cold collisions in the presence of...

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united nations educational, scientific and cultural organization national atomic energy agency the 2 international centre for theoretical physics SMR 1302- 4 WINTER SCHOOL ON LASER SPECTROSCOPY AND APPLICATIONS 19 February - 2 March 2001 COLD COLLISIONS IN THE PRESENCE OF LIGHT Vanderlei S. BAGNATO Univ. de Sao Paulo, IFSC - Center for Optical Science & Photonics SP-13560-970 Sao Carlos Brazil These are preliminary lecture notes, intended only for distribution to participants. strada costiera, I I - 34OI4trieste italy - tel.+39 04022401 I I fax +39 040224163 - [email protected] - www.ictp.trieste.it

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Page 1: COLD COLLISIONS IN THE PRESENCE OF LIGHTindico.ictp.it/event/a0111/contribution/4/material/0/0.pdf · gcneralcd from FSC collisions arc cscitrd lo Wj/j sl;ilc by a first photon from

united nationseducational, scientific

and culturalorganization

national atomicenergy agency

the2international centre for theoretical physics

SMR 1302- 4

WINTER SCHOOL ON LASER SPECTROSCOPY AND APPLICATIONS

19 February - 2 March 2001

COLD COLLISIONS IN THE PRESENCE OF LIGHT

Vanderlei S. BAGNATOUniv. de Sao Paulo, IFSC - Center for Optical Science & Photonics

SP-13560-970 Sao CarlosBrazil

These are preliminary lecture notes, intended only for distribution to participants.

strada costiera, I I - 34OI4trieste italy - tel.+39 04022401 I I fax +39 040224163 - [email protected] - www.ictp.trieste.it

Page 2: COLD COLLISIONS IN THE PRESENCE OF LIGHTindico.ictp.it/event/a0111/contribution/4/material/0/0.pdf · gcneralcd from FSC collisions arc cscitrd lo Wj/j sl;ilc by a first photon from
Page 3: COLD COLLISIONS IN THE PRESENCE OF LIGHTindico.ictp.it/event/a0111/contribution/4/material/0/0.pdf · gcneralcd from FSC collisions arc cscitrd lo Wj/j sl;ilc by a first photon from

3T-Z

re ~ l e VAS\6*-

M \

102. '

c i

s=.4-oite

>>

i s s f or) is

p

S

Louo coHi'sfawa.? oUoou

a~t aoayrWyi

l

Page 4: COLD COLLISIONS IN THE PRESENCE OF LIGHTindico.ictp.it/event/a0111/contribution/4/material/0/0.pdf · gcneralcd from FSC collisions arc cscitrd lo Wj/j sl;ilc by a first photon from

Temperature

r

1000 K

IK

lmK

I B K

\Chemistry

ConventionalAtomic Beams

\Liquid He

Velocity SelectedAtomic Beams

0.01

Dopplef CoolingOptical Traps

\Optical Molasses

\Magnetic Traps

\Evaporation

BEC

j i i i i\

100 10*

dee B r g Cp ts m v = h/X

10*lmro

or) 3-H-cxre

eJ - J—

Page 5: COLD COLLISIONS IN THE PRESENCE OF LIGHTindico.ictp.it/event/a0111/contribution/4/material/0/0.pdf · gcneralcd from FSC collisions arc cscitrd lo Wj/j sl;ilc by a first photon from

JJ -•'

Seoef ak- Stoo

600

400-

-600

\l\oA intermediate state r-otentials

30

W

0.10

0.05-

0.00-

-0.05 -

-0.10 -

-0.15 -

-0 .20 -

180

\

]

foc<fss -

y

bv

pop ^ dsd

u JC H-CCJ

"c0l

Page 6: COLD COLLISIONS IN THE PRESENCE OF LIGHTindico.ictp.it/event/a0111/contribution/4/material/0/0.pdf · gcneralcd from FSC collisions arc cscitrd lo Wj/j sl;ilc by a first photon from

Lena ^A J dbecaroe

»o i

vv

^ y

are

ci decay0elocf4v cti sf ri hok

y\ v\

I

Page 7: COLD COLLISIONS IN THE PRESENCE OF LIGHTindico.ictp.it/event/a0111/contribution/4/material/0/0.pdf · gcneralcd from FSC collisions arc cscitrd lo Wj/j sl;ilc by a first photon from

ar-s or-

gy\

a n ^ g» <^> p h \ &

C

«S>VaWs

r o<2 cf= .̂ ̂ e s Q

Page 8: COLD COLLISIONS IN THE PRESENCE OF LIGHTindico.ictp.it/event/a0111/contribution/4/material/0/0.pdf · gcneralcd from FSC collisions arc cscitrd lo Wj/j sl;ilc by a first photon from

f c e o 11< s f

V( \ vi -fi-ls

^ p

CotY) b-

4

4-aUes

fak losses,

>

or)7 p

N

o.j

^

Jt _ tp=̂ _̂ !L j j

I 2 O

J./v

Page 9: COLD COLLISIONS IN THE PRESENCE OF LIGHTindico.ictp.it/event/a0111/contribution/4/material/0/0.pdf · gcneralcd from FSC collisions arc cscitrd lo Wj/j sl;ilc by a first photon from

^

mo

u*v\ber £4. cxWvus

pressure

3T-I2

- H

cJ V7

Tc

=T *Kyi

si*h

3 -

2 -

• 96r

_ • 70r

nW/cm2 >

nW/cm2 /

• 38mW/cm2 / /*• ft 23n

• I6r

"* + lOr

nW/cm2 / /y*

nW/cm2 7 / / /

• typ.n //SZ&'trap

A0F1 • ! •

I 2

TIME (»ec)

UNIFORM DENSITY DIST.' INTRA-TRAP COLLISIONS

6AUSSIAN DENSITY DIST.INTRA-TRAP COLLISIONS

GAUSSIAN DENSITY DIST.BACKGROUND GAS COLLISIONS

~1 1 1 1 1 1 —20 40 60 80 100 120

TIME (sec)

Page 10: COLD COLLISIONS IN THE PRESENCE OF LIGHTindico.ictp.it/event/a0111/contribution/4/material/0/0.pdf · gcneralcd from FSC collisions arc cscitrd lo Wj/j sl;ilc by a first photon from

o t k <a|

Cx, A ,

-QoadvVj

Load

Nc

3q

C V)CX Y)

FIG. 26. Fluorescence-time spectrum. The abrupt drop at theinitial moment is due to a change in light intensity withoutvariation in the number of trapped atoms. From Santos et al.(1996).

x]

ioqj iJ

_LT

TIyf''

0 20 40 60 80 100 120 140 160

Intensity (mW/cm2)

SeuemL C 3H*\ -̂e

0LOCJO

/Kv

v

H-CC2

HrO

Page 11: COLD COLLISIONS IN THE PRESENCE OF LIGHTindico.ictp.it/event/a0111/contribution/4/material/0/0.pdf · gcneralcd from FSC collisions arc cscitrd lo Wj/j sl;ilc by a first photon from

•x-

JT-lc

X1

ie> a

cevr)i ela ssicoL

%+%

n

# A <o

^

/ *is ex* c ttteq

T

JT-&

Once 11\ b

p

AiF5C

4 = U5^TT^d^'B

Page 12: COLD COLLISIONS IN THE PRESENCE OF LIGHTindico.ictp.it/event/a0111/contribution/4/material/0/0.pdf · gcneralcd from FSC collisions arc cscitrd lo Wj/j sl;ilc by a first photon from

I,

c3iowe

bv pa/rp

coLII10

- 9'o 8S 7e 6

° 57 4

2 3^ 2

10

_

*~ Ja— ^ y

—7 T

0

V,«.2O,r

nf H•!# !t 1

100

INTENSITY

WVIII

m $ec""'

r - 1 " ^TI

• i i i200 300

ImWcm"2 )

2.3

1.0

i

5- 5-l i i i i i i • i i 1

- 1 0 0 0 - 6 0 0 - 6 0 0 - 4 0 0 -200

FIG. 28. Measurement of the trap loss rate constant as a func-tion of MOT light intensity. The wider range of light intensityreveals an increase in /3 with MOT intensity. Dotted, full, anddot-dash curves are theory calculations using the optical-Blochequation method of Band and Julienne (1992) with differentassumptions about the maximum escape velocity of the MOT.The curve VtK= V{1) results from a simple model in which theescape velocity is a function of the MOT intensity. Data arefrom Marcassa el al. (1993).

1.3

o.e

0.3

0 .0

(b» P«/2 H

- i . i , , , , , I ,

-1000 -B00 - 6 0 0 - 4 0 0 -200 0Wp-w, (MHz)

FIG. 29. Trap-loss spectrum in a Na MOT for cat.il>sis laserdetuned to the red from both atomic line-structure .-isympintes.From Marriicco ot „ / MOO^

Page 13: COLD COLLISIONS IN THE PRESENCE OF LIGHTindico.ictp.it/event/a0111/contribution/4/material/0/0.pdf · gcneralcd from FSC collisions arc cscitrd lo Wj/j sl;ilc by a first photon from

1 0 " 4

i.o-'N

20

It(mW/cmz)

FIG. 32. Trap-loss spectrum for two isotopes of rubidium.Right-hand branch shows trap loss due FCC and RE. Left-hand branch shows trap loss due to HCC. From Wallace el al.(1992).

1 O It

Os A

10

10 3 € 9 12

INTENSITY lmW/cm2)

. 30. Trap-loss rate constant ft as a function of MOT in-ity for Cs collisions: comparison of experiment with GPry. from Sesko et al. (1989).

-1200 - 9 0 0 - 6 0 0 - 3 0 0 0

DETUNING OF CATALYST LASER (MHz)

.„-»

io-n

"I10"

10"

10,-13

€yc\\e

- 3

0 30 60 90 120 0 30 60 90 120

10"

iri

• I

A--3.5T

i i i i

10",-10

30 60 90 12010"

" I

30 60 90 120INTENSITY (mW/cm2)

FIG. 40. Trap-loss rate constant /3 for four different detuningsand a range of intensities in the Rice group's Li MOT. Thevertical lines in each plot denote / r the calculated critical in-tensity required to recapture an atom released in the shallow-est direction. From Ritchie et al. (1995).

Page 14: COLD COLLISIONS IN THE PRESENCE OF LIGHTindico.ictp.it/event/a0111/contribution/4/material/0/0.pdf · gcneralcd from FSC collisions arc cscitrd lo Wj/j sl;ilc by a first photon from

JT-23

* X-t

*

" ^ 4Jr5 60 80 100 120 140 160 180

INTENSITY lmW/cm z )

'Bcas/LM

r f»a)

j Diode Laser(repumper)

Krypton ion laser

Dichroic mirror

to,

1—/•'

— r

= 4

= 3

= 3

= ?

Continuum

RC. ., ~

• V | / 2 -

Kryplonw,, (X =

135 MHz

160MII7.

ion laser640 nm)F' = 3

F' ~ 2[JOH mn)

F = .1

F = 2

Fig. 2. Cw dcfccljon scheme. I he pniduccd 5l\n alumsgcneralcd from FSC collisions arc cscitrd lo Wj / j sl;ilc bya first photon from a dye laser (X = 607 nm) and then ioni7t-dby a second photon (A. = 640 nm) pmvcnicnl of a Kryptonion laser.

pjg. l. Experimental setup. Rubidium is trapped in a MOTsing a Ti:sapphire laser while a dye laser is tuned to the

_p _>. 8S1/2 transition and the krypton laser ionizes atomsoUtof the 8Sj/2 state. A channeltron particle multiplier detectsthe ions.

(Joser.

0\CH\S

Page 15: COLD COLLISIONS IN THE PRESENCE OF LIGHTindico.ictp.it/event/a0111/contribution/4/material/0/0.pdf · gcneralcd from FSC collisions arc cscitrd lo Wj/j sl;ilc by a first photon from

OY).

0 500 1000

Laser Frequency (MHz)

\N e v i

i s

v uJ.P. Shaffer et a/.-. Cs radiative escape and fine structure changing collisio

100 ISO 200

INTENSITY [ mW cm'2 ]

Fig. 6. Th« ratio 0FS/0HF; for a detunin<; of A - -\AF. The scatter in tho plot givevalue. The dit.i points wor.; fit to A constant to establish lh.U 0Fs/pns = 0.58 T 0.03.

Jo A

3. u

nit

s)

kJ

1.4

1.2

1.0

0.8

0.6

0 .

0.2

0 0

-

* i

_ - —

• • • • I . I

35 40 45

Intensity (m\V/cmJ)

60.0-

50.0-

40.0-

30.0-

20.0-

10.0-

0.0-

/ •

/ T"'

• // 1

-1200 1000 -BOO -600 -400 -200 0

Catalysis laser detuning (MHz)

Fig. 3 . Additional trap loss rate due to FSC introduced by thecatalysis laser, 5pSC , as a function of catalysis laser detuning,operating below the transition 5S|/2(i'n = 3) —• 5P3/2(i r ' = 4);in the frequency range of -1200 MHz < Ac < - 5 0 MHz. Thefull line represents the theoretical prediction.

Page 16: COLD COLLISIONS IN THE PRESENCE OF LIGHTindico.ictp.it/event/a0111/contribution/4/material/0/0.pdf · gcneralcd from FSC collisions arc cscitrd lo Wj/j sl;ilc by a first photon from

Mot oV Cr

iU 4:ro p

~3^«^) \

Exciled Stale Fraction0.0-1 n.on o.i? 01

1 2 3 4

MOT Laser Intensity I (mW/mm1)

i s ooct

"tTGp2J

0 50 60 70 80 90

Page 17: COLD COLLISIONS IN THE PRESENCE OF LIGHTindico.ictp.it/event/a0111/contribution/4/material/0/0.pdf · gcneralcd from FSC collisions arc cscitrd lo Wj/j sl;ilc by a first photon from

3T-2S

20 . 40 60 80 100 120 140 160

.|fto.a

Intensity (mW/cm2)

u e crt> <

9

CVKcJ

Tra pV3 u/ fffcp

\je\octly CVe)

\M o^.

IT-

77

our arcupJ

\

10 15 20 2 25

Intensity (mW/cm)

^ How

Page 18: COLD COLLISIONS IN THE PRESENCE OF LIGHTindico.ictp.it/event/a0111/contribution/4/material/0/0.pdf · gcneralcd from FSC collisions arc cscitrd lo Wj/j sl;ilc by a first photon from

>0

1

**

l

**> i

4ooelues-

-tfoppin^ ©omoll

4 o

^ U/YI. Bonn - / ^ f •]

Page 19: COLD COLLISIONS IN THE PRESENCE OF LIGHTindico.ictp.it/event/a0111/contribution/4/material/0/0.pdf · gcneralcd from FSC collisions arc cscitrd lo Wj/j sl;ilc by a first photon from

J2I- OorJT-33

«

CI) \TO-̂ erosc( 4 revn o u r

coil/

RENEE C. NHSNIDAL AND TIIAD O. WALKKR PHYSICAL REVIEW A 62 O3O7Ol(R)

-111-

I t ) .

5 10liilinsity hnW

FIG. I. Loss rales due to ullmcold collisions as a function oftotal trap laser intensity with a deluning of A = - 1 l \ The circlesand squares indicate data taken with a magnetic-field gradient of 10and 18 G/cm, respectively. The solid lines have been included toguide the eye.

intensity (mW/cniJ)

FIG. 2. Loss rales as a function of total trap laser intensity forlarger laser detuning*, l i te -f's and circles indicate data tqken atA ~ - 1 . 5 f and - 2 ! ' , rcspcdivrly.

tvj

Page 20: COLD COLLISIONS IN THE PRESENCE OF LIGHTindico.ictp.it/event/a0111/contribution/4/material/0/0.pdf · gcneralcd from FSC collisions arc cscitrd lo Wj/j sl;ilc by a first photon from

op

as

4 or

40 80'

Intensity (mW/cm3)

ao.

d o.-wpi

R(a0)

JT-i

u) fib I d

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1.0

0.8

0.2

0.0

R («„)

"3e

T>fonumced

•50 mW/cm

•20 mW/cm2

• 5 mW/cm

1 mW/cm2

0.22 mW/cm2

0.08 mW/cm2

0.03 mW/cm'

6000

ft-

Ve

2,0x10*

« 1,5x10"

L0X105

5,0x104

0,0

R(a0)

ITo /not

50 mW/cm

20 mW/cm2

5 mW/cm2

1 mW/cm2

0.22 mW/cm2

0.08 mW/cm

0.03 mW/cm2

4000 6000

u j

i v\ j

Page 22: COLD COLLISIONS IN THE PRESENCE OF LIGHTindico.ictp.it/event/a0111/contribution/4/material/0/0.pdf · gcneralcd from FSC collisions arc cscitrd lo Wj/j sl;ilc by a first photon from

al beloauror (5

c

0 10 20 30 40 50 60 70

Intensity (mW/cm2) *

can pi cute// or?<&7 /m<rf

-H

c

•903

T-31

Fig.1: G.D. Telles et s/., Alternative Interpretation for theMagneto Optical Trap Losses at Low Light Intensil

V)

c

c5

1 -

10 20 30 40 50 60Intensity (mW/cm )

i 1 » i •> i

0.1 10

Intensity; (mW/cm )

O

Page 23: COLD COLLISIONS IN THE PRESENCE OF LIGHTindico.ictp.it/event/a0111/contribution/4/material/0/0.pdf · gcneralcd from FSC collisions arc cscitrd lo Wj/j sl;ilc by a first photon from

to

f

J

SpeciesLi

NaK

Rb

Cs

-3.5

-1-7

-1

-1

Icxp(mW/cm2)28

580

3

4

inKxKmW/cm2)25

7.981

2.5

1.4

ReferenceN.W.M. Rilchie e( aJ PRA 51, R890

(95)S.R. Muniz et al, PRA 55, 4407 (97)L.G. Marcassa et al, accepted PRA

(00)CD. Wallace et al, PRL 69, 897

(92)Seskoetal, PRL 63, 961(89)

.0,0 0,2 0, 6

intensity (mW/cm )

4 -

~ 3 -

CO. 2 -

1 -

0,8

dB/dx = 10 G/cm;A = -2rFFT smooth: 4ptsA = - i ,5rFFT smooth: 4pts

7

Intensity (mW/cm )

c l<CJ

Page 24: COLD COLLISIONS IN THE PRESENCE OF LIGHTindico.ictp.it/event/a0111/contribution/4/material/0/0.pdf · gcneralcd from FSC collisions arc cscitrd lo Wj/j sl;ilc by a first photon from

Svs+sre^i s

5.63 .6 3 .1

( oL ftB)

- R .

Qvccj

V

c/)eoses : *-^<^ ^ctn'ies Civideos

l f

Page 25: COLD COLLISIONS IN THE PRESENCE OF LIGHTindico.ictp.it/event/a0111/contribution/4/material/0/0.pdf · gcneralcd from FSC collisions arc cscitrd lo Wj/j sl;ilc by a first photon from

Sodium loss rate (10"" cmVs) 8.ib

Iri>c

7t> 3c

P

ID

0c

1

Trap loss rates (ft? cm3/s)

c

12K

C L

CL

Ci

"3

CPCD

q-Zf.

.0

Trap loss rates (10~12cm3/s)

CD

•r

08

Page 26: COLD COLLISIONS IN THE PRESENCE OF LIGHTindico.ictp.it/event/a0111/contribution/4/material/0/0.pdf · gcneralcd from FSC collisions arc cscitrd lo Wj/j sl;ilc by a first photon from

Doubl

V(R)

K(4P3;2)-Rb(5P3/2)

(b)

K(4S,,2)-Rb(5P3/2)

K(4S1/2)-^Rb(5S1/2)

esc Internuclear separation, R

i ^O

3.0

0.0K-Rb ( x 1 0 )

70 80 90 100 110

Potassium trap laser intensity (mW/cm )

Page 27: COLD COLLISIONS IN THE PRESENCE OF LIGHTindico.ictp.it/event/a0111/contribution/4/material/0/0.pdf · gcneralcd from FSC collisions arc cscitrd lo Wj/j sl;ilc by a first photon from

Heteronuclear trap loss rate, p' (10~12 cmVs) HTrap loss rates, p/p1 (10" cm /s)

3=

o

3

3-3

f9*

to

P(cm3/sec)

CD ^

IS JSCD £

$

Page 28: COLD COLLISIONS IN THE PRESENCE OF LIGHTindico.ictp.it/event/a0111/contribution/4/material/0/0.pdf · gcneralcd from FSC collisions arc cscitrd lo Wj/j sl;ilc by a first photon from

MS S c

- r50

— A— p expeiimonlal— |) Modulo GP: Rb/Rb*

—T—1»' experimental— \Y Modelo GP: Rb/Cs"

T100 150 200

Intensidade (mW/cin1)

250

50 60 70

Inten9idade (mW/cm2)

100 110

1 -

• - |» oxporlmental

|l Modelo GP: Hb/Ub"• A— p" eKpeiliTienlnl

- — H 1 Modelo GP.Rb/Cn'

.1- 1 1 • 1 • 1 « 1 • 1 • 1 ' 10 50 100 150 200 250 300 350

Intenaldade (mW/cm1)

50 60 70 80 90 100 110

Intensidade (mW/cm3)

Page 29: COLD COLLISIONS IN THE PRESENCE OF LIGHTindico.ictp.it/event/a0111/contribution/4/material/0/0.pdf · gcneralcd from FSC collisions arc cscitrd lo Wj/j sl;ilc by a first photon from

13. 1 0 -

(D4-*

CD

</)

O

CL

£is"o

100

Probe laser detuning (MHz)

"Vo

TELLES, G.D.

/vvo

U(R)

10-

1 -

0.1 -

Sodium

• I* I

trap laser iniensuy.

« 140mW/cm2

= 70 mW/cm2

= 40 mW/cm2

1000

Probe laser detuning (MHz)

Theoretical modef

1E-12-

1E-13-

1E-14-

Re

i!c1'c1'c

Internuclear

= 40 mw/cm2

= 70 mw/cm2

= 140 mw/cm2

separation, RDouble excited <3P model

—i 1 1—i—i—i—i—

|A|, detuning (MHz)

Page 30: COLD COLLISIONS IN THE PRESENCE OF LIGHTindico.ictp.it/event/a0111/contribution/4/material/0/0.pdf · gcneralcd from FSC collisions arc cscitrd lo Wj/j sl;ilc by a first photon from

Sod

y- Los,. fKy*. J i , IO6-2C

+ K ^ T f t . A, R2S-43

^v?T. ?

?kvs.!W, A

C

S.-\e\\es