond standard model. system EDM limit SM e (electron) 10-27 10-40 n (neutron) 3.0x10-26 10-32 225 Ra 1.4x10-23

Many-body enhancements

• Proximity of levels of opposite parity • Many-body complexity

• Chaotic dynamics • Collective dynamics (parity doublets)

• Solid state or molecular mechanisms

Page 10: Exploring EDM enhancements in quadrupole-octupole ...€¦ · • Physics beyond standard model. system EDM limit SM e (electron) 10-27 10-40 n (neutron) 3.0x10-26 10-32 225 Ra 1.4x10-23

Parity-doublet octupole shape

Strongly enhanced Schiff moment

Body-fixed frame:

Lab frame:

V. Spevak, N. Auerbach, and V. V. Flambaum, Enhanced T-odd, P-odd electromagnetic moments in reflection asymmetric nuclei, Phys. Rev. C 56, 1357--1369 (1997).

Page 11: Exploring EDM enhancements in quadrupole-octupole ...€¦ · • Physics beyond standard model. system EDM limit SM e (electron) 10-27 10-40 n (neutron) 3.0x10-26 10-32 225 Ra 1.4x10-23

The path to a large Schiff moment

• 1. The quadrupole +octupole deformation leads to large intrinsic Schiff moments [1].

• 2. The parity doublets in the reflection asymmetric nuclei are very close in energy.

• 3. Parity and time reversal violating matrix element between the members of the doublet is relatively large.

• 4. Heavy nuclei - large Z.• Candidates 223Ra, 225Ra, 223Rn, 221Fr, 223FrQuestions:• Is enhancement possible in dynamical regions of soft

shape?

[1] V. Spevak, N. Auerbach, and V. V. Flambaum Phys. Rev. C 56, 1357 - 1369 (1997)

Page 12: Exploring EDM enhancements in quadrupole-octupole ...€¦ · • Physics beyond standard model. system EDM limit SM e (electron) 10-27 10-40 n (neutron) 3.0x10-26 10-32 225 Ra 1.4x10-23

Soft octupole mode in a deformed nucleus

V. V. Flambaum and V. G. Zelevinsky, Enhancement of nuclear Schiff moments and time-reversal violation in atoms due to soft nuclear octupole vibrations, Phys. Rev. C 68, 035502 (2003).

Soft octupole

Soft dipole + octupole?

Soft dipole + soft octupole?

Vibration-rotation shape transition?

Coupling between phonons?

Page 13: Exploring EDM enhancements in quadrupole-octupole ...€¦ · • Physics beyond standard model. system EDM limit SM e (electron) 10-27 10-40 n (neutron) 3.0x10-26 10-32 225 Ra 1.4x10-23

Interacting Boson Model (IBM)

Consistent Q model

F. Iachello and A. Arima, The Interacting Boson Model (Cambridge University Press, 1987).

R. Casten (ed.) Algebraic Approaches to Nuclear Structure, Interacting Boson and Fermion Models (Harwood Academic Publishers, Switzerland, 1993).

Page 14: Exploring EDM enhancements in quadrupole-octupole ...€¦ · • Physics beyond standard model. system EDM limit SM e (electron) 10-27 10-40 n (neutron) 3.0x10-26 10-32 225 Ra 1.4x10-23

IBM shape triangle

prolateoblate

0+

2+

4+

Page 15: Exploring EDM enhancements in quadrupole-octupole ...€¦ · • Physics beyond standard model. system EDM limit SM e (electron) 10-27 10-40 n (neutron) 3.0x10-26 10-32 225 Ra 1.4x10-23

IBM: Quadrupole moment of the 2+

0+

2+

4+

Page 16: Exploring EDM enhancements in quadrupole-octupole ...€¦ · • Physics beyond standard model. system EDM limit SM e (electron) 10-27 10-40 n (neutron) 3.0x10-26 10-32 225 Ra 1.4x10-23

f-boson

Angular momentum

Schiff operator

Page 17: Exploring EDM enhancements in quadrupole-octupole ...€¦ · • Physics beyond standard model. system EDM limit SM e (electron) 10-27 10-40 n (neutron) 3.0x10-26 10-32 225 Ra 1.4x10-23

Quadrupole-octupole coupling

3-

3-

2+

Coupling between modes, three-body force?

Mueller, et.al. PRC 73, (2006) 014316 V. Zelevinsky Phys. At. Nucl. 72, 1107 (2009)

Page 18: Exploring EDM enhancements in quadrupole-octupole ...€¦ · • Physics beyond standard model. system EDM limit SM e (electron) 10-27 10-40 n (neutron) 3.0x10-26 10-32 225 Ra 1.4x10-23

Quadrupole-octupole collectivity

3-

3-

2+

Coupling between modes, three-body force?Cocks, et.al. PRL 78, 2920

Mueller, et.al. PRC 73, (2006) 014316 V. Zelevinsky Phys. At. Nucl. 72, 1107 (2009) B=0.7 MeV

Page 19: Exploring EDM enhancements in quadrupole-octupole ...€¦ · • Physics beyond standard model. system EDM limit SM e (electron) 10-27 10-40 n (neutron) 3.0x10-26 10-32 225 Ra 1.4x10-23

Quadrupole-octupole coupling

Page 20: Exploring EDM enhancements in quadrupole-octupole ...€¦ · • Physics beyond standard model. system EDM limit SM e (electron) 10-27 10-40 n (neutron) 3.0x10-26 10-32 225 Ra 1.4x10-23

Quadrupole-octupole coupling (revisited)

From Xe

Page 21: Exploring EDM enhancements in quadrupole-octupole ...€¦ · • Physics beyond standard model. system EDM limit SM e (electron) 10-27 10-40 n (neutron) 3.0x10-26 10-32 225 Ra 1.4x10-23

Schiff moment

Page 22: Exploring EDM enhancements in quadrupole-octupole ...€¦ · • Physics beyond standard model. system EDM limit SM e (electron) 10-27 10-40 n (neutron) 3.0x10-26 10-32 225 Ra 1.4x10-23

vibrational rotational

Schiff moment

Page 23: Exploring EDM enhancements in quadrupole-octupole ...€¦ · • Physics beyond standard model. system EDM limit SM e (electron) 10-27 10-40 n (neutron) 3.0x10-26 10-32 225 Ra 1.4x10-23

Prolate to oblate transition

oblate prolate

Page 24: Exploring EDM enhancements in quadrupole-octupole ...€¦ · • Physics beyond standard model. system EDM limit SM e (electron) 10-27 10-40 n (neutron) 3.0x10-26 10-32 225 Ra 1.4x10-23

Particle-core coupling

IBM s.p.

Page 25: Exploring EDM enhancements in quadrupole-octupole ...€¦ · • Physics beyond standard model. system EDM limit SM e (electron) 10-27 10-40 n (neutron) 3.0x10-26 10-32 225 Ra 1.4x10-23

Particle-core coupling

Page 26: Exploring EDM enhancements in quadrupole-octupole ...€¦ · • Physics beyond standard model. system EDM limit SM e (electron) 10-27 10-40 n (neutron) 3.0x10-26 10-32 225 Ra 1.4x10-23

Explicit PT-violation

Page 27: Exploring EDM enhancements in quadrupole-octupole ...€¦ · • Physics beyond standard model. system EDM limit SM e (electron) 10-27 10-40 n (neutron) 3.0x10-26 10-32 225 Ra 1.4x10-23

Dipole moment of excited states

0+

2+

E-field

Page 28: Exploring EDM enhancements in quadrupole-octupole ...€¦ · • Physics beyond standard model. system EDM limit SM e (electron) 10-27 10-40 n (neutron) 3.0x10-26 10-32 225 Ra 1.4x10-23

The “minimal” Shell Model Hamiltonian Two-level system with single-particle states of

opposite parity j+ and j-

Parity Mixing operator

Schiff vector

Page 29: Exploring EDM enhancements in quadrupole-octupole ...€¦ · • Physics beyond standard model. system EDM limit SM e (electron) 10-27 10-40 n (neutron) 3.0x10-26 10-32 225 Ra 1.4x10-23

Dynamics• Single-particle gap: • Pairing: P-pair operator• Quadrupole interaction: Q2 -phonon• Octupole interaction: Q3 –phonon

V. Zelevinsky, A. Volya, and N. Auerbach, Phys. Rev. C 78, 014310 (2008).

Page 30: Exploring EDM enhancements in quadrupole-octupole ...€¦ · • Physics beyond standard model. system EDM limit SM e (electron) 10-27 10-40 n (neutron) 3.0x10-26 10-32 225 Ra 1.4x10-23

Details

V. Zelevinsky, A. Volya, and N. Auerbach, Phys. Rev. C 78, 014310 (2008).

Page 31: Exploring EDM enhancements in quadrupole-octupole ...€¦ · • Physics beyond standard model. system EDM limit SM e (electron) 10-27 10-40 n (neutron) 3.0x10-26 10-32 225 Ra 1.4x10-23

Spectra of the two-level model

Page 32: Exploring EDM enhancements in quadrupole-octupole ...€¦ · • Physics beyond standard model. system EDM limit SM e (electron) 10-27 10-40 n (neutron) 3.0x10-26 10-32 225 Ra 1.4x10-23

Spectra of the two-level model

Page 33: Exploring EDM enhancements in quadrupole-octupole ...€¦ · • Physics beyond standard model. system EDM limit SM e (electron) 10-27 10-40 n (neutron) 3.0x10-26 10-32 225 Ra 1.4x10-23

Spectra of the two-level model

Page 34: Exploring EDM enhancements in quadrupole-octupole ...€¦ · • Physics beyond standard model. system EDM limit SM e (electron) 10-27 10-40 n (neutron) 3.0x10-26 10-32 225 Ra 1.4x10-23

Spectra of the two-level model

Page 35: Exploring EDM enhancements in quadrupole-octupole ...€¦ · • Physics beyond standard model. system EDM limit SM e (electron) 10-27 10-40 n (neutron) 3.0x10-26 10-32 225 Ra 1.4x10-23

Degenerate levels level interchange symmetry

•Even particle system can be classified with the additional symmetry•Odd particle system: all states are degenerate parity doublets.

Page 36: Exploring EDM enhancements in quadrupole-octupole ...€¦ · • Physics beyond standard model. system EDM limit SM e (electron) 10-27 10-40 n (neutron) 3.0x10-26 10-32 225 Ra 1.4x10-23

Degenerate levels level interchange symmetry

•Even particle system can be classified with the additional symmetry•Odd particle system: all states are degenerate parity doublets.

Page 37: Exploring EDM enhancements in quadrupole-octupole ...€¦ · • Physics beyond standard model. system EDM limit SM e (electron) 10-27 10-40 n (neutron) 3.0x10-26 10-32 225 Ra 1.4x10-23

Two-level j=17/2 model Schiff and Weak Operators G=0.2 κ3=1

Left: N=6 system•Schiff operator <2|S|3>•Excitation energy of 2+ and 3- states Right: N=7 system•Energy of the g.s. doublet 17/2+ and 17/2-

•Schiff operator <17/2+|S|17/2->•Weak Matrix element <17/2+|W|17/2->•Enhancement product

Page 38: Exploring EDM enhancements in quadrupole-octupole ...€¦ · • Physics beyond standard model. system EDM limit SM e (electron) 10-27 10-40 n (neutron) 3.0x10-26 10-32 225 Ra 1.4x10-23

Two-level j=17/2 model Schiff and Weak Operators G=0.2 κ3=1

Left: N=6 system•Schiff operator <2|S|3>•Excitation energy of 2+ and 3- states Right: N=7 system•Energy of the g.s. doublet 17/2+ and 17/2-

•Schiff operator <17/2+|S|17/2->•Weak Matrix element <17/2+|W|17/2->•Enhancement product

Page 39: Exploring EDM enhancements in quadrupole-octupole ...€¦ · • Physics beyond standard model. system EDM limit SM e (electron) 10-27 10-40 n (neutron) 3.0x10-26 10-32 225 Ra 1.4x10-23

Support:• U.S. Department of Energy DE-SC0009883. • Binational Science Foundation USA-Israel • U.S. National Science Foundation

CollaboratorsNaftali AuerbachVladimir ZelevinskyCharles White

Acknowledgments