behaviour of rn - max-planck-institut für kernphysik · long and short exposition time ssp in n2...

30
1 Marcin Marcin Wójcik Wójcik , Nikodem , Nikodem Frodyma Frodyma , Krzysztof , Krzysztof Pelczar Pelczar GERDA GERDA Collaboration Meeting Collaboration Meeting Jagellonian Jagellonian University University , Kraków 2008 , Kraków 2008 Behaviour of Behaviour of 222 222 Rn Rn and its daughters and its daughters in liquid nitrogen in liquid nitrogen

Upload: others

Post on 11-Jun-2020

1 views

Category:

Documents


0 download

TRANSCRIPT

Page 1: Behaviour of Rn - Max-Planck-Institut für Kernphysik · Long and short exposition time SSP in N2 gas -----SSP in liquid N2-----Behaviour of Rn 222 and its daughters in LN 2, GERDA

1

Marcin Marcin WójcikWójcik , Nikodem , Nikodem FrodymaFrodyma , Krzysztof , Krzysztof PelczarPelczar

GERDA GERDA Collaboration MeetingCollaboration Meeting

JagellonianJagellonian UniversityUniversity, Kraków 2008, Kraków 2008

Behaviour ofBehaviour of

222222RnRnand its daughtersand its daughters

in liquid nitrogenin liquid nitrogen

Page 2: Behaviour of Rn - Max-Planck-Institut für Kernphysik · Long and short exposition time SSP in N2 gas -----SSP in liquid N2-----Behaviour of Rn 222 and its daughters in LN 2, GERDA

2

�� RnRn as aas a timetime--dependentdependent background source inbackground source in e.g.e.g. thethe

GERDAGERDA experimentexperiment

�� Rn and RnRn and Rn--daughters location in cryostat with liquid gasdaughters location in cryostat with liquid gas

�� Rn partition between liquid and gas phaseRn partition between liquid and gas phase

�� Behaviour of Rn and its daughtersBehaviour of Rn and its daughters in in LNLN22 in electric fieldin electric field

Problems and Questions Problems and Questions

Behaviour of Rn222 and its daughters in LN2, GERDA Collaboration Meeting, Kraków 2008

M. Wójcik, N. Frodyma, K. Pelczar, Jagiellonian Univers ity, Kraków

Page 3: Behaviour of Rn - Max-Planck-Institut für Kernphysik · Long and short exposition time SSP in N2 gas -----SSP in liquid N2-----Behaviour of Rn 222 and its daughters in LN 2, GERDA

3

222222RnRn and itsand its daughtersdaughters

222Rn

226Ra

218Po

214Pb

214Bi

214Po

210Pb

α

α

ββ

α α

210Bi

210Po

206Pb

α

β

T1/2 = 1622 y

E = 4.8 MeV

T1/2 = 3.8 dE = 5.5 MeV

T1/2 = 3.1 m

E = 6.0 MeV

T1/2 = 26.8 m

Em = 0.7 MeV

β T1/2 = 19.8 m

Em = 1.5 MeV

T1/2 = 164 µsE = 7.7 MeV

T1/2 = 22.3 yEm = 0.06 MeV

T1/2 = 5.0 dEm = 1.2 MeV

T1/2 = 138.4 d

E = 5.3 MeV

Stable

Behaviour of Rn222 and its daughters in LN2, GERDA Collaboration Meeting, Kraków 2008

M. Wójcik, N. Frodyma, K. Pelczar, Jagiellonian Univers ity, Kraków

Page 4: Behaviour of Rn - Max-Planck-Institut für Kernphysik · Long and short exposition time SSP in N2 gas -----SSP in liquid N2-----Behaviour of Rn 222 and its daughters in LN 2, GERDA

4Behaviour of Rn222 and its daughters in LN2, GERDA Collaboration Meeting, Kraków 2008

M. Wójcik, N. Frodyma, K. Pelczar, Jagiellonian Univers ity, Kraków

222222RnRn and itsand its daughtersdaughters

222Rn 218Po 214Pb 214Bi 214Po α βα β

+ +_ _ + + ?

in gas:

in liquid:

++

Page 5: Behaviour of Rn - Max-Planck-Institut für Kernphysik · Long and short exposition time SSP in N2 gas -----SSP in liquid N2-----Behaviour of Rn 222 and its daughters in LN 2, GERDA

5

GERDAGERDA –– model model of the detectorof the detector

Behaviour of Rn222 and its daughters in LN2, GERDA Collaboration Meeting, Kraków 2008

M. Wójcik, N. Frodyma, K. Pelczar, Jagiellonian Univers ity, Kraków

Page 6: Behaviour of Rn - Max-Planck-Institut für Kernphysik · Long and short exposition time SSP in N2 gas -----SSP in liquid N2-----Behaviour of Rn 222 and its daughters in LN 2, GERDA

6

RnRn dissolving in LNdissolving in LN22

Behaviour of Rn222 and its daughters in LN2, GERDA Collaboration Meeting, Kraków 2008

M. Wójcik, N. Frodyma, K. Pelczar, Jagiellonian Univers ity, Kraków

Page 7: Behaviour of Rn - Max-Planck-Institut für Kernphysik · Long and short exposition time SSP in N2 gas -----SSP in liquid N2-----Behaviour of Rn 222 and its daughters in LN 2, GERDA

7

„„Free evaporationFree evaporation”” of of LLNN22 with with RnRn

Behaviour of Rn222 and its daughters in LN2, GERDA Collaboration Meeting, Kraków 2008

M. Wójcik, N. Frodyma, K. Pelczar, Jagiellonian Univers ity, Kraków

Page 8: Behaviour of Rn - Max-Planck-Institut für Kernphysik · Long and short exposition time SSP in N2 gas -----SSP in liquid N2-----Behaviour of Rn 222 and its daughters in LN 2, GERDA

8

„„Free evaporationFree evaporation”” of of LLNN22 with with RnRn

Behaviour of Rn222 and its daughters in LN2, GERDA Collaboration Meeting, Kraków 2008

M. Wójcik, N. Frodyma, K. Pelczar, Jagiellonian Univers ity, Kraków

Page 9: Behaviour of Rn - Max-Planck-Institut für Kernphysik · Long and short exposition time SSP in N2 gas -----SSP in liquid N2-----Behaviour of Rn 222 and its daughters in LN 2, GERDA

9

„„Free evaporationFree evaporation”” of of LLNN22 with with RnRn

Behaviour of Rn222 and its daughters in LN2, GERDA Collaboration Meeting, Kraków 2008

M. Wójcik, N. Frodyma, K. Pelczar, Jagiellonian Univers ity, Kraków

Page 10: Behaviour of Rn - Max-Planck-Institut für Kernphysik · Long and short exposition time SSP in N2 gas -----SSP in liquid N2-----Behaviour of Rn 222 and its daughters in LN 2, GERDA

10

„„Free evaporationFree evaporation”” of of LLNN22 with with RnRn

Behaviour of Rn222 and its daughters in LN2, GERDA Collaboration Meeting, Kraków 2008

M. Wójcik, N. Frodyma, K. Pelczar, Jagiellonian Univers ity, Kraków

0

2

4

6

8

10

12

14

16

0:00:00 6:00:00 12:00:00 18:00:00 24:00:00time [hh:mm:ss]

coun

t rat

e[c

ount

s/m

in]

Page 11: Behaviour of Rn - Max-Planck-Institut für Kernphysik · Long and short exposition time SSP in N2 gas -----SSP in liquid N2-----Behaviour of Rn 222 and its daughters in LN 2, GERDA

11

„„Free evaporationFree evaporation”” of of LLNN22 with with RnRn

Behaviour of Rn222 and its daughters in LN2, GERDA Collaboration Meeting, Kraków 2008

M. Wójcik, N. Frodyma, K. Pelczar, Jagiellonian Univers ity, Kraków

0

2

4

6

8

10

12

14

16

144:00:00 150:00:00 156:00:00 162:00:00 168:00:00

time [hh:mm:ss]

coun

t rat

e[c

ount

s/m

in]

Fit parameters (y = ax +b)a = 7.6E-5 ± 2.3E-5 cpm/mb = 1.565 ± 0.025 cpm

Page 12: Behaviour of Rn - Max-Planck-Institut für Kernphysik · Long and short exposition time SSP in N2 gas -----SSP in liquid N2-----Behaviour of Rn 222 and its daughters in LN 2, GERDA

12

„„Free evaporationFree evaporation”” of of LLNN22 with with RnRn

Behaviour of Rn222 and its daughters in LN2, GERDA Collaboration Meeting, Kraków 2008

M. Wójcik, N. Frodyma, K. Pelczar, Jagiellonian Univers ity, Kraków

0,1

1

10

100

1000

303:30:00 309:30:00 315:30:00 321:30:00 327:30:00time [hh:mm:ss]

coun

t rat

e[c

ount

s/m

]

Page 13: Behaviour of Rn - Max-Planck-Institut für Kernphysik · Long and short exposition time SSP in N2 gas -----SSP in liquid N2-----Behaviour of Rn 222 and its daughters in LN 2, GERDA

13

RnRn count rate growth after LNcount rate growth after LN22 evaporationevaporation

Behaviour of Rn222 and its daughters in LN2, GERDA Collaboration Meeting, Kraków 2008

M. Wójcik, N. Frodyma, K. Pelczar, Jagiellonian Univers ity, Kraków

Page 14: Behaviour of Rn - Max-Planck-Institut für Kernphysik · Long and short exposition time SSP in N2 gas -----SSP in liquid N2-----Behaviour of Rn 222 and its daughters in LN 2, GERDA

14

Measurement of the Measurement of the RnRn concentration in LNconcentration in LN22

Behaviour of Rn222 and its daughters in LN2, GERDA Collaboration Meeting, Kraków 2008

M. Wójcik, N. Frodyma, K. Pelczar, Jagiellonian Univers ity, Kraków

Page 15: Behaviour of Rn - Max-Planck-Institut für Kernphysik · Long and short exposition time SSP in N2 gas -----SSP in liquid N2-----Behaviour of Rn 222 and its daughters in LN 2, GERDA

15

RnRn concentration in liquid and gaseous nitrogenconcentration in liquid and gaseous nitrogen

Behaviour of Rn222 and its daughters in LN2, GERDA Collaboration Meeting, Kraków 2008

M. Wójcik, N. Frodyma, K. Pelczar, Jagiellonian Univers ity, Kraków

Page 16: Behaviour of Rn - Max-Planck-Institut für Kernphysik · Long and short exposition time SSP in N2 gas -----SSP in liquid N2-----Behaviour of Rn 222 and its daughters in LN 2, GERDA

16

Variable heating inside the DewarVariable heating inside the Dewar

Behaviour of Rn222 and its daughters in LN2, GERDA Collaboration Meeting, Kraków 2008

M. Wójcik, N. Frodyma, K. Pelczar, Jagiellonian Univers ity, Kraków

Page 17: Behaviour of Rn - Max-Planck-Institut für Kernphysik · Long and short exposition time SSP in N2 gas -----SSP in liquid N2-----Behaviour of Rn 222 and its daughters in LN 2, GERDA

17Behaviour of Rn222 and its daughters in LN2, GERDA Collaboration Meeting, Kraków 2008

M. Wójcik, N. Frodyma, K. Pelczar, Jagiellonian Univers ity, Kraków

Variable heating inside the DewarVariable heating inside the Dewar

Page 18: Behaviour of Rn - Max-Planck-Institut für Kernphysik · Long and short exposition time SSP in N2 gas -----SSP in liquid N2-----Behaviour of Rn 222 and its daughters in LN 2, GERDA

18

RnRn--daughters depositiondaughters deposition on on stainless steel platesstainless steel plates(SSP)(SSP) andand alfaalfa --spectrometryspectrometry

SSP placed in different posotions

and under different conditions:

� Liquid nitrogen

� Gaseous nitrogen

� High voltage applied

� Long and short exposition time

SSP in N2 gas ----------------

SSP in liquid N2 ----------------

Behaviour of Rn222 and its daughters in LN2, GERDA Collaboration Meeting, Kraków 2008

M. Wójcik, N. Frodyma, K. Pelczar, Jagiellonian Univers ity, Kraków

Page 19: Behaviour of Rn - Max-Planck-Institut für Kernphysik · Long and short exposition time SSP in N2 gas -----SSP in liquid N2-----Behaviour of Rn 222 and its daughters in LN 2, GERDA

19

alfaalfa--spectrometerspectrometer

Behaviour of Rn222 and its daughters in LN2, GERDA Collaboration Meeting, Kraków 2008

M. Wójcik, N. Frodyma, K. Pelczar, Jagiellonian Univers ity, Kraków

Page 20: Behaviour of Rn - Max-Planck-Institut für Kernphysik · Long and short exposition time SSP in N2 gas -----SSP in liquid N2-----Behaviour of Rn 222 and its daughters in LN 2, GERDA

20Behaviour of Rn222 and its daughters in LN2, GERDA Collaboration Meeting, Kraków 2008

M. Wójcik, N. Frodyma, K. Pelczar, Jagiellonian Univers ity, Kraków

214Po

218Po

T1/2 = 186 s

T1/2 = 1188 s

alfaalfa--spectrometerspectrometer

Page 21: Behaviour of Rn - Max-Planck-Institut für Kernphysik · Long and short exposition time SSP in N2 gas -----SSP in liquid N2-----Behaviour of Rn 222 and its daughters in LN 2, GERDA

21

High voltage influenceHigh voltage influence on counts of on counts of 214214PPoo

Behaviour of Rn222 and its daughters in LN2, GERDA Collaboration Meeting, Kraków 2008

M. Wójcik, N. Frodyma, K. Pelczar, Jagiellonian Univers ity, Kraków

Page 22: Behaviour of Rn - Max-Planck-Institut für Kernphysik · Long and short exposition time SSP in N2 gas -----SSP in liquid N2-----Behaviour of Rn 222 and its daughters in LN 2, GERDA

22

Counts of Counts of 214214Po and Po and 218218Po Po vsvs applied voltageapplied voltagennegativeegative voltagevoltage

Behaviour of Rn222 and its daughters in LN2, GERDA Collaboration Meeting, Kraków 2008

M. Wójcik, N. Frodyma, K. Pelczar, Jagiellonian Univers ity, Kraków

LN2

Page 23: Behaviour of Rn - Max-Planck-Institut für Kernphysik · Long and short exposition time SSP in N2 gas -----SSP in liquid N2-----Behaviour of Rn 222 and its daughters in LN 2, GERDA

23

Counts of Counts of 214214Po and Po and 218218Po Po vsvs applied voltageapplied voltageppositiveositive voltagevoltage

LN2

Behaviour of Rn222 and its daughters in LN2, GERDA Collaboration Meeting, Kraków 2008

M. Wójcik, N. Frodyma, K. Pelczar, Jagiellonian Univers ity, Kraków

Page 24: Behaviour of Rn - Max-Planck-Institut für Kernphysik · Long and short exposition time SSP in N2 gas -----SSP in liquid N2-----Behaviour of Rn 222 and its daughters in LN 2, GERDA

24

RnRn (and daughters) concentration(and daughters) concentrationgrowth in time (with growth in time (with ––2000V applied)2000V applied)

LN2

Behaviour of Rn222 and its daughters in LN2, GERDA Collaboration Meeting, Kraków 2008

M. Wójcik, N. Frodyma, K. Pelczar, Jagiellonian Univers ity, Kraków

Page 25: Behaviour of Rn - Max-Planck-Institut für Kernphysik · Long and short exposition time SSP in N2 gas -----SSP in liquid N2-----Behaviour of Rn 222 and its daughters in LN 2, GERDA

25

Plans Plans for further measurementsfor further measurements

� Germanium plates

� Liquid argon

� Dynamics simulations

Behaviour of Rn222 and its daughters in LN2, GERDA Collaboration Meeting, Kraków 2008

M. Wójcik, N. Frodyma, K. Pelczar, Jagiellonian Univers ity, Kraków

Page 26: Behaviour of Rn - Max-Planck-Institut für Kernphysik · Long and short exposition time SSP in N2 gas -----SSP in liquid N2-----Behaviour of Rn 222 and its daughters in LN 2, GERDA

26

Preliminary conclusionsPreliminary conclusions

Behaviour of Rn222 and its daughters in LN2, GERDA Collaboration Meeting, Kraków 2008

M. Wójcik, N. Frodyma, K. Pelczar, Jagiellonian Univers ity, Kraków

� Large part of Rn is dissolved in LN2

� The Rn concentration in evaporated gas is lower than in liquid gas and depends on the evaporating rate (heating power)

� High voltage forces Rn to concentrate around the SSP� The polarity of HV is not meaningless� The concentration of Rn depends on time of SSP exposure

Open questionsOpen questions

� Mechanism of Rn and Rn – daughters concentration

Page 27: Behaviour of Rn - Max-Planck-Institut für Kernphysik · Long and short exposition time SSP in N2 gas -----SSP in liquid N2-----Behaviour of Rn 222 and its daughters in LN 2, GERDA

27

Marcin Marcin WójcikWójcik , Nikodem , Nikodem FrodymaFrodyma , Krzysztof , Krzysztof PelczarPelczar

GERDA GERDA Collaboration MeetingCollaboration Meeting

Jagellonian UniversityJagellonian University, Kraków 2008, Kraków 2008

Behaviour ofBehaviour of

222222RnRnand its daughtersand its daughters

in liquid nitrogenin liquid nitrogen

Page 28: Behaviour of Rn - Max-Planck-Institut für Kernphysik · Long and short exposition time SSP in N2 gas -----SSP in liquid N2-----Behaviour of Rn 222 and its daughters in LN 2, GERDA

28

Temperature inside the Temperature inside the dewardewar(top and bottom, after N(top and bottom, after N22 evaporation)evaporation)

Behaviour of Rn222 and its daughters in LN2, GERDA Collaboration Meeting, Kraków 2008

M. Wójcik, N. Frodyma, K. Pelczar, Jagiellonian Univers ity, Kraków

Page 29: Behaviour of Rn - Max-Planck-Institut für Kernphysik · Long and short exposition time SSP in N2 gas -----SSP in liquid N2-----Behaviour of Rn 222 and its daughters in LN 2, GERDA

29

Temperature difference between top and bottom Temperature difference between top and bottom wall wall of the of the dewardewar (after nitrogen evaporated)(after nitrogen evaporated)

Behaviour of Rn222 and its daughters in LN2, GERDA Collaboration Meeting, Kraków 2008

M. Wójcik, N. Frodyma, K. Pelczar, Jagiellonian Univers ity, Kraków

Page 30: Behaviour of Rn - Max-Planck-Institut für Kernphysik · Long and short exposition time SSP in N2 gas -----SSP in liquid N2-----Behaviour of Rn 222 and its daughters in LN 2, GERDA

30

Rn concentrationRn concentration growthgrowth (after LN2 evaporated)(after LN2 evaporated)with constant flow ratewith constant flow rate

Behaviour of Rn222 and its daughters in LN2, GERDA Collaboration Meeting, Kraków 2008

M. Wójcik, N. Frodyma, K. Pelczar, Jagiellonian Univers ity, Kraków