an optical tweezer array of ultracold molecules · 2019. 12. 6. · microsoft powerpoint -...

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An Optical Tweezer Array of Ultracold Molecules Original Researchers: Loïc Anderegg1,2, Lawrence W. Cheuk1,2, Yicheng Bao1,2, Sean Burchesky1,2, Wolfgang Ketterle2,3, Kang‐Kuen Ni1,2,4, John M. Doyle1,2 Presented by: Garrett Williams, Danielle Woods, Drew Wild, and Yiqi, Xie Anderegg, Loïc et al. “An Optical Tweezer Array of Ultracold Molecules.” Science 365.6458 (2019): 1156–1158. Crossref. Web.

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Page 1: An Optical Tweezer Array of Ultracold Molecules · 2019. 12. 6. · Microsoft PowerPoint - Team10_final.pptx Author: slcooper Created Date: 12/6/2019 10:00:12 AM

An Optical Tweezer Array of UltracoldMolecules

Original Researchers: Loïc Anderegg1,2, Lawrence W. Cheuk1,2, Yicheng Bao1,2, Sean Burchesky1,2, Wolfgang Ketterle2,3, Kang‐Kuen Ni1,2,4, John M. Doyle1,2

Presented by: Garrett Williams, Danielle Woods, Drew Wild, and Yiqi, Xie

Anderegg, Loïc et al. “An Optical Tweezer Array of Ultracold Molecules.” Science 365.6458 (2019): 1156–1158. Crossref. Web.

Page 2: An Optical Tweezer Array of Ultracold Molecules · 2019. 12. 6. · Microsoft PowerPoint - Team10_final.pptx Author: slcooper Created Date: 12/6/2019 10:00:12 AM

Outline

• Motivation• Overview• Theoretical Background

• Doppler Cooling• Magneto‐optical traps

• Summary of Results• Critical analysis and citation summary

Page 3: An Optical Tweezer Array of Ultracold Molecules · 2019. 12. 6. · Microsoft PowerPoint - Team10_final.pptx Author: slcooper Created Date: 12/6/2019 10:00:12 AM

Motivation

• Quantum Computation• Polar molecules can potentially provide stable qubits with ~5s coherence

• Improved Quantum Simulation • Dipole forces can introduce long range interactions

• Sensitive Detectors and Ultracold Chemistry

Page 4: An Optical Tweezer Array of Ultracold Molecules · 2019. 12. 6. · Microsoft PowerPoint - Team10_final.pptx Author: slcooper Created Date: 12/6/2019 10:00:12 AM

Overview

● This paper builds on previous experiments that created arrays of ultracold atoms

● A gas of CaF is trapped and cooled to the ultracold regime <1mK and further trapped by optical tweezers to form a 1‐D array

Page 5: An Optical Tweezer Array of Ultracold Molecules · 2019. 12. 6. · Microsoft PowerPoint - Team10_final.pptx Author: slcooper Created Date: 12/6/2019 10:00:12 AM

A Two‐Level System

ωo

E1

E2

Two‐Level system

Gaseous state of atoms

Orientation ‐ Making an Optical Array  ‐‐‐ Comparison with Other Work   ‐‐ Citation Analysis 

Page 6: An Optical Tweezer Array of Ultracold Molecules · 2019. 12. 6. · Microsoft PowerPoint - Team10_final.pptx Author: slcooper Created Date: 12/6/2019 10:00:12 AM

“Sub‐levels” in the two‐level system

ωo

E1

E2

ωo

ωo+ dω

ωo+ dω

Absorptio

n

Frequency

Orientation ‐ Making an Optical Array  ‐‐‐ Comparison with Other Work   ‐‐ Citation Analysis 

Page 7: An Optical Tweezer Array of Ultracold Molecules · 2019. 12. 6. · Microsoft PowerPoint - Team10_final.pptx Author: slcooper Created Date: 12/6/2019 10:00:12 AM

Spectral Linewidth

Frequency

Absorptio

n

ωo

ωo

E1

E2

ωo

E1

E2

ωo

ωo+ dω

ωo+ dω

Absorptio

nFrequency

Spectral Linewidth

Orientation ‐ Making an Optical Array  ‐‐‐ Comparison with Other Work   ‐‐ Citation Analysis 

Page 8: An Optical Tweezer Array of Ultracold Molecules · 2019. 12. 6. · Microsoft PowerPoint - Team10_final.pptx Author: slcooper Created Date: 12/6/2019 10:00:12 AM

The Doppler Effect

ω

Orientation ‐ Making an Optical Array  ‐‐‐ Comparison with Other Work   ‐‐ Citation Analysis 

Page 9: An Optical Tweezer Array of Ultracold Molecules · 2019. 12. 6. · Microsoft PowerPoint - Team10_final.pptx Author: slcooper Created Date: 12/6/2019 10:00:12 AM

p0

Blue‐shifting laser wavelength

*Where         <

p   ‐ p0 = p 

Orientation ‐ Making an Optical Array  ‐‐‐ Comparison with Other Work   ‐‐ Citation Analysis 

Page 10: An Optical Tweezer Array of Ultracold Molecules · 2019. 12. 6. · Microsoft PowerPoint - Team10_final.pptx Author: slcooper Created Date: 12/6/2019 10:00:12 AM

p0

Detuned‐light can slow atoms/molecule

p < p0

p   ‐ p0 = p 

p   ‐ p0 = p 

Orientation ‐ Making an Optical Array  ‐‐‐ Comparison with Other Work   ‐‐ Citation Analysis 

*Kinetic Energy is proportional to temperature

Page 11: An Optical Tweezer Array of Ultracold Molecules · 2019. 12. 6. · Microsoft PowerPoint - Team10_final.pptx Author: slcooper Created Date: 12/6/2019 10:00:12 AM

z

xy

Optical Molasses

Orientation ‐ Making an Optical Array  ‐‐‐ Comparison with Other Work   ‐‐ Citation Analysis 

Page 12: An Optical Tweezer Array of Ultracold Molecules · 2019. 12. 6. · Microsoft PowerPoint - Team10_final.pptx Author: slcooper Created Date: 12/6/2019 10:00:12 AM

z

xy

Optical Molasses

Orientation ‐ Making an Optical Array  ‐‐‐ Comparison with Other Work   ‐‐ Citation Analysis 

*Good but not good enough!

Page 13: An Optical Tweezer Array of Ultracold Molecules · 2019. 12. 6. · Microsoft PowerPoint - Team10_final.pptx Author: slcooper Created Date: 12/6/2019 10:00:12 AM

Magneto‐Optical Trap (MOT)

B

I

Helmholtz

‐ I

Anti‐Helmholtz

‐ I

I

Orientation ‐ Making an Optical Array  ‐‐‐ Comparison with Other Work   ‐‐ Citation Analysis 

Page 14: An Optical Tweezer Array of Ultracold Molecules · 2019. 12. 6. · Microsoft PowerPoint - Team10_final.pptx Author: slcooper Created Date: 12/6/2019 10:00:12 AM

m = 0 m = ‐1m = 1

xx

*Imparting units of angular momentum on the system

Lz = m

MOT Beams use circularly polarized light

Orientation ‐ Making an Optical Array  ‐‐‐ Comparison with Other Work   ‐‐ Citation Analysis 

Page 15: An Optical Tweezer Array of Ultracold Molecules · 2019. 12. 6. · Microsoft PowerPoint - Team10_final.pptx Author: slcooper Created Date: 12/6/2019 10:00:12 AM

MOT Beams use circularly polarized light

Orientation ‐ Making an Optical Array  ‐‐‐ Comparison with Other Work   ‐‐ Citation Analysis 

Page 16: An Optical Tweezer Array of Ultracold Molecules · 2019. 12. 6. · Microsoft PowerPoint - Team10_final.pptx Author: slcooper Created Date: 12/6/2019 10:00:12 AM

MOT Beams use circularly polarized light

Orientation ‐ Making an Optical Array  ‐‐‐ Comparison with Other Work   ‐‐ Citation Analysis 

Page 17: An Optical Tweezer Array of Ultracold Molecules · 2019. 12. 6. · Microsoft PowerPoint - Team10_final.pptx Author: slcooper Created Date: 12/6/2019 10:00:12 AM

Treating an atom/molecule as two‐level system

ωR

Orientation ‐ Making an Optical Array  ‐‐‐ Comparison with Other Work   ‐‐ Citation Analysis 

Δm = ‐1,0,1Δl = ‐1,1ΔF = ‐1,1

Page 18: An Optical Tweezer Array of Ultracold Molecules · 2019. 12. 6. · Microsoft PowerPoint - Team10_final.pptx Author: slcooper Created Date: 12/6/2019 10:00:12 AM

Optical Tweezers

Orientation ‐ Making an Optical Array  ‐‐‐ Comparison with Other Work   ‐‐ Citation Analysis 

Page 19: An Optical Tweezer Array of Ultracold Molecules · 2019. 12. 6. · Microsoft PowerPoint - Team10_final.pptx Author: slcooper Created Date: 12/6/2019 10:00:12 AM

Optical Array – probabilistic recapture

Orientation  ‐ Making an Optical Array  ‐‐‐ Comparison with Other Work   ‐‐ Citation Analysis 

Page 20: An Optical Tweezer Array of Ultracold Molecules · 2019. 12. 6. · Microsoft PowerPoint - Team10_final.pptx Author: slcooper Created Date: 12/6/2019 10:00:12 AM

Optical Array – dynamic traps

Orientation  ‐ Making an Optical Array  ‐‐‐ Comparison with Other Work   ‐‐ Citation Analysis 

Page 21: An Optical Tweezer Array of Ultracold Molecules · 2019. 12. 6. · Microsoft PowerPoint - Team10_final.pptx Author: slcooper Created Date: 12/6/2019 10:00:12 AM

Experiment Apparatus and Summary of Results

I. Optical trap from red‐detuned beam

II. MOT magnetic field coilsIII. Window that prevents optical 

lattice formationIV. Microscope objectiveV. Dichroic mirrorVI. Camera pathVII. Optical tweezer traps

Orientation  ‐‐ Making an Optical Array  ‐‐‐ Comparison with Other Work   ‐‐ Citation Analysis 

Page 22: An Optical Tweezer Array of Ultracold Molecules · 2019. 12. 6. · Microsoft PowerPoint - Team10_final.pptx Author: slcooper Created Date: 12/6/2019 10:00:12 AM

Discussion of Results 

• “Fully control and detect individual molecules”• “Creation and detection of an array of ultracold calcium minifluoride(CaF) molecules trapped in optical tweezers”

• Verified occupancy was just one molecule• Their light‐collision rates are similar to that measured for rubidium atoms in optical tweezers. 

• Dipole moment also similar: suggests that molecular systems should have similar collision rates to those of atomic systems. 

Orientation  ‐‐ Making an Optical Array  ‐‐‐ Comparison with Other Work   ‐‐ Citation Analysis 

Page 23: An Optical Tweezer Array of Ultracold Molecules · 2019. 12. 6. · Microsoft PowerPoint - Team10_final.pptx Author: slcooper Created Date: 12/6/2019 10:00:12 AM

Comparison with previous works

• This work:• Loading of diatomic molecules into optical tweezer arrays

Orientation  ‐‐ Making an Optical Array  ‐‐‐ Comparison with Other Work ‐‐ Citation Analysis 

Page 24: An Optical Tweezer Array of Ultracold Molecules · 2019. 12. 6. · Microsoft PowerPoint - Team10_final.pptx Author: slcooper Created Date: 12/6/2019 10:00:12 AM

Comparison with previous works

• This work:• Loading of diatomic molecules into optical tweezer arrays

• Previous works:

Orientation  ‐‐ Making an Optical Array  ‐‐‐ Comparison with Other Work ‐‐ Citation Analysis 

Page 25: An Optical Tweezer Array of Ultracold Molecules · 2019. 12. 6. · Microsoft PowerPoint - Team10_final.pptx Author: slcooper Created Date: 12/6/2019 10:00:12 AM

Comparison with previous works

• This work:• Loading of diatomic molecules into optical tweezer arrays

• Previous works:• Optical trapping of diatomic [1] and polyatomic [2] molecules

Orientation  ‐‐ Making an Optical Array  ‐‐‐ Comparison with Other Work ‐‐ Citation Analysis 

Page 26: An Optical Tweezer Array of Ultracold Molecules · 2019. 12. 6. · Microsoft PowerPoint - Team10_final.pptx Author: slcooper Created Date: 12/6/2019 10:00:12 AM

Comparison with previous works

• This work:• Loading of diatomic molecules into optical tweezer arrays

• Previous works:• Optical trapping of diatomic [1] and polyatomic [2] molecules• Controlled molecular synthesis using optical tweezers [3]

Orientation  ‐‐ Making an Optical Array  ‐‐‐ Comparison with Other Work ‐‐ Citation Analysis 

Page 27: An Optical Tweezer Array of Ultracold Molecules · 2019. 12. 6. · Microsoft PowerPoint - Team10_final.pptx Author: slcooper Created Date: 12/6/2019 10:00:12 AM

Comparison with previous works

• This work:• Loading of diatomic molecules into optical tweezer arrays

• Previous works:• Optical trapping of diatomic [1] and polyatomic [2] molecules• Controlled molecular synthesis using optical tweezers [3]• Deterministic loading of atoms into 1D [4] and 2D [5] optical tweezer arrays

[1] Blackmore et al (2018), doi: 10.1088/2058‐9565/aaee35[2] Kozyryev & Hutzler (2017), doi: 10.1103/PhysRevLett.119.133002[3] Liu et al (2018), doi: 10.1126/science.aar7797[4] Endres et al (2016), doi: 10.1126/science.aah3752[5] Barredo et al (2016), doi: 10.1126/science.aah3778

Orientation  ‐‐ Making an Optical Array  ‐‐‐ Comparison with Other Work ‐‐ Citation Analysis 

Page 28: An Optical Tweezer Array of Ultracold Molecules · 2019. 12. 6. · Microsoft PowerPoint - Team10_final.pptx Author: slcooper Created Date: 12/6/2019 10:00:12 AM

Citation Report

• Low citation number since it’s new

• 2 citations according to Web of Science:• Making perfectly controlled arrays of molecules at rest

(a Science perspective)• A scalable quantum computing platform using symmetric‐top molecules

(recent progress of the same team)

Orientation  ‐ Making an Optical Array  ‐‐‐ Comparison with Other Work   ‐‐ Citation Analysis 

Page 29: An Optical Tweezer Array of Ultracold Molecules · 2019. 12. 6. · Microsoft PowerPoint - Team10_final.pptx Author: slcooper Created Date: 12/6/2019 10:00:12 AM

Broader Impacts

• Quantum computation• Searching• Solving linear equations• Cryptography

Orientation  ‐ Making an Optical Array  ‐‐‐ Comparison with Other Work   ‐‐ Citation Analysis

Page 30: An Optical Tweezer Array of Ultracold Molecules · 2019. 12. 6. · Microsoft PowerPoint - Team10_final.pptx Author: slcooper Created Date: 12/6/2019 10:00:12 AM

Broader Impacts

• Quantum computation• Searching• Solving linear equations• Cryptography

• Quantum simulation• Solving a wide range of many‐body physics problems

Orientation  ‐ Making an Optical Array  ‐‐‐ Comparison with Other Work   ‐‐ Citation Analysis

Page 31: An Optical Tweezer Array of Ultracold Molecules · 2019. 12. 6. · Microsoft PowerPoint - Team10_final.pptx Author: slcooper Created Date: 12/6/2019 10:00:12 AM

Broader Impacts

• Quantum computation• Searching• Solving linear equations• Cryptography

• Quantum simulation• Solving a wide range of many‐body physics problems

• Ultracold chemistry• Brand new methodology for chemistry research• Controlled reaction at molecular level

Orientation  ‐ Making an Optical Array  ‐‐‐ Comparison with Other Work   ‐‐ Citation Analysis

Page 32: An Optical Tweezer Array of Ultracold Molecules · 2019. 12. 6. · Microsoft PowerPoint - Team10_final.pptx Author: slcooper Created Date: 12/6/2019 10:00:12 AM

Conclusion

• Realized novel technique

• Demonstrated valid scientific approach

• Paved the way to future research involving ultracold molecules

• Raised broad interest in topics such as molecular dynamics, quantum information, quantum simulation, etc

• Not targeted for general audience

Orientation  ‐ Making an Optical Array  ‐‐‐ Comparison with Other Work   ‐‐ Citation Analysis 

Page 33: An Optical Tweezer Array of Ultracold Molecules · 2019. 12. 6. · Microsoft PowerPoint - Team10_final.pptx Author: slcooper Created Date: 12/6/2019 10:00:12 AM

Thanks you for Listening!