evaluation of model performance using new …...håkan grahn1 peter tunved2 1. dispersion modelling...
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![Page 1: Evaluation of model performance using new …...Håkan Grahn1 Peter Tunved2 1. Dispersion modelling Group, CBRN Environment and protection, Swedish Defense Research Agency, FOI Sweden](https://reader034.vdocuments.us/reader034/viewer/2022050519/5fa2dddbb3212c69ad63893c/html5/thumbnails/1.jpg)
Pontus von Schoenberg1
Håkan Grahn1
Peter Tunved2
1. Dispersion modelling Group, CBRN Environment and protection, Swedish Defense Research Agency, FOI Sweden
2. Department of Environmental Science and Analytical Chemistry, ACES Stockholm University, Sweden
Evaluation of model performance using new deposition
schemes in the Random displacement Particle model
PELLO using Fukushima power plant accident data
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Content
• PELLO – dispersion model
– Radiation preparedness system in Sweden
• Improved particle dynamics
– Below cloud scavenging
– In cloud scavenging
• Comparison with Fukushima NPP accident data
• Improved model
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PELLO – Stochastic particle model
• Dispersion model for regional to global scales
• Developed at Swedish Defense Research
Institute, FOI
• Used in the Swedish radiation preparedness
system at the Swedish radiation Authority, SSM
– Run operationally at the Swedish meteorological and
Hydrological institute, SMHI
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PELLO – Stochastic particle model
• Lagrangian Random Displacement Model (RDM)
• The source is represented with model particles
• Each model particle have unique properties
– Mass or amount of Becquerel
– Size, sedimentation velocity,
– Time from release (i.e. for radioactive decay etc.)
– Each model particle represents a great number of real
particles with the same properties (or an amount of gas)
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Fukushima accident comparisonModel Measurement (JAEA 2014)
10 30 60 100 300 600 1000 3000 10000
[Deposition kBq/m2]
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PELLO - size distribution
• Each model particle are randomly given a radius
• All model particles fill up the prescribed distribution
• 1M – 100M model particles used normally
Ref: Guide to Global Aerosol Models, 1999
AIAA (American Institute for Aeronautics and Astronautics)
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PELLO – Stochastic particle model
• The weather (wind, turbulence, precipitation etc.)
controls the particle movements
– Moved with the average wind (transport)
– Random displacement step representing the turbulent
diffusion (dilution)
• NWP – Numerical Weather Prediction models are
used
• ECMWF – European Centre for Medium-Range
Weather Forecasts
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NWP – Deposition parameters
Height parameters:
CIWC, Specific Cloud Ice Water Content [kg/kg]
CLWC, Specific Cloud Liquid Water Content [kg/kg]
Ground level parameters:
LSP, Large Scale Precipitation, [m]
CP, Convective Scale Precipitation, [m]
CIWC
CLWC
Ground LSP, CP
H4
H1
H2
H3
• Cloud location is calculated
• LSP and CP is distributed in height
with aid of CIWC and CIWC Into
Height parameters:
• LSP in cloud, LSP below cloud
• CP in cloud, CP below cloud
In cloud
In cloud
Below
cloud
Below
cloud
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PELLO – Particle dynamics considered
• Dry deposition
• Wet deposition
– Height above ground
– Particle size
• Is this sufficient?
• Mechanism based wet deposition
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Residence time as a function of size for
atmospheric particles103
102
101
100
10-1
10-2
10-3
10-4
Resid
ence t
ime
(days)
101 103102 10410010-110-210-310-4
Particle diameter (µm)
107
106
105
104
103
102
101
Resid
ence t
ime
(s)
Near
tropopause
In middle
troposphere
Below ~1.5 km
NucleationCoagulationCondensationDeposition(BrownianDiffusion)
Clouds!Wet deposition
Deposition(sedimentation)
Ref: Hobbs 2000
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Wet deposition
Below-cloud
scavenging
In Cloud
scavenging
Aerosol
Cloud formation
Cloud droplet
Formation
”nucleation”
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Wet deposition – below cloud
• Washout (below
cloud scavenging)
• Current scheme
– Baklanov and
Sørensen 2001
• New scheme
– Seinfeld and
Pandis 1997
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New scheme - below cloud
Seinfeld & Pandis
• Impaction
• Interception
• Brownian diffusion
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Wet deposition – In cloud
• In cloud scavenging (rainout)– Calculate the amount of water (kg) in the cloud
• from clwc and ciwc
– Calculate the amount of rain (kg) from the cloud
– Calculate fraction of cloud that is rained out (%), FoC
• Particles– Calculate how many real radioactive particles that the model
particle represent
– Calculate the fraction of radioactive particles compared to background aerosol within the cloud (%), FoR
– Assume that all particles with diameter > 100 nm within the cloud was there to create the water droplets forming the cloud
– Number of all radioactive particles, NoR
• Assume coalesces is the only process for precipitation– Washout = FoC*FoR*NoR
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Fukushima accident comparison
• Particulate 137Cs
• Cesium assumed to attach on the surface of the
ambient aerosol – Surface distribution
• Source term from Katata et. al (2014)
– Source strength variations in time
• Compared with
– Ground deposition measurements from JAEA
– Filter measurements in Sweden
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Fukushima accident comparisonAll deposition (wet and dry)
Baklanov and Sørensen 2001 Seinfeld and Pandis 1997
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Preliminary results
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Conclusions
• Altitude dependent wet removal scheme– In cloud and below cloud scavenging
• Parameterization still needs improvement– Representation of emitted particles
• Dynamical change of emitted particles– Coagulation, condensational growth
• Particles insensitive to wet removal moves into size ranges where they act as condensation nuclei
• Include information about and interaction with background aerosol
• New ways of describing both wet removal and interaction in the dry atmosphere is required
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Thank you for your attention